Organic Letters

, том 18 , издание 10 , страницы 2427-2430

A Versatile, Traceless C–H Activation-Based Approach for the Synthesis of Heterocycles

Тип публикации: Journal Article

Дата публикации: 2016-05-02

American Chemical Society (ACS)

Organic Letters

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SJR: 1.007

CiteScore: 7.7

Impact factor: 4.7

ISSN: 15237060, 15237052

DOI: 10.1021/acs.orglett.6b00949

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PubMed ID: 27135982

Organic Chemistry

Biochemistry

Physical and Theoretical Chemistry

Краткое описание

A versatile, traceless C-H activation-based approach for the synthesis of diversified heterocycles is reported. Rh(III)-catalyzed, N-amino-directed C-H alkenylation generates either olefination products or indoles (in situ annulation) in an atom- and step-economic manner at room temperature. The remarkable reactivity endowed by this directing group enables scale-up of the reaction to a 10 g scale at a very low catalyst loading (0.01 mol %/0.1 mol %). Ex situ annulation of olefination product provides entry into an array of heterocycles.

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Zhou S. et al. A Versatile, Traceless C–H Activation-Based Approach for the Synthesis of Heterocycles // Organic Letters. 2016. Vol. 18. No. 10. pp. 2427-2430.

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Zhou S., Wang J., Zhang F., Song C., Zhu J. A Versatile, Traceless C–H Activation-Based Approach for the Synthesis of Heterocycles // Organic Letters. 2016. Vol. 18. No. 10. pp. 2427-2430.

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TY - JOUR

DO - 10.1021/acs.orglett.6b00949

UR - https://doi.org/10.1021/acs.orglett.6b00949

TI - A Versatile, Traceless C–H Activation-Based Approach for the Synthesis of Heterocycles

T2 - Organic Letters

AU - Zhou, Shuguang

AU - Wang, Jinhu

AU - Zhang, Feifei

AU - Song, Chao

AU - Zhu, Jin

PY - 2016

DA - 2016/05/02

PB - American Chemical Society (ACS)

SP - 2427-2430

IS - 10

VL - 18

PMID - 27135982

SN - 1523-7060

SN - 1523-7052

ER -

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@article{2016_Zhou,

author = {Shuguang Zhou and Jinhu Wang and Feifei Zhang and Chao Song and Jin Zhu},

title = {A Versatile, Traceless C–H Activation-Based Approach for the Synthesis of Heterocycles},

journal = {Organic Letters},

year = {2016},

volume = {18},

publisher = {American Chemical Society (ACS)},

month = {may},

url = {https://doi.org/10.1021/acs.orglett.6b00949},

number = {10},

pages = {2427--2430},

doi = {10.1021/acs.orglett.6b00949}

}

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Zhou, Shuguang, et al. “A Versatile, Traceless C–H Activation-Based Approach for the Synthesis of Heterocycles.” Organic Letters, vol. 18, no. 10, May. 2016, pp. 2427-2430. https://doi.org/10.1021/acs.orglett.6b00949.

Издатель

American Chemical Society (ACS)

Журнал

Organic Letters

SCImago Q1

Tоп 10% SCImago

WOS Q1

БС1