Nanoscaled Na3PS4 Solid Electrolyte for All-Solid-State FeS2/Na Batteries with Ultrahigh Initial Coulombic Efficiency of 95% and Excellent Cyclic Performances
HONGLI WAN
1, 2
,
Jean Pierre Mwizerwa
1, 2
,
Xingguo Qi
2, 3
,
Xiaoxiong Xu
1
,
Hong Li
3
,
Vijay Kumar Singh
1, 2
,
Liangting Cai
1
,
Yong-Sheng Hu
3
,
Publication type: Journal Article
Publication date: 2018-04-02
scimago Q1
wos Q1
SJR: 1.921
CiteScore: 14.5
Impact factor: 8.2
ISSN: 19448244, 19448252
PubMed ID:
29608273
General Materials Science
Abstract
Nanosized Na3PS4 solid electrolyte with an ionic conductivity of 8.44 × 10-5 S cm-1 at room temperature is synthesized by a liquid-phase reaction. The resultant all-solid-state FeS2/Na3PS4/Na batteries show an extraordinary high initial Coulombic efficiency of 95% and demonstrate high energy density of 611 Wh kg-1 at current density of 20 mA g-1 at room temperature. The outstanding performances of the battery can be ascribed to good interface compatibility and intimate solid-solid contact at FeS2 electrode/nanosized Na3PS4 solid electrolytes interface. Meanwhile, excellent cycling stability is achieved for the battery after cycling at 60 mA g-1 for 100 cycles, showing a high capacity of 287 mAh g-1 with the capacity retention of 80%.
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GOST
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WAN H. et al. Nanoscaled Na3PS4 Solid Electrolyte for All-Solid-State FeS2/Na Batteries with Ultrahigh Initial Coulombic Efficiency of 95% and Excellent Cyclic Performances // ACS applied materials & interfaces. 2018. Vol. 10. No. 15. pp. 12300-12304.
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WAN H., Mwizerwa J. P., Qi X., Xu X., Li H., Singh V. K., Cai L., Hu Y., Yao X. Nanoscaled Na3PS4 Solid Electrolyte for All-Solid-State FeS2/Na Batteries with Ultrahigh Initial Coulombic Efficiency of 95% and Excellent Cyclic Performances // ACS applied materials & interfaces. 2018. Vol. 10. No. 15. pp. 12300-12304.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acsami.8b01805
UR - https://doi.org/10.1021/acsami.8b01805
TI - Nanoscaled Na3PS4 Solid Electrolyte for All-Solid-State FeS2/Na Batteries with Ultrahigh Initial Coulombic Efficiency of 95% and Excellent Cyclic Performances
T2 - ACS applied materials & interfaces
AU - WAN, HONGLI
AU - Mwizerwa, Jean Pierre
AU - Qi, Xingguo
AU - Xu, Xiaoxiong
AU - Li, Hong
AU - Singh, Vijay Kumar
AU - Cai, Liangting
AU - Hu, Yong-Sheng
AU - Yao, Xiayin
PY - 2018
DA - 2018/04/02
PB - American Chemical Society (ACS)
SP - 12300-12304
IS - 15
VL - 10
PMID - 29608273
SN - 1944-8244
SN - 1944-8252
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_WAN,
author = {HONGLI WAN and Jean Pierre Mwizerwa and Xingguo Qi and Xiaoxiong Xu and Hong Li and Vijay Kumar Singh and Liangting Cai and Yong-Sheng Hu and Xiayin Yao},
title = {Nanoscaled Na3PS4 Solid Electrolyte for All-Solid-State FeS2/Na Batteries with Ultrahigh Initial Coulombic Efficiency of 95% and Excellent Cyclic Performances},
journal = {ACS applied materials & interfaces},
year = {2018},
volume = {10},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/acsami.8b01805},
number = {15},
pages = {12300--12304},
doi = {10.1021/acsami.8b01805}
}
Cite this
MLA
Copy
WAN, HONGLI, et al. “Nanoscaled Na3PS4 Solid Electrolyte for All-Solid-State FeS2/Na Batteries with Ultrahigh Initial Coulombic Efficiency of 95% and Excellent Cyclic Performances.” ACS applied materials & interfaces, vol. 10, no. 15, Apr. 2018, pp. 12300-12304. https://doi.org/10.1021/acsami.8b01805.
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