ACS applied materials & interfaces, volume 12, issue 39, pages 43933-43941
Luminescent Nanothermometer Operating at Very High Temperature—Sensing up to 1000 K with Upconverting Nanoparticles (Yb3+/Tm3+)
Runowski Marcin
1
,
Woźny Przemysław
1
,
Stopikowska Natalia
1
,
Martin I.
2
,
Lavin V.
2
,
Lis S.
1
1
Faculty of Chemistry, Adam Mickiewicz University, Uniwersytetu Poznańskiego 8, 61-614 Poznań, Poland
|
2
Departamento de Física, MALTA Consolider Team, IMN and IUdEA, Universidad de La Laguna, Apdo. Correos 456, E-38200 San Cristóbal de La Laguna, Santa Cruz de Tenerife, Spain
|
Publication type: Journal Article
Publication date: 2020-09-01
Journal:
ACS applied materials & interfaces
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 9.5
ISSN: 19448244, 19448252
PubMed ID:
32869638
General Materials Science
Abstract
Lanthanide-based luminescent nanothermometers play a crucial role in optical temperature determination. However, because of the strong thermal quenching of the luminescence, as well as the deterioration of their sensitivity and resolution with temperature elevation, they can operate in a relatively low-temperature range, usually from cryogenic to ≈800 K. In this work, we show how to overcome these limitations and monitor very high-temperature values, with high sensitivity (≈2.1% K–1) and good thermal resolution (≈1.4 K) at around 1000 K. As an optical probe of temperature, we chose upconverting Yb3+–Tm3+ codoped YVO4 nanoparticles. For ratiometric sensing in the low-temperature range, we used the relative intensities of the Tm3+ emissions associated with the 3F2,3 and 3H4 thermally coupled levels, that is, 3F2,3 → 3H6/3H4 → 3H6 (700/800 nm) band intensity ratio. In order to improve sensitivity and resolution in the high-temperature range, we used the 940/800 nm band intensity ratio of the nonthermally coupled levels of Yb3+ (2F5/2 → 2F7/2) and Tm3+ (3H4 → 3H6). These NIR bands are very intense, even at extreme temperature values, and their intensity ratio changes significantly, allowing accurate temperature sensing with high thermal and spatial resolutions. The results presented in this work may be particularly important for industrial applications, such as metallurgy, catalysis, high-temperature synthesis, materials processing and engineering, and so forth, which require rapid, contactless temperature monitoring at extreme conditions.
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- We do not take into account publications that without a DOI.
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- Statistics recalculated weekly.
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Runowski M. et al. Luminescent Nanothermometer Operating at Very High Temperature—Sensing up to 1000 K with Upconverting Nanoparticles (Yb3+/Tm3+) // ACS applied materials & interfaces. 2020. Vol. 12. No. 39. pp. 43933-43941.
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Runowski M., Woźny P., Stopikowska N., Martin I., Lavin V., Lis S. Luminescent Nanothermometer Operating at Very High Temperature—Sensing up to 1000 K with Upconverting Nanoparticles (Yb3+/Tm3+) // ACS applied materials & interfaces. 2020. Vol. 12. No. 39. pp. 43933-43941.
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TY - JOUR
DO - 10.1021/acsami.0c13011
UR - https://doi.org/10.1021%2Facsami.0c13011
TI - Luminescent Nanothermometer Operating at Very High Temperature—Sensing up to 1000 K with Upconverting Nanoparticles (Yb3+/Tm3+)
T2 - ACS applied materials & interfaces
AU - Runowski, Marcin
AU - Lis, S.
AU - Woźny, Przemysław
AU - Stopikowska, Natalia
AU - Martin, I.
AU - Lavin, V.
PY - 2020
DA - 2020/09/01 00:00:00
PB - American Chemical Society (ACS)
SP - 43933-43941
IS - 39
VL - 12
PMID - 32869638
SN - 1944-8244
SN - 1944-8252
ER -
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@article{2020_Runowski,
author = {Marcin Runowski and S. Lis and Przemysław Woźny and Natalia Stopikowska and I. Martin and V. Lavin},
title = {Luminescent Nanothermometer Operating at Very High Temperature—Sensing up to 1000 K with Upconverting Nanoparticles (Yb3+/Tm3+)},
journal = {ACS applied materials & interfaces},
year = {2020},
volume = {12},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021%2Facsami.0c13011},
number = {39},
pages = {43933--43941},
doi = {10.1021/acsami.0c13011}
}
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MLA
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Runowski, Marcin, et al. “Luminescent Nanothermometer Operating at Very High Temperature—Sensing up to 1000 K with Upconverting Nanoparticles (Yb3+/Tm3+).” ACS applied materials & interfaces, vol. 12, no. 39, Sep. 2020, pp. 43933-43941. https://doi.org/10.1021%2Facsami.0c13011.