ACS applied materials & interfaces

, том 12 , издание 18 , страницы 20563-20569

Material and Interfacial Modification toward a Stable Room-Temperature Solid-State Na–S Battery

Тип публикации: Journal Article

Дата публикации: 2020-04-14

American Chemical Society (ACS)

ACS applied materials & interfaces

scimago Q1

wos Q1

БС1

SJR: 1.921

CiteScore: 14.5

Impact factor: 8.2

ISSN: 19448244, 19448252

DOI: 10.1021/acsami.0c03899

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PubMed ID: 32286042

General Materials Science

Краткое описание

Room-temperature solid-state sodium batteries have the remarkable potential to simultaneously achieve high safety, high energy density and low cost. Yet their current performance is far below expectations. Through material and interfacial modification based on Na3PS4 solid electrolytes, progress is made toward stable room-temperature solid-state sodium-sulfur (Na-S) batteries. First, ionic liquid N-butyl-N-methylpyrrolidinium bis(fluorosulfonyl)imide (Pyr14FSI) is employed to modify anode/electrolyte interface. An overpotential of 0.55 V after 900 h of a symmetrical battery indicates enhanced interfacial stability. A stable in-situ solid electrolyte interphase layer is formed between the interface of NaSn and Na3PS4, proved by X-ray photoelectron spectroscopy measurements. Furthermore, selenium-doped sulfurized polyacrylonitrile (Se0.05S0.95@pPAN) is used to boost the ionic and electronic conductivity of the sulfur cathode. As a result, the Na-S battery using a Se0.05S0.95@pPAN cathode and the interfacial modification delivers stable cycle performance and enhanced rate capability.

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Воропаева Дарья

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33 публикации, 538 цитирований, 20 рецензий

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Институт общей и неорганической химии им. Н.С. Курнакова РАН

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An T. et al. Material and Interfacial Modification toward a Stable Room-Temperature Solid-State Na–S Battery // ACS applied materials & interfaces. 2020. Vol. 12. No. 18. pp. 20563-20569.

ГОСТ со всеми авторами (до 50) Скопировать

An T., Jia H., Peng L., Xie J. Material and Interfacial Modification toward a Stable Room-Temperature Solid-State Na–S Battery // ACS applied materials & interfaces. 2020. Vol. 12. No. 18. pp. 20563-20569.

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TY - JOUR

DO - 10.1021/acsami.0c03899

UR - https://doi.org/10.1021/acsami.0c03899

TI - Material and Interfacial Modification toward a Stable Room-Temperature Solid-State Na–S Battery

T2 - ACS applied materials & interfaces

AU - An, Tao

AU - Jia, Huanhuan

AU - Peng, Linfeng

AU - Xie, Jia

PY - 2020

DA - 2020/04/14

PB - American Chemical Society (ACS)

SP - 20563-20569

IS - 18

VL - 12

PMID - 32286042

SN - 1944-8244

SN - 1944-8252

ER -

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@article{2020_An,

author = {Tao An and Huanhuan Jia and Linfeng Peng and Jia Xie},

title = {Material and Interfacial Modification toward a Stable Room-Temperature Solid-State Na–S Battery},

journal = {ACS applied materials & interfaces},

year = {2020},

volume = {12},

publisher = {American Chemical Society (ACS)},

month = {apr},

url = {https://doi.org/10.1021/acsami.0c03899},

number = {18},

pages = {20563--20569},

doi = {10.1021/acsami.0c03899}

}

MLA

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An, Tao, et al. “Material and Interfacial Modification toward a Stable Room-Temperature Solid-State Na–S Battery.” ACS applied materials & interfaces, vol. 12, no. 18, Apr. 2020, pp. 20563-20569. https://doi.org/10.1021/acsami.0c03899.

Издатель

American Chemical Society (ACS)

Журнал

ACS applied materials & interfaces

scimago Q1

wos Q1

БС1

SJR

1.921

CiteScore

14.5

Impact factor

8.2

ISSN

19448244 (Print)

19448252 (Electronic)