Chemodivergent Couplings of N-Arylureas and Methyleneoxetanones via Rh(III)-Catalyzed and Solvent-Controlled C–H Activation
Publication type: Journal Article
Publication date: 2019-05-24
scimago Q1
wos Q1
SJR: 1.235
CiteScore: 8.7
Impact factor: 5.0
ISSN: 15237060, 15237052
PubMed ID:
31124685
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
The efficient couplings of diverse N-arylureas and methyleneoxetanones have been realized via Rh(III)-catalyzed and solvent-controlled chemoselective C-H functionalization, which involved the tunable β-H elimination and β-O elimination processes, thereby giving divergent access to quinolin-2(1 H)-ones and ortho-allylated N-arylureas with broad substrate compatibility and good functional group tolerance. the divergent synthetic utilities of the transformations have also been exemplified by subsequently tandem C-H allylation, unsymmetrical C-H functionalization, alternative reaction mode, as well as removal of the carbamoyl group.
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Total citations:
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Citations from 2024:
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GOST
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Zhu G. et al. Chemodivergent Couplings of N-Arylureas and Methyleneoxetanones via Rh(III)-Catalyzed and Solvent-Controlled C–H Activation // Organic Letters. 2019. Vol. 21. No. 11. pp. 4143-4147.
GOST all authors (up to 50)
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Zhu G., Shi W., Gao H., Zhou Z., Song H., Yi W. Chemodivergent Couplings of N-Arylureas and Methyleneoxetanones via Rh(III)-Catalyzed and Solvent-Controlled C–H Activation // Organic Letters. 2019. Vol. 21. No. 11. pp. 4143-4147.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.orglett.9b01333
UR - https://doi.org/10.1021/acs.orglett.9b01333
TI - Chemodivergent Couplings of N-Arylureas and Methyleneoxetanones via Rh(III)-Catalyzed and Solvent-Controlled C–H Activation
T2 - Organic Letters
AU - Zhu, Guoxun
AU - Shi, Wendi
AU - Gao, Hui
AU - Zhou, Zhi
AU - Song, Huacan
AU - Yi, Wei
PY - 2019
DA - 2019/05/24
PB - American Chemical Society (ACS)
SP - 4143-4147
IS - 11
VL - 21
PMID - 31124685
SN - 1523-7060
SN - 1523-7052
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2019_Zhu,
author = {Guoxun Zhu and Wendi Shi and Hui Gao and Zhi Zhou and Huacan Song and Wei Yi},
title = {Chemodivergent Couplings of N-Arylureas and Methyleneoxetanones via Rh(III)-Catalyzed and Solvent-Controlled C–H Activation},
journal = {Organic Letters},
year = {2019},
volume = {21},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/acs.orglett.9b01333},
number = {11},
pages = {4143--4147},
doi = {10.1021/acs.orglett.9b01333}
}
Cite this
MLA
Copy
Zhu, Guoxun, et al. “Chemodivergent Couplings of N-Arylureas and Methyleneoxetanones via Rh(III)-Catalyzed and Solvent-Controlled C–H Activation.” Organic Letters, vol. 21, no. 11, May. 2019, pp. 4143-4147. https://doi.org/10.1021/acs.orglett.9b01333.