ACS applied materials & interfaces, volume 11, issue 9, pages 8954-8960
Advanced Nanoclay-Based Nanocomposite Solid Polymer Electrolyte for Lithium Iron Phosphate Batteries
1
Department of Metallurgical Engineering, College of Mines and Earth Sciences, University of Utah, 135 S 1460 E, Room 412, Salt Lake City, Utah 84112-0114, United States
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Publication type: Journal Article
Publication date: 2019-02-06
Journal:
ACS applied materials & interfaces
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 9.5
ISSN: 19448244, 19448252
General Materials Science
Abstract
High-performance solid polymer electrolytes (SPEs) have long been desired for the next generation of lithium batteries. One of the most promising ways to improve the morphological and electrochemical properties of SPEs is the addition of fillers with specific nanostructures. However, the production of such fillers is generally expensive and requires complicated preparation procedures. Halloysite nanotubes (HNTs), with their tubular structure, resemble carbon nanotubes in terms of geometric features and can be obtained at a relatively low cost. Previously, we reported that the HNT poly(ethylene oxide) composite SPE possesses excellent electrochemical and mechanical properties and outstanding cycling performance for all-solid-state lithium sulfur batteries. However, the HNT/SPE was not effective for lithium iron phosphate (LFP) batteries. The compatibility between the electrodes and the electrolyte sharply decreased, and no decent cycling performance was achieved. Therefore, a modification was studied which involves a minor addition of LFP during the preparation procedure. With this modification, good ionic conductivity (9.23 × 10-5 S cm-1 at 25 °C) is achieved, and compatibility between the electrodes and the electrolyte is enhanced. At the same time, an electrochemical stability window of 5.14 V and lithium-ion transference number of 0.46 are found. All-solid-state LFP batteries possessing excellent cycling performance are further demonstrated.
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Citations by publishers
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1 publication, 1.92%
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5
10
15
20
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Zhu Q., Wang X., Miller J. D. Advanced Nanoclay-Based Nanocomposite Solid Polymer Electrolyte for Lithium Iron Phosphate Batteries // ACS applied materials & interfaces. 2019. Vol. 11. No. 9. pp. 8954-8960.
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Zhu Q., Wang X., Miller J. D. Advanced Nanoclay-Based Nanocomposite Solid Polymer Electrolyte for Lithium Iron Phosphate Batteries // ACS applied materials & interfaces. 2019. Vol. 11. No. 9. pp. 8954-8960.
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TY - JOUR
DO - 10.1021/acsami.8b13735
UR - https://doi.org/10.1021/acsami.8b13735
TI - Advanced Nanoclay-Based Nanocomposite Solid Polymer Electrolyte for Lithium Iron Phosphate Batteries
T2 - ACS applied materials & interfaces
AU - Zhu, Qinyu
AU - Wang, Xuming
AU - Miller, Jan D.
PY - 2019
DA - 2019/02/06 00:00:00
PB - American Chemical Society (ACS)
SP - 8954-8960
IS - 9
VL - 11
SN - 1944-8244
SN - 1944-8252
ER -
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@article{2019_Zhu,
author = {Qinyu Zhu and Xuming Wang and Jan D. Miller},
title = {Advanced Nanoclay-Based Nanocomposite Solid Polymer Electrolyte for Lithium Iron Phosphate Batteries},
journal = {ACS applied materials & interfaces},
year = {2019},
volume = {11},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/acsami.8b13735},
number = {9},
pages = {8954--8960},
doi = {10.1021/acsami.8b13735}
}
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Zhu, Qinyu, et al. “Advanced Nanoclay-Based Nanocomposite Solid Polymer Electrolyte for Lithium Iron Phosphate Batteries.” ACS applied materials & interfaces, vol. 11, no. 9, Feb. 2019, pp. 8954-8960. https://doi.org/10.1021/acsami.8b13735.