ACS applied materials & interfaces, volume 11, issue 38, pages 34930-34938

Remarkable Conductivity of a Self-Healing Single-Ion Conducting Polymer Electrolyte, Poly(ethylene-co-acrylic lithium (fluoro sulfonyl)imide), for All-Solid-State Li-Ion Batteries

Faiz Ahmed ¹

Inhwan Choi ¹

Md. Mahbubur Rahman ¹

Hohyoun Jang ¹

Taewook Ryu ¹

Sujin Yoon ¹

Lei Jin ¹

Yongcheng Jin ²

Whangi Kim ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

Department of Energy and Materials, Konkuk University, Chungju 27478, South Korea |

Qingdao Institute of Bioenergy and Bioprocess Technology, Chinese Academy of Sciences, Xinyuan Road, Laoshan Qu, Qingdao Shi, Shandong Sheng 266000, China |

Publication type: Journal Article

Publication date: 2019-08-30

American Chemical Society (ACS)

Journal: ACS applied materials & interfaces

Quartile SCImago

Quartile WOS

Impact factor: 9.5

ISSN: 19448244, 19448252

DOI: 10.1021/acsami.9b10474

Copy DOI

General Materials Science

Abstract

Single-ion conducting polymer electrolyte (SICPE) is a safer alternative to the conventional high-performance liquid electrolyte for Li-ion batteries. The performance of SICPEs-based Li-ion batteries is limited due to the low Li+ conductivities of SICPEs at room temperature. Herein, we demonstrated the synthesis of a novel SICPE, poly(ethylene-co-acrylic lithium (fluoro sulfonyl)imide) (PEALiFSI), with acrylic (fluoro sulfonyl)imide anion (AFSI). The solvent- and plasticizer-free PEALiFSI electrolyte, which was assembled at 90 °C under pressure, exhibited self-healing properties with remarkably high Li+ conductivity (5.84 × 10-4 S cm-1 at 25 °C). This is mainly due to the self-healing behavior of this electrolyte, which induced to increase the proportion of the amorphous phase. Additionally, the weak interaction of Li+ with the resonance-stabilized AFSI anion is also responsible for high Li+ conductivity. This self-healed SICPE showed high Li+ transference number (ca. 0.91), flame and heat retardancy, and good thermal stability, which concurrently delivered ca. 88.25% (150 mAh g-1 at 0.1C) of the theoretical capacitance of LiFePO4 cathode material at 25 °C with the full-cell configuration of LiFePO4/PEALiFSI/graphite. Furthermore, the self-healed PEALiFSI-based all-solid-state Li battery showed high electrochemical cycling stability with the capacity retention of 95% after 500 charge-discharge cycles.

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	2 4 6 8 10 12 14 16 18
American Chemical Society (ACS)	American Chemical Society (ACS), 18, 30.51% American Chemical Society (ACS) 18 publications, 30.51%
Elsevier	Elsevier, 17, 28.81% Elsevier 17 publications, 28.81%
Wiley	Wiley, 9, 15.25% Wiley 9 publications, 15.25%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 4, 6.78% Multidisciplinary Digital Publishing Institute (MDPI) 4 publications, 6.78%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 4, 6.78% Royal Society of Chemistry (RSC) 4 publications, 6.78%
Springer Nature	Springer Nature, 2, 3.39% Springer Nature 2 publications, 3.39%
IOP Publishing	IOP Publishing, 1, 1.69% IOP Publishing 1 publication, 1.69%
The Electrochemical Society	The Electrochemical Society, 1, 1.69% The Electrochemical Society 1 publication, 1.69%
Frontiers Media S.A.	Frontiers Media S.A., 1, 1.69% Frontiers Media S.A. 1 publication, 1.69%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.69% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.69%
	2 4 6 8 10 12 14 16 18

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Ahmed F. et al. Remarkable Conductivity of a Self-Healing Single-Ion Conducting Polymer Electrolyte, Poly(ethylene-co-acrylic lithium (fluoro sulfonyl)imide), for All-Solid-State Li-Ion Batteries // ACS applied materials & interfaces. 2019. Vol. 11. No. 38. pp. 34930-34938.

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Ahmed F., Choi I., Rahman M. M., Jang H., Ryu T., Yoon S., Jin L., Jin Y., Kim W. Remarkable Conductivity of a Self-Healing Single-Ion Conducting Polymer Electrolyte, Poly(ethylene-co-acrylic lithium (fluoro sulfonyl)imide), for All-Solid-State Li-Ion Batteries // ACS applied materials & interfaces. 2019. Vol. 11. No. 38. pp. 34930-34938.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/acsami.9b10474

UR - https://doi.org/10.1021/acsami.9b10474

TI - Remarkable Conductivity of a Self-Healing Single-Ion Conducting Polymer Electrolyte, Poly(ethylene-co-acrylic lithium (fluoro sulfonyl)imide), for All-Solid-State Li-Ion Batteries

T2 - ACS applied materials & interfaces

AU - Ahmed, Faiz

AU - Choi, Inhwan

AU - Ryu, Taewook

AU - Jin, Yongcheng

AU - Kim, Whangi

AU - Rahman, Md. Mahbubur

AU - Jang, Hohyoun

AU - Yoon, Sujin

AU - Jin, Lei

PY - 2019

DA - 2019/08/30 00:00:00

PB - American Chemical Society (ACS)

SP - 34930-34938

IS - 38

VL - 11

SN - 1944-8244

SN - 1944-8252

ER -

BibTex |

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BibTex Copy

@article{2019_Ahmed,

author = {Faiz Ahmed and Inhwan Choi and Taewook Ryu and Yongcheng Jin and Whangi Kim and Md. Mahbubur Rahman and Hohyoun Jang and Sujin Yoon and Lei Jin},

title = {Remarkable Conductivity of a Self-Healing Single-Ion Conducting Polymer Electrolyte, Poly(ethylene-co-acrylic lithium (fluoro sulfonyl)imide), for All-Solid-State Li-Ion Batteries},

journal = {ACS applied materials & interfaces},

year = {2019},

volume = {11},

publisher = {American Chemical Society (ACS)},

month = {aug},

url = {https://doi.org/10.1021/acsami.9b10474},

number = {38},

pages = {34930--34938},

doi = {10.1021/acsami.9b10474}

}

MLA

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MLA Copy

Ahmed, Faiz, et al. “Remarkable Conductivity of a Self-Healing Single-Ion Conducting Polymer Electrolyte, Poly(ethylene-co-acrylic lithium (fluoro sulfonyl)imide), for All-Solid-State Li-Ion Batteries.” ACS applied materials & interfaces, vol. 11, no. 38, Aug. 2019, pp. 34930-34938. https://doi.org/10.1021/acsami.9b10474.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS applied materials & interfaces

Quartile SCImago

Quartile WOS

Impact factor

9.5

ISSN

19448244 (Print)
19448252 (Electronic)