volume 25 issue 12 pages 2145-2150

Diverse Synthesis of Alkenylsilanes via Pd-Catalyzed Alkenyl C–H Silylation

Zi-Hang Ye 1, 2
Fei Hu Gou 2
Fei-Hu Gou 2
Yichen Wu 2
Chuan Ying Li 1
Chuanying Li 1
Peng Wang 2, 3, 4
Publication typeJournal Article
Publication date2023-03-15
scimago Q1
wos Q1
SJR1.235
CiteScore8.7
Impact factor5.0
ISSN15237060, 15237052
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
Here, we disclose a general approach for the diverse synthesis of alkenylsilanes in a highly efficient, stereoselective, and atom-economic manner by leveraging the palladium-catalyzed disilylation reaction of 2-bromostyrene derivatives with hexamethyldisilane, which is suitable for the preparation of a series of disubstituted, trisubstituted, and tetrasubstituted alkenylsilanes. Furthermore, the resulting tetrasubstituted alkenylsilanes could be readily transformed into the corresponding diarylated benzosiloles, which have been proven to be a potential AIE material and a fluorene material.
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GOST Copy
Ye Z. et al. Diverse Synthesis of Alkenylsilanes via Pd-Catalyzed Alkenyl C–H Silylation // Organic Letters. 2023. Vol. 25. No. 12. pp. 2145-2150.
GOST all authors (up to 50) Copy
Ye Z., Gou F. H., Gou F., Wu Y., Li C. Y., Li C., Wang P. Diverse Synthesis of Alkenylsilanes via Pd-Catalyzed Alkenyl C–H Silylation // Organic Letters. 2023. Vol. 25. No. 12. pp. 2145-2150.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1021/acs.orglett.3c00633
UR - https://pubs.acs.org/doi/10.1021/acs.orglett.3c00633
TI - Diverse Synthesis of Alkenylsilanes via Pd-Catalyzed Alkenyl C–H Silylation
T2 - Organic Letters
AU - Ye, Zi-Hang
AU - Gou, Fei Hu
AU - Gou, Fei-Hu
AU - Wu, Yichen
AU - Li, Chuan Ying
AU - Li, Chuanying
AU - Wang, Peng
PY - 2023
DA - 2023/03/15
PB - American Chemical Society (ACS)
SP - 2145-2150
IS - 12
VL - 25
PMID - 36921249
SN - 1523-7060
SN - 1523-7052
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2023_Ye,
author = {Zi-Hang Ye and Fei Hu Gou and Fei-Hu Gou and Yichen Wu and Chuan Ying Li and Chuanying Li and Peng Wang},
title = {Diverse Synthesis of Alkenylsilanes via Pd-Catalyzed Alkenyl C–H Silylation},
journal = {Organic Letters},
year = {2023},
volume = {25},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://pubs.acs.org/doi/10.1021/acs.orglett.3c00633},
number = {12},
pages = {2145--2150},
doi = {10.1021/acs.orglett.3c00633}
}
MLA
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MLA Copy
Ye, Zi-Hang, et al. “Diverse Synthesis of Alkenylsilanes via Pd-Catalyzed Alkenyl C–H Silylation.” Organic Letters, vol. 25, no. 12, Mar. 2023, pp. 2145-2150. https://pubs.acs.org/doi/10.1021/acs.orglett.3c00633.
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