ACS Applied Electronic Materials, volume 3, issue 7, pages 3106-3113

A Rapidly Stabilizing Water-Gated Field-Effect Transistor Based on Printed Single-Walled Carbon Nanotubes for Biosensing Applications

Publication typeJournal Article
Publication date2021-07-01
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor4.7
ISSN26376113, 26376113
Materials Chemistry
Electronic, Optical and Magnetic Materials
Electrochemistry
Abstract
Biosensors are expected to revolutionize disease management through provision of low-cost diagnostic platforms for molecular and pathogenic detection with high sensitivity and short response time. In this context, there has been an ever-increasing interest in using electrolyte-gated field-effect transistors (EG-FETs) for biosensing applications owing to their expanding potential of being employed for label-free detection of a broad range of biomarkers with high selectivity and sensitivity while operating at sub-volt working potentials. Although organic semiconductors have been widely utilized as the channel in EG-FETs, primarily due to their compatibility with cost-effective low-temperature solution-processing fabrication techniques, alternative carbon-based platforms have the potential to provide similar advantages with improved electronic performances. Here, we propose the use of inkjet-printed polymer-wrapped monochiral single-walled carbon nanotubes (s-SWCNTs) for the channel of EG-FETs in an aqueous environment. In particular, we show that our EG-CNTFETs require only an hour of stabilization before producing a highly stable response suitable for biosensing, with a drastic time reduction with respect to the most exploited organic semiconductor for biosensors. As a proof-of-principle, we successfully employed our water-gated device to detect the well-known biotin–streptavidin binding event.

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Molazemhosseini A. et al. A Rapidly Stabilizing Water-Gated Field-Effect Transistor Based on Printed Single-Walled Carbon Nanotubes for Biosensing Applications // ACS Applied Electronic Materials. 2021. Vol. 3. No. 7. pp. 3106-3113.
GOST all authors (up to 50) Copy
Molazemhosseini A., Viola F. A., Berger F., Zorn N. F., Zaumseil J., Caironi M. A Rapidly Stabilizing Water-Gated Field-Effect Transistor Based on Printed Single-Walled Carbon Nanotubes for Biosensing Applications // ACS Applied Electronic Materials. 2021. Vol. 3. No. 7. pp. 3106-3113.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1021/acsaelm.1c00332
UR - https://doi.org/10.1021/acsaelm.1c00332
TI - A Rapidly Stabilizing Water-Gated Field-Effect Transistor Based on Printed Single-Walled Carbon Nanotubes for Biosensing Applications
T2 - ACS Applied Electronic Materials
AU - Molazemhosseini, Alireza
AU - Zorn, Nicolas Frederic
AU - Zaumseil, Jana
AU - Caironi, Mario
AU - Viola, Fabrizio Antonio
AU - Berger, Felix
PY - 2021
DA - 2021/07/01 00:00:00
PB - American Chemical Society (ACS)
SP - 3106-3113
IS - 7
VL - 3
SN - 2637-6113
SN - 2637-6113
ER -
BibTex |
Cite this
BibTex Copy
@article{2021_Molazemhosseini,
author = {Alireza Molazemhosseini and Nicolas Frederic Zorn and Jana Zaumseil and Mario Caironi and Fabrizio Antonio Viola and Felix Berger},
title = {A Rapidly Stabilizing Water-Gated Field-Effect Transistor Based on Printed Single-Walled Carbon Nanotubes for Biosensing Applications},
journal = {ACS Applied Electronic Materials},
year = {2021},
volume = {3},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/acsaelm.1c00332},
number = {7},
pages = {3106--3113},
doi = {10.1021/acsaelm.1c00332}
}
MLA
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MLA Copy
Molazemhosseini, Alireza, et al. “A Rapidly Stabilizing Water-Gated Field-Effect Transistor Based on Printed Single-Walled Carbon Nanotubes for Biosensing Applications.” ACS Applied Electronic Materials, vol. 3, no. 7, Jul. 2021, pp. 3106-3113. https://doi.org/10.1021/acsaelm.1c00332.
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