Oligogermanes containing only electron-withdrawing substituents: Synthesis and properties
K V Zaitsev
1, 2
,
Kevin Lam
3
,
Zhaisan Zhanabil
3, 4
,
Yerlan Melsuly Suleimen
3
,
Yerlan Suleimen
4
,
Anastasia V Kharcheva
1, 2
,
В. А. Тафеенко
1
,
Viktor A. Tafeenko
2
,
Yuri F. Oprunenko
1, 2
,
Oleg Kh Poleshchuk
5, 6
,
Elmira Kh. Lermontova
7, 8
,
Publication type: Journal Article
Publication date: 2016-12-22
scimago Q2
wos Q1
SJR: 0.676
CiteScore: 5.1
Impact factor: 2.9
ISSN: 02767333, 15206041
Organic Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
A series of germanes Ar3GeX, containing electron-withdrawing substituents [Ar = p-FC6H4, 1a–d, 1a (X = Cl), 1b (X = Br), 1c (X = H), 1d (X = NMe2); p-F3CC6H4, 2a–d, 2a (X = Cl), 2b (X = Br), 2c (X = H), 2d (X = NMe2)], was synthesized and used to prepare symmetrical digermanes Ar3Ge–GeAr3, (p-FC6H4)3GeGe(C6H4F-p)3 (3), and (p-F3CC6H4)3GeGe(C6H4CF3-p)3 (4) and trigermane [(p-F3CC6H4)3Ge]2Ge(C6F5)2 (5) by hydrogermolysis reaction. The properties of all compounds were investigated by multinuclear NMR and for oligogermanes by UV/vis and fluorescence spectroscopy, as well as by electrochemical methods. In addition, the molecular structures of 1a, 1b, 2b, 2c, and 3–5 were studied by X-ray diffraction analysis. Compound 5 showed a significantly shifted UV/visible absorption to the red field in comparison with previously described derivatives.
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Total citations:
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Citations from 2024:
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Zaitsev K. V. et al. Oligogermanes containing only electron-withdrawing substituents: Synthesis and properties // Organometallics. 2016. Vol. 36. No. 2. pp. 298-309.
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Zaitsev K. V., Lam K., Zhanabil Z., Suleimen Y. M., Suleimen Y., Kharcheva A. V., Тафеенко В. А., Tafeenko V. A., Oprunenko Y. F., Poleshchuk O. Kh., Lermontova E. K., Churakov A. V. Oligogermanes containing only electron-withdrawing substituents: Synthesis and properties // Organometallics. 2016. Vol. 36. No. 2. pp. 298-309.
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TY - JOUR
DO - 10.1021/acs.organomet.6b00767
UR - https://pubs.acs.org/doi/10.1021/acs.organomet.6b00767
TI - Oligogermanes containing only electron-withdrawing substituents: Synthesis and properties
T2 - Organometallics
AU - Zaitsev, K V
AU - Lam, Kevin
AU - Zhanabil, Zhaisan
AU - Suleimen, Yerlan Melsuly
AU - Suleimen, Yerlan
AU - Kharcheva, Anastasia V
AU - Тафеенко, В. А.
AU - Tafeenko, Viktor A.
AU - Oprunenko, Yuri F.
AU - Poleshchuk, Oleg Kh
AU - Lermontova, Elmira Kh.
AU - Churakov, Andrei V.
PY - 2016
DA - 2016/12/22
PB - American Chemical Society (ACS)
SP - 298-309
IS - 2
VL - 36
SN - 0276-7333
SN - 1520-6041
ER -
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BibTex (up to 50 authors)
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@article{2016_Zaitsev,
author = {K V Zaitsev and Kevin Lam and Zhaisan Zhanabil and Yerlan Melsuly Suleimen and Yerlan Suleimen and Anastasia V Kharcheva and В. А. Тафеенко and Viktor A. Tafeenko and Yuri F. Oprunenko and Oleg Kh Poleshchuk and Elmira Kh. Lermontova and Andrei V. Churakov},
title = {Oligogermanes containing only electron-withdrawing substituents: Synthesis and properties},
journal = {Organometallics},
year = {2016},
volume = {36},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://pubs.acs.org/doi/10.1021/acs.organomet.6b00767},
number = {2},
pages = {298--309},
doi = {10.1021/acs.organomet.6b00767}
}
Cite this
MLA
Copy
Zaitsev, K. V., et al. “Oligogermanes containing only electron-withdrawing substituents: Synthesis and properties.” Organometallics, vol. 36, no. 2, Dec. 2016, pp. 298-309. https://pubs.acs.org/doi/10.1021/acs.organomet.6b00767.