Concurrent Sensing of CO2 and H2O from Air Using Ultramicroporous Fluorinated Metal-Organic Frameworks: Effect of Transduction Mechanism on the Sensing Performance.
Publication type: Journal Article
Publication date: 2018-12-10
scimago Q1
wos Q1
SJR: 1.921
CiteScore: 14.5
Impact factor: 8.2
ISSN: 19448244, 19448252
PubMed ID:
30525415
General Materials Science
Abstract
Conventional materials for gas/vapor sensing are limited to a single probe detection ability for specific analytes. However, materials capable of concurrent detection of two different probes in their respective harmful levels and using two types of sensing modes have yet to be explored. In particular, the concurrent detection of uncomfortable humidity levels and CO2 concentration (400-5000 ppm) in confined spaces is of extreme importance in a great variety of fields, such as submarine technology, aerospace, mining, and rescue operations. Herein, we report the deliberate construction and performance assessment of extremely sensitive sensors using an interdigitated electrode (IDE)-based capacitor and a quartz crystal microbalance (QCM) as transducing substrates. The unveiled sensors are able to simultaneously detect CO2 within the 400-5000 ppm range and relative humidity levels below 40 and above 60%, using two fluorinated metal-organic frameworks, namely, NbOFFIVE-1-Ni and AlFFIVE-1-Ni, fabricated as a thin film. Their subtle difference in a structure-adsorption relationship for H2O and CO2 was analyzed to unveil the corresponding structure-sensing property relationships using both QCM- and IDE-based sensing modes.
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GOST
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Tchalala M. R. et al. Concurrent Sensing of CO2 and H2O from Air Using Ultramicroporous Fluorinated Metal-Organic Frameworks: Effect of Transduction Mechanism on the Sensing Performance. // ACS applied materials & interfaces. 2018. Vol. 11. No. 1. pp. 1706-1712.
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Tchalala M. R., Belmabkhout Y., Adil K., Chappanda K. N., Cadiau A., Bhatt P. M., Salama K. N., Eddaoudi M. Concurrent Sensing of CO2 and H2O from Air Using Ultramicroporous Fluorinated Metal-Organic Frameworks: Effect of Transduction Mechanism on the Sensing Performance. // ACS applied materials & interfaces. 2018. Vol. 11. No. 1. pp. 1706-1712.
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RIS
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TY - JOUR
DO - 10.1021/acsami.8b18327
UR - https://doi.org/10.1021/acsami.8b18327
TI - Concurrent Sensing of CO2 and H2O from Air Using Ultramicroporous Fluorinated Metal-Organic Frameworks: Effect of Transduction Mechanism on the Sensing Performance.
T2 - ACS applied materials & interfaces
AU - Tchalala, Mohamed Rachid
AU - Belmabkhout, Youssef
AU - Adil, K.
AU - Chappanda, Karumbaiah N.
AU - Cadiau, A.
AU - Bhatt, Prashant M.
AU - Salama, Khaled Nabil
AU - Eddaoudi, Mohamed
PY - 2018
DA - 2018/12/10
PB - American Chemical Society (ACS)
SP - 1706-1712
IS - 1
VL - 11
PMID - 30525415
SN - 1944-8244
SN - 1944-8252
ER -
Cite this
BibTex (up to 50 authors)
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@article{2018_Tchalala,
author = {Mohamed Rachid Tchalala and Youssef Belmabkhout and K. Adil and Karumbaiah N. Chappanda and A. Cadiau and Prashant M. Bhatt and Khaled Nabil Salama and Mohamed Eddaoudi},
title = {Concurrent Sensing of CO2 and H2O from Air Using Ultramicroporous Fluorinated Metal-Organic Frameworks: Effect of Transduction Mechanism on the Sensing Performance.},
journal = {ACS applied materials & interfaces},
year = {2018},
volume = {11},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/acsami.8b18327},
number = {1},
pages = {1706--1712},
doi = {10.1021/acsami.8b18327}
}
Cite this
MLA
Copy
Tchalala, Mohamed Rachid, et al. “Concurrent Sensing of CO2 and H2O from Air Using Ultramicroporous Fluorinated Metal-Organic Frameworks: Effect of Transduction Mechanism on the Sensing Performance..” ACS applied materials & interfaces, vol. 11, no. 1, Dec. 2018, pp. 1706-1712. https://doi.org/10.1021/acsami.8b18327.