ACS applied materials & interfaces

, том 13 , издание 48 , страницы 57489-57496

Polymer Zwitterion-Based Artificial Interphase Layers for Stable Lithium Metal Anodes

Тип публикации: Journal Article

Дата публикации: 2021-11-29

American Chemical Society (ACS)

ACS applied materials & interfaces

scimago Q1

wos Q1

БС1

SJR: 1.921

CiteScore: 14.5

Impact factor: 8.2

ISSN: 19448244, 19448252

DOI: 10.1021/acsami.1c19479

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PubMed ID: 34839656

General Materials Science

Краткое описание

Lithium (Li) metal batteries are promising future rechargeable batteries with high-energy density as the Li metal anode (LMA) possesses a high specific capacity and the lowest potential. However, the commercial application of the LMA has been hindered by a low Coulombic efficiency and dendrite growth, which are related to the unstable interphase with poor Li+ ion transport. Herein, we report novel polymer zwitterion-based artificial interphase layers (AILs) with improved Li+ ion transport and high stability for long-life LMAs. Benefitting from the unique zwitterion effect within the polymer zwitterion-based AILs, a high Li+ ion transference number (0.81) and a good ionic conductivity (0.75 × 10-4 S cm-1) can be realized simultaneously at the interface. By regulating the weight ratio of the sulfonate group and the phosphate group in polymer zwitterion-based AILs, the modified LMA enables long-term Li plating/stripping for 1400 h at 1 mA cm-2 and stable cycling in a full cell. This interfacial engineering concept could shed light on the development of safe LMAs.

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Jin T. et al. Polymer Zwitterion-Based Artificial Interphase Layers for Stable Lithium Metal Anodes // ACS applied materials & interfaces. 2021. Vol. 13. No. 48. pp. 57489-57496.

ГОСТ со всеми авторами (до 50) Скопировать

Jin T., Liu M., Su K., Lu Y., Cheng G., Liu Y., Li N., Yu L. Polymer Zwitterion-Based Artificial Interphase Layers for Stable Lithium Metal Anodes // ACS applied materials & interfaces. 2021. Vol. 13. No. 48. pp. 57489-57496.

RIS |

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TY - JOUR

DO - 10.1021/acsami.1c19479

UR - https://doi.org/10.1021/acsami.1c19479

TI - Polymer Zwitterion-Based Artificial Interphase Layers for Stable Lithium Metal Anodes

T2 - ACS applied materials & interfaces

AU - Jin, Tong

AU - Liu, Ming

AU - Su, Kai

AU - Lu, Yue

AU - Cheng, Guang

AU - Liu, Yao

AU - Li, Nianwu

AU - Yu, Le

PY - 2021

DA - 2021/11/29

PB - American Chemical Society (ACS)

SP - 57489-57496

IS - 48

VL - 13

PMID - 34839656

SN - 1944-8244

SN - 1944-8252

ER -

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@article{2021_Jin,

author = {Tong Jin and Ming Liu and Kai Su and Yue Lu and Guang Cheng and Yao Liu and Nianwu Li and Le Yu},

title = {Polymer Zwitterion-Based Artificial Interphase Layers for Stable Lithium Metal Anodes},

journal = {ACS applied materials & interfaces},

year = {2021},

volume = {13},

publisher = {American Chemical Society (ACS)},

month = {nov},

url = {https://doi.org/10.1021/acsami.1c19479},

number = {48},

pages = {57489--57496},

doi = {10.1021/acsami.1c19479}

}

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Jin, Tong, et al. “Polymer Zwitterion-Based Artificial Interphase Layers for Stable Lithium Metal Anodes.” ACS applied materials & interfaces, vol. 13, no. 48, Nov. 2021, pp. 57489-57496. https://doi.org/10.1021/acsami.1c19479.

Издатель

American Chemical Society (ACS)

Журнал

ACS applied materials & interfaces

scimago Q1

wos Q1

БС1

SJR

1.921

CiteScore

14.5

Impact factor

8.2

ISSN

19448244 (Print)

19448252 (Electronic)