ACS applied materials & interfaces, volume 9, issue 15, pages 13694-13702

Suppression of Lithium Dendrite Formation by Using LAGP-PEO (LiTFSI) Composite Solid Electrolyte and Lithium Metal Anode Modified by PEO (LiTFSI) in All-Solid-State Lithium Batteries.

Chunhua Wang ¹

Yifu Yang ¹

Xingjiang Liu ²

Hai Zhong ²

Han Xu ²

Zhibin Xu ²

Huixia Shao ¹

Fei Ding ²

Hide authors affiliations Show authors affiliations: 2 affiliations

College of Chemistry and Molecular Sciences, Wuhan University, Wuhan 430072, P.R. China |

National Key Lab of Power Sources, Tianjin Institute of Power Sources, Tianjin 300384, P.R. China |

Publication type: Journal Article

Publication date: 2017-04-07

American Chemical Society (ACS)

Journal: ACS applied materials & interfaces

Quartile SCImago

Quartile WOS

Impact factor: 9.5

ISSN: 19448244, 19448252

DOI: 10.1021/acsami.7b00336

Copy DOI

General Materials Science

Abstract

The formation of lithium dendrites is suppressed using a Li1.5Al0.5Ge1.5(PO4)3-poly(ethylene oxide) (LAGP-PEO) composite solid electrolyte and a PEO (lithium bis(trifluoromethane)sulfonimide) [PEO (LiTFSI)]-modified lithium metal anode in all-solid-state lithium batteries. The effects on the anode performance based on the PEO content in the composite solid electrolyte and the molecular weight of PEO used to modify the Li anode are studied. The structure, surface morphology, and stability of the composite solid electrolyte are examined by X-ray diffraction spectroscopy, scanning electron microscopy, and electrochemical tests. Results show that the presence of a PEO-500000(LiTFSI) film on a Li anode results in good mechanical properties and satisfactory interface contact features. The film can also prevent Li from reacting with LAGP. Furthermore, the formation of lithium dendrites can be effectively inhibited as the composite solid electrolyte is combined with the PEO film on the Li anode. The ratio of PEO in the composite solid electrolyte can be reduced to a low level of 1 wt %. PEO remains stable even at a high potential of 5.12 V (vs Li/Li+). The assembled Li-PEO (LiTFSI)/LAGP-PEO/LiMn0.8Fe0.2PO4 all-solid-state cell can deliver an initial discharge capacity of 160.8 mAh g-1 and exhibit good cycling stability and rate performance at 50 °C.

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Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 4, 1.18% Physical Chemistry Chemical Physics 4 publications, 1.18%
RSC Advances	RSC Advances, 4, 1.18% RSC Advances 4 publications, 1.18%
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Nano Research	Nano Research, 3, 0.88% Nano Research 3 publications, 0.88%
Advanced Science	Advanced Science, 3, 0.88% Advanced Science 3 publications, 0.88%
Small	Small, 3, 0.88% Small 3 publications, 0.88%
	5 10 15 20 25 30 35

Citations by publishers

	20 40 60 80 100 120 140
Elsevier	Elsevier, 128, 37.65% Elsevier 128 publications, 37.65%
American Chemical Society (ACS)	American Chemical Society (ACS), 63, 18.53% American Chemical Society (ACS) 63 publications, 18.53%
Wiley	Wiley, 50, 14.71% Wiley 50 publications, 14.71%
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Springer Nature	Springer Nature, 26, 7.65% Springer Nature 26 publications, 7.65%
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Frontiers Media S.A.	Frontiers Media S.A., 2, 0.59% Frontiers Media S.A. 2 publications, 0.59%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 2, 0.59% Nonferrous Metals Society of China 2 publications, 0.59%
IOP Publishing	IOP Publishing, 2, 0.59% IOP Publishing 2 publications, 0.59%
University of Science and Technology Beijing	University of Science and Technology Beijing, 1, 0.29% University of Science and Technology Beijing 1 publication, 0.29%
Tsinghua University Press	Tsinghua University Press, 1, 0.29% Tsinghua University Press 1 publication, 0.29%
Taylor & Francis	Taylor & Francis, 1, 0.29% Taylor & Francis 1 publication, 0.29%
OAE Publishing Inc.	OAE Publishing Inc., 1, 0.29% OAE Publishing Inc. 1 publication, 0.29%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.29% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.29%
	20 40 60 80 100 120 140

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Wang C. et al. Suppression of Lithium Dendrite Formation by Using LAGP-PEO (LiTFSI) Composite Solid Electrolyte and Lithium Metal Anode Modified by PEO (LiTFSI) in All-Solid-State Lithium Batteries. // ACS applied materials & interfaces. 2017. Vol. 9. No. 15. pp. 13694-13702.

GOST all authors (up to 50) Copy

Wang C., Yang Y., Liu X., Zhong H., Xu H., Xu Z., Shao H., Ding F. Suppression of Lithium Dendrite Formation by Using LAGP-PEO (LiTFSI) Composite Solid Electrolyte and Lithium Metal Anode Modified by PEO (LiTFSI) in All-Solid-State Lithium Batteries. // ACS applied materials & interfaces. 2017. Vol. 9. No. 15. pp. 13694-13702.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acsami.7b00336

UR - https://doi.org/10.1021/acsami.7b00336

TI - Suppression of Lithium Dendrite Formation by Using LAGP-PEO (LiTFSI) Composite Solid Electrolyte and Lithium Metal Anode Modified by PEO (LiTFSI) in All-Solid-State Lithium Batteries.

T2 - ACS applied materials & interfaces

AU - Wang, Chunhua

AU - Liu, Xingjiang

AU - Zhong, Hai

AU - Xu, Han

AU - Xu, Zhibin

AU - Shao, Huixia

AU - Yang, Yifu

AU - Ding, Fei

PY - 2017

DA - 2017/04/07 00:00:00

PB - American Chemical Society (ACS)

SP - 13694-13702

IS - 15

VL - 9

SN - 1944-8244

SN - 1944-8252

ER -

BibTex |

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BibTex Copy

@article{2017_Wang,

author = {Chunhua Wang and Xingjiang Liu and Hai Zhong and Han Xu and Zhibin Xu and Huixia Shao and Yifu Yang and Fei Ding},

title = {Suppression of Lithium Dendrite Formation by Using LAGP-PEO (LiTFSI) Composite Solid Electrolyte and Lithium Metal Anode Modified by PEO (LiTFSI) in All-Solid-State Lithium Batteries.},

journal = {ACS applied materials & interfaces},

year = {2017},

volume = {9},

publisher = {American Chemical Society (ACS)},

month = {apr},

url = {https://doi.org/10.1021/acsami.7b00336},

number = {15},

pages = {13694--13702},

doi = {10.1021/acsami.7b00336}

}

MLA

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MLA Copy

Wang, Chunhua, et al. “Suppression of Lithium Dendrite Formation by Using LAGP-PEO (LiTFSI) Composite Solid Electrolyte and Lithium Metal Anode Modified by PEO (LiTFSI) in All-Solid-State Lithium Batteries..” ACS applied materials & interfaces, vol. 9, no. 15, Apr. 2017, pp. 13694-13702. https://doi.org/10.1021/acsami.7b00336.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS applied materials & interfaces

Quartile SCImago

Quartile WOS

Impact factor

9.5

ISSN

19448244 (Print)
19448252 (Electronic)