ACS applied materials & interfaces, volume 14, issue 4, pages 5932-5939
Ultrahigh Elastic Polymer Electrolytes for Solid-State Lithium Batteries with Robust Interfaces
Publication type: Journal Article
Publication date: 2022-01-18
Journal:
ACS applied materials & interfaces
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 9.5
ISSN: 19448244, 19448252
General Materials Science
Abstract
Solid polymer electrolytes (SPEs) are promising for solid-state lithium batteries, but their practical application is significantly impeded by their low ionic conductivity and poor compatibility. Here, we report an ultrahigh elastic SPE based on cross-linked polyurethane (PU), succinonitrile (SN), and lithium bistrifluoromethanesulfonimide (LiTFSI). The resulting electrolyte (PU-SN-LiTFSI) exhibits an ionic conductivity of 2.86 × 10-4 S cm-1, a tensile strength of 3.8 MPa, and a breaking elongation exceeding 3000% at room temperature. A solid-state lithium battery using the electrolyte exhibits a high specific capacity of 150 mAh g-1 at 0.2C and a long cycling life of up to 700 cycles at 0.5C at room temperature, showing one of the best performances among its counterparts. The excellent performances are attributed to the fact that its ultrahigh elasticity, good ionic conductivity, tensile strength, and electrochemical stability contribute to robust electrode/electrolyte interfaces, thus greatly decreasing the charge-transfer resistance in charge/discharge processes. Our investigations provide a novel strategy to address the intrinsic interfacial issue of solid-state batteries.
Top-30
Citations by journals
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Journal of Materials Chemistry A
1 publication, 4.17%
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Chemical Engineering Journal
1 publication, 4.17%
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ACS applied materials & interfaces
1 publication, 4.17%
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Chemical Record
1 publication, 4.17%
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EcoMat
1 publication, 4.17%
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1 publication, 4.17%
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European Polymer Journal
1 publication, 4.17%
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1 publication, 4.17%
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1 publication, 4.17%
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1 publication, 4.17%
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Polymers
1 publication, 4.17%
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Russian Chemical Reviews
1 publication, 4.17%
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Journal of Molecular Structure
1 publication, 4.17%
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Journal of Materials Science and Technology
1 publication, 4.17%
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Citations by publishers
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2
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10
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Elsevier
10 publications, 41.67%
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Wiley
8 publications, 33.33%
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American Chemical Society (ACS)
2 publications, 8.33%
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Royal Society of Chemistry (RSC)
1 publication, 4.17%
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Frontiers Media S.A.
1 publication, 4.17%
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 4.17%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 4.17%
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zheng T. et al. Ultrahigh Elastic Polymer Electrolytes for Solid-State Lithium Batteries with Robust Interfaces // ACS applied materials & interfaces. 2022. Vol. 14. No. 4. pp. 5932-5939.
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Zheng T., Cui X., Chu Y., Li H., Pan Q. Ultrahigh Elastic Polymer Electrolytes for Solid-State Lithium Batteries with Robust Interfaces // ACS applied materials & interfaces. 2022. Vol. 14. No. 4. pp. 5932-5939.
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TY - JOUR
DO - 10.1021/acsami.1c20243
UR - https://doi.org/10.1021/acsami.1c20243
TI - Ultrahigh Elastic Polymer Electrolytes for Solid-State Lithium Batteries with Robust Interfaces
T2 - ACS applied materials & interfaces
AU - Zheng, Tianxiang
AU - Cui, Ximing
AU - Li, Haijuan
AU - Chu, Ying
AU - Pan, Qinmin
PY - 2022
DA - 2022/01/18 00:00:00
PB - American Chemical Society (ACS)
SP - 5932-5939
IS - 4
VL - 14
SN - 1944-8244
SN - 1944-8252
ER -
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@article{2022_Zheng,
author = {Tianxiang Zheng and Ximing Cui and Haijuan Li and Ying Chu and Qinmin Pan},
title = {Ultrahigh Elastic Polymer Electrolytes for Solid-State Lithium Batteries with Robust Interfaces},
journal = {ACS applied materials & interfaces},
year = {2022},
volume = {14},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acsami.1c20243},
number = {4},
pages = {5932--5939},
doi = {10.1021/acsami.1c20243}
}
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MLA
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Zheng, Tianxiang, et al. “Ultrahigh Elastic Polymer Electrolytes for Solid-State Lithium Batteries with Robust Interfaces.” ACS applied materials & interfaces, vol. 14, no. 4, Jan. 2022, pp. 5932-5939. https://doi.org/10.1021/acsami.1c20243.