Metal–Organic Frameworks as Heterogeneous Catalysts in Hydrogen Production from Lightweight Inorganic Hydrides
Publication type: Journal Article
Publication date: 2017-07-05
scimago Q1
wos Q1
SJR: 3.782
CiteScore: 19.5
Impact factor: 13.1
ISSN: 21555435
General Chemistry
Catalysis
Abstract
Ammonia–borane (NH3·BH3, AB), hydrazine (NH2NH2), lithium borohydride (Li(BH4)), and sodium alanate (Na(AlH4)) are popular chemical hydrogen storage inorganic solid materials featuring high gravimetric hydrogen contents (H wt %) and remarkable stability under ambient conditions. Ultrapure H2 is formed from these compounds either via pyrolysis (i.e., a simple material heating) or via hydrolysis (chemical reaction with water). In both cases, a series of homogeneous and heterogeneous catalysts have been designed to assist the process. Among the latter, metal–organic frameworks (MOFs, crystalline 3D porous lattices made of metallic nodes and organic polytopic linkers) have rapidly emerged as versatile candidates for this role. The nanoconfinement of lightweight hydrides in MOFs produces a “hydride@MOF” composite material. Hydride coordination to MOF exposed metal sites or its reaction with functional groups on the organic linkers facilitates the thermal decomposition, lowering the hydrogen release temperature...
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103
Total citations:
103
Citations from 2024:
19
(18%)
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GOST
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Rossin A. et al. Metal–Organic Frameworks as Heterogeneous Catalysts in Hydrogen Production from Lightweight Inorganic Hydrides // ACS Catalysis. 2017. Vol. 7. No. 8. pp. 5035-5045.
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Rossin A., Tuci G., Luconi L., Giambastiani G. Metal–Organic Frameworks as Heterogeneous Catalysts in Hydrogen Production from Lightweight Inorganic Hydrides // ACS Catalysis. 2017. Vol. 7. No. 8. pp. 5035-5045.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acscatal.7b01495
UR - https://doi.org/10.1021/acscatal.7b01495
TI - Metal–Organic Frameworks as Heterogeneous Catalysts in Hydrogen Production from Lightweight Inorganic Hydrides
T2 - ACS Catalysis
AU - Rossin, Andrea
AU - Tuci, Giulia
AU - Luconi, Lapo
AU - Giambastiani, Giuliano
PY - 2017
DA - 2017/07/05
PB - American Chemical Society (ACS)
SP - 5035-5045
IS - 8
VL - 7
SN - 2155-5435
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2017_Rossin,
author = {Andrea Rossin and Giulia Tuci and Lapo Luconi and Giuliano Giambastiani},
title = {Metal–Organic Frameworks as Heterogeneous Catalysts in Hydrogen Production from Lightweight Inorganic Hydrides},
journal = {ACS Catalysis},
year = {2017},
volume = {7},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/acscatal.7b01495},
number = {8},
pages = {5035--5045},
doi = {10.1021/acscatal.7b01495}
}
Cite this
MLA
Copy
Rossin, Andrea, et al. “Metal–Organic Frameworks as Heterogeneous Catalysts in Hydrogen Production from Lightweight Inorganic Hydrides.” ACS Catalysis, vol. 7, no. 8, Jul. 2017, pp. 5035-5045. https://doi.org/10.1021/acscatal.7b01495.
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