Stable and Reproducible 2D/3D Formamidinium–Lead–Iodide Perovskite Solar Cells
Abhishek Thote
1
,
Il Jeon
1
,
Jinwook Lee
2
,
Seungju Seo
1
,
Hao-Sheng Lin
1
,
Yang Yang
2
,
Hirofumi Daiguji
1
,
Shigeo Maruyama
1, 3
,
Publication type: Journal Article
Publication date: 2019-03-08
scimago Q1
wos Q2
SJR: 1.378
CiteScore: 10.2
Impact factor: 5.5
ISSN: 25740962
Materials Chemistry
Electrochemistry
Electrical and Electronic Engineering
Energy Engineering and Power Technology
Chemical Engineering (miscellaneous)
Abstract
2D perovskite-stabilized FACsPbI3 (FA = formamidinium) perovskite solar cells were fabricated in both normal-type and inverted-type architectures. While the normal-type devices exhibited a high power conversion efficiency of 20.2%, their reproducibility was limited. On the other hand, the inverted-type devices exhibited an efficiency of 18.2% with a greater stability and higher reproducibility than those of the normal-type devices. The reduced reproducibility of the normal-type devices was associated with the crack formation on the perovskite films during a spin-coating process. The hardness of both the perovskite and the sublayer was directly linked to the crack formation. Inverted-type 2D/3D FACsPbI3 with ozone-treated poly(triarylamine) as sublayer exhibited the highest phase stability owing to the hydrophobic nature of poly(triarylamine) and improved energy level alignment upon an ozone treatment. In addition, strong interaction between phenethylamine cations of the 2D perovskite and of the 3D FACsPbI...
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Total citations:
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GOST
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Thote A. et al. Stable and Reproducible 2D/3D Formamidinium–Lead–Iodide Perovskite Solar Cells // ACS Applied Energy Materials. 2019. Vol. 2. No. 4. pp. 2486-2493.
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Thote A., Jeon I., Lee J., Seo S., Lin H., Yang Y., Daiguji H., Maruyama S., MATSUO Y. Stable and Reproducible 2D/3D Formamidinium–Lead–Iodide Perovskite Solar Cells // ACS Applied Energy Materials. 2019. Vol. 2. No. 4. pp. 2486-2493.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acsaem.8b01964
UR - https://doi.org/10.1021/acsaem.8b01964
TI - Stable and Reproducible 2D/3D Formamidinium–Lead–Iodide Perovskite Solar Cells
T2 - ACS Applied Energy Materials
AU - Thote, Abhishek
AU - Jeon, Il
AU - Lee, Jinwook
AU - Seo, Seungju
AU - Lin, Hao-Sheng
AU - Yang, Yang
AU - Daiguji, Hirofumi
AU - Maruyama, Shigeo
AU - MATSUO, Yutaka
PY - 2019
DA - 2019/03/08
PB - American Chemical Society (ACS)
SP - 2486-2493
IS - 4
VL - 2
SN - 2574-0962
ER -
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BibTex (up to 50 authors)
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@article{2019_Thote,
author = {Abhishek Thote and Il Jeon and Jinwook Lee and Seungju Seo and Hao-Sheng Lin and Yang Yang and Hirofumi Daiguji and Shigeo Maruyama and Yutaka MATSUO},
title = {Stable and Reproducible 2D/3D Formamidinium–Lead–Iodide Perovskite Solar Cells},
journal = {ACS Applied Energy Materials},
year = {2019},
volume = {2},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/acsaem.8b01964},
number = {4},
pages = {2486--2493},
doi = {10.1021/acsaem.8b01964}
}
Cite this
MLA
Copy
Thote, Abhishek, et al. “Stable and Reproducible 2D/3D Formamidinium–Lead–Iodide Perovskite Solar Cells.” ACS Applied Energy Materials, vol. 2, no. 4, Mar. 2019, pp. 2486-2493. https://doi.org/10.1021/acsaem.8b01964.