Synthesis of Functionalized Vinylsilanes via Metal-Free Dehydrogenative Silylation of Enamides
Xi Hao Chang
1
,
Zi Lu Wang
1
,
Meng Zhao
1
,
Chao Yang
1
,
Jie Jun Li
1
,
Wei-Wei Ma
1
,
Yunhe Xu
1
Publication type: Journal Article
Publication date: 2020-01-30
scimago Q1
wos Q1
SJR: 1.235
CiteScore: 8.7
Impact factor: 5.0
ISSN: 15237060, 15237052
PubMed ID:
31999462
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
A novel method of metal-free dehydrogenative silylation of enamides has been developed. The desired functionalized vinylsilane products were obtained in moderate to good yield and with high stereoselectivities. This protocol displays good tolerance of various functionalities. Furthermore, the high chemoselectivity of this reaction enables us to introduce different unsaturated C-C moieties to the products. The ease of further derivatization of the products to other useful compounds also demonstrates the highly synthetic utility of the current methodology.
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Metrics
33
Total citations:
33
Citations from 2024:
10
(30.3%)
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MLA
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GOST
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Chang X. H. et al. Synthesis of Functionalized Vinylsilanes via Metal-Free Dehydrogenative Silylation of Enamides // Organic Letters. 2020. Vol. 22. No. 4. pp. 1326-1330.
GOST all authors (up to 50)
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Chang X. H., Wang Z. L., Zhao M., Yang C., Li J. J., Ma W., Xu Y. Synthesis of Functionalized Vinylsilanes via Metal-Free Dehydrogenative Silylation of Enamides // Organic Letters. 2020. Vol. 22. No. 4. pp. 1326-1330.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acs.orglett.9b04645
UR - https://doi.org/10.1021/acs.orglett.9b04645
TI - Synthesis of Functionalized Vinylsilanes via Metal-Free Dehydrogenative Silylation of Enamides
T2 - Organic Letters
AU - Chang, Xi Hao
AU - Wang, Zi Lu
AU - Zhao, Meng
AU - Yang, Chao
AU - Li, Jie Jun
AU - Ma, Wei-Wei
AU - Xu, Yunhe
PY - 2020
DA - 2020/01/30
PB - American Chemical Society (ACS)
SP - 1326-1330
IS - 4
VL - 22
PMID - 31999462
SN - 1523-7060
SN - 1523-7052
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2020_Chang,
author = {Xi Hao Chang and Zi Lu Wang and Meng Zhao and Chao Yang and Jie Jun Li and Wei-Wei Ma and Yunhe Xu},
title = {Synthesis of Functionalized Vinylsilanes via Metal-Free Dehydrogenative Silylation of Enamides},
journal = {Organic Letters},
year = {2020},
volume = {22},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acs.orglett.9b04645},
number = {4},
pages = {1326--1330},
doi = {10.1021/acs.orglett.9b04645}
}
Cite this
MLA
Copy
Chang, Xi Hao, et al. “Synthesis of Functionalized Vinylsilanes via Metal-Free Dehydrogenative Silylation of Enamides.” Organic Letters, vol. 22, no. 4, Jan. 2020, pp. 1326-1330. https://doi.org/10.1021/acs.orglett.9b04645.