IrIII/AuI and RhIII/AuI Heterobimetallic Complexes as Catalysts for the Coupling of Nitrobenzene and Benzylic Alcohol
Publication type: Journal Article
Publication date: 2018-10-31
scimago Q2
wos Q1
SJR: 0.676
CiteScore: 5.1
Impact factor: 2.9
ISSN: 02767333, 15206041
Organic Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Two simple bisimidazolium salts derived from m- or p-bisimidazolebenzenes have been used as ligand precursors for the preparation of a series of heterobimetallic RhIII/AuI and IrIII/AuI complexes. All complexes have been fully characterized, and the molecular structures of selected derivatives have been determined by X-ray diffraction studies. These analyses showed that, regardless of the ligand used, the direct coordination environment of the metals is composed of identical donors (MIII: CNHC, Cbenzene, η5-Cp*, and I–; AuI: CNHC and I–) and is rather similar in the heterobimetallic complexes. The catalytic activity of the heterobimetallic complexes in the coupling of nitrobenzene with benzylic alcohol has been investigated. In all cases, the performance observed for the heterobimetallic complexes was superior to that shown by mixtures of homometallic MIII/AuI complexes, suggesting a cooperative effect between the two metal centers. In addition and in spite of the similarity of the donor groups of the two...
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45
Total citations:
45
Citations from 2024:
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(15%)
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GOST
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Böhmer M. et al. IrIII/AuI and RhIII/AuI Heterobimetallic Complexes as Catalysts for the Coupling of Nitrobenzene and Benzylic Alcohol // Organometallics. 2018. Vol. 37. No. 21. pp. 4092-4099.
GOST all authors (up to 50)
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Böhmer M., Kampert F., Tan T. T. Y., Guisado Barrios G., Peris E., Hahn F. E. IrIII/AuI and RhIII/AuI Heterobimetallic Complexes as Catalysts for the Coupling of Nitrobenzene and Benzylic Alcohol // Organometallics. 2018. Vol. 37. No. 21. pp. 4092-4099.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.organomet.8b00642
UR - https://doi.org/10.1021/acs.organomet.8b00642
TI - IrIII/AuI and RhIII/AuI Heterobimetallic Complexes as Catalysts for the Coupling of Nitrobenzene and Benzylic Alcohol
T2 - Organometallics
AU - Böhmer, Maximilian
AU - Kampert, Florian
AU - Tan, Tristan Tsai Yuan
AU - Guisado Barrios, Gregorio
AU - Peris, Eduardo
AU - Hahn, F. Ekkehardt
PY - 2018
DA - 2018/10/31
PB - American Chemical Society (ACS)
SP - 4092-4099
IS - 21
VL - 37
SN - 0276-7333
SN - 1520-6041
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Böhmer,
author = {Maximilian Böhmer and Florian Kampert and Tristan Tsai Yuan Tan and Gregorio Guisado Barrios and Eduardo Peris and F. Ekkehardt Hahn},
title = {IrIII/AuI and RhIII/AuI Heterobimetallic Complexes as Catalysts for the Coupling of Nitrobenzene and Benzylic Alcohol},
journal = {Organometallics},
year = {2018},
volume = {37},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/acs.organomet.8b00642},
number = {21},
pages = {4092--4099},
doi = {10.1021/acs.organomet.8b00642}
}
Cite this
MLA
Copy
Böhmer, Maximilian, et al. “IrIII/AuI and RhIII/AuI Heterobimetallic Complexes as Catalysts for the Coupling of Nitrobenzene and Benzylic Alcohol.” Organometallics, vol. 37, no. 21, Oct. 2018, pp. 4092-4099. https://doi.org/10.1021/acs.organomet.8b00642.
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