ACS applied materials & interfaces, volume 14, issue 3, pages 4170-4178
Double-Protected Layers with Solid–Liquid Hybrid Electrolytes for Long-Cycle-Life Lithium Batteries
Jiantao Tang
1
,
Leidanyang Wang
2
,
Changhao Tian
1
,
Chunguang Chen
3
,
Tao Huang
4
,
Lecai Zeng
2
,
Aishui Yu
1, 4
2
Shanghai Electric Group Co., Ltd., Central Academe, No. 960 Zhongxing Road, Shanghai 200070, China
|
Publication type: Journal Article
Publication date: 2022-01-14
Journal:
ACS applied materials & interfaces
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 9.5
ISSN: 19448244, 19448252
General Materials Science
Abstract
Lithium-ion batteries (LIBs) with liquid electrolytes (LEs) have problems such as electrolyte leakage, low safety profiles, and low energy density, which limit their further development. However, LIBs with solid electrolytes are safer with better energy and high-temperature performance. Thus, solid electrolyte system batteries have attracted widespread attention. However, due to the inherent rigidity of the LATP solid electrolyte, there is a high interface impedance at the LATP/electrode. In addition, the Ti element in LATP easily reacts with the Li metal. Here, we dripped an LE at the LATP/electrode interface (solid-liquid hybrid electrolytes) to reduce its interface impedance. A composite polymer electrolyte (CPE) protective film (containing PVDF, SN, and LiTFSI) was then cured in situ at the LATP/Li interface to avoid side reactions of LATP. The discharge specific capacity of the LiFePO4/LATP-12% LE-CPE/Li system is up to 150 mAh g-1, and the capacity retention rate is still 96% after 250 cycles. In addition, the NCM622/PVDF-LATP-12% LE/Li system has an initial reversible capacity of 170 mAh g-1. This study reports an approach that can protect solid electrolytes from lithium metal instability.
Top-30
Citations by journals
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1
2
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Journal of Power Sources
2 publications, 12.5%
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ACS applied materials & interfaces
2 publications, 12.5%
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ACS Applied Energy Materials
1 publication, 6.25%
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Batteries & Supercaps
1 publication, 6.25%
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Ceramics International
1 publication, 6.25%
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Angewandte Chemie
1 publication, 6.25%
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Angewandte Chemie - International Edition
1 publication, 6.25%
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ACS Sustainable Chemistry and Engineering
1 publication, 6.25%
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Batteries
1 publication, 6.25%
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International Journal of Applied Ceramic Technology
1 publication, 6.25%
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Energy Storage Materials
1 publication, 6.25%
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Aggregate
1 publication, 6.25%
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Small
1 publication, 6.25%
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Russian Chemical Reviews
1 publication, 6.25%
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1
2
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Citations by publishers
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1
2
3
4
5
6
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Wiley
6 publications, 37.5%
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American Chemical Society (ACS)
4 publications, 25%
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Elsevier
4 publications, 25%
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Multidisciplinary Digital Publishing Institute (MDPI)
1 publication, 6.25%
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Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii
1 publication, 6.25%
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1
2
3
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6
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Tang J. et al. Double-Protected Layers with Solid–Liquid Hybrid Electrolytes for Long-Cycle-Life Lithium Batteries // ACS applied materials & interfaces. 2022. Vol. 14. No. 3. pp. 4170-4178.
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Tang J., Wang L., Tian C., Chen C., Huang T., Zeng L., Yu A. Double-Protected Layers with Solid–Liquid Hybrid Electrolytes for Long-Cycle-Life Lithium Batteries // ACS applied materials & interfaces. 2022. Vol. 14. No. 3. pp. 4170-4178.
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TY - JOUR
DO - 10.1021/acsami.1c21457
UR - https://doi.org/10.1021/acsami.1c21457
TI - Double-Protected Layers with Solid–Liquid Hybrid Electrolytes for Long-Cycle-Life Lithium Batteries
T2 - ACS applied materials & interfaces
AU - Tang, Jiantao
AU - Wang, Leidanyang
AU - Tian, Changhao
AU - Chen, Chunguang
AU - Zeng, Lecai
AU - Yu, Aishui
AU - Huang, Tao
PY - 2022
DA - 2022/01/14 00:00:00
PB - American Chemical Society (ACS)
SP - 4170-4178
IS - 3
VL - 14
SN - 1944-8244
SN - 1944-8252
ER -
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@article{2022_Tang,
author = {Jiantao Tang and Leidanyang Wang and Changhao Tian and Chunguang Chen and Lecai Zeng and Aishui Yu and Tao Huang},
title = {Double-Protected Layers with Solid–Liquid Hybrid Electrolytes for Long-Cycle-Life Lithium Batteries},
journal = {ACS applied materials & interfaces},
year = {2022},
volume = {14},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acsami.1c21457},
number = {3},
pages = {4170--4178},
doi = {10.1021/acsami.1c21457}
}
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MLA
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Tang, Jiantao, et al. “Double-Protected Layers with Solid–Liquid Hybrid Electrolytes for Long-Cycle-Life Lithium Batteries.” ACS applied materials & interfaces, vol. 14, no. 3, Jan. 2022, pp. 4170-4178. https://doi.org/10.1021/acsami.1c21457.