Insight on Reaction Pathways of Photocatalytic CO2 Conversion
Publication type: Journal Article
Publication date: 2022-06-03
scimago Q1
wos Q1
SJR: 3.782
CiteScore: 19.5
Impact factor: 13.1
ISSN: 21555435
PubMed ID:
35747201
General Chemistry
Catalysis
Abstract
Photocatalytic CO2 conversion to value-added chemicals is a promising solution to mitigate the current energy and environmental issues but is a challenging process. The main obstacles include the inertness of CO2 molecule, the sluggish multi-electron process, the unfavorable thermodynamics, and the selectivity control to preferable products. Furthermore, the lack of fundamental understanding of the reaction pathways accounts for the very moderate performance in the field. Therefore, in this Perspective, we attempt to discuss the possible reaction mechanisms toward all C1 and C2 value-added products, taking into account the experimental evidence and theoretical calculation on the surface adsorption, proton and electron transfer, and products desorption. Finally, the remaining challenges in the field, including mechanistic understanding, reactor design, economic consideration, and potential solutions, are critically discussed by us.
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Metrics
391
Total citations:
391
Citations from 2024:
296
(75.7%)
Cite this
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GOST
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Wang Y. et al. Insight on Reaction Pathways of Photocatalytic CO2 Conversion // ACS Catalysis. 2022. Vol. 12. No. 12. pp. 7300-7316.
GOST all authors (up to 50)
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Wang Y., Chen E., Tang J. Insight on Reaction Pathways of Photocatalytic CO2 Conversion // ACS Catalysis. 2022. Vol. 12. No. 12. pp. 7300-7316.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acscatal.2c01012
UR - https://doi.org/10.1021/acscatal.2c01012
TI - Insight on Reaction Pathways of Photocatalytic CO2 Conversion
T2 - ACS Catalysis
AU - Wang, Yiou
AU - Chen, Enqi
AU - Tang, Junwang
PY - 2022
DA - 2022/06/03
PB - American Chemical Society (ACS)
SP - 7300-7316
IS - 12
VL - 12
PMID - 35747201
SN - 2155-5435
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2022_Wang,
author = {Yiou Wang and Enqi Chen and Junwang Tang},
title = {Insight on Reaction Pathways of Photocatalytic CO2 Conversion},
journal = {ACS Catalysis},
year = {2022},
volume = {12},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acscatal.2c01012},
number = {12},
pages = {7300--7316},
doi = {10.1021/acscatal.2c01012}
}
Cite this
MLA
Copy
Wang, Yiou, et al. “Insight on Reaction Pathways of Photocatalytic CO2 Conversion.” ACS Catalysis, vol. 12, no. 12, Jun. 2022, pp. 7300-7316. https://doi.org/10.1021/acscatal.2c01012.