Selenium-π-Acid Catalyzed Oxidative Functionalization of Alkynes: Facile Access to Ynones and Multisubstituted Oxazoles
Тип публикации: Journal Article
Дата публикации: 2018-06-19
scimago Q1
wos Q1
БС1
SJR: 3.847
CiteScore: 20.8
Impact factor: 13.1
ISSN: 21555435
General Chemistry
Catalysis
Краткое описание
Unprecedented selenium-catalyzed propargylic oxidation of alkynes is disclosed. Various propargylphosphonates and 3-alkynoates were efficiently converted to valuable ynones via unusual C–C triple bond migration and deselenenylation at a vinyl carbon. By the strategies of tautomerization of enamine intermediate and SN2 displacement, similar conditions were effective for the oxidative difunctionalization of ynamides to afford multisubstituted oxazoles with high regioselectivity. Mechanistic studies revealed these detailed processes.
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ГОСТ
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Liao L., Hang Z., Zhao X. Selenium-π-Acid Catalyzed Oxidative Functionalization of Alkynes: Facile Access to Ynones and Multisubstituted Oxazoles // ACS Catalysis. 2018. Vol. 8. No. 7. pp. 6745-6750.
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Liao L., Hang Z., Zhao X. Selenium-π-Acid Catalyzed Oxidative Functionalization of Alkynes: Facile Access to Ynones and Multisubstituted Oxazoles // ACS Catalysis. 2018. Vol. 8. No. 7. pp. 6745-6750.
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TY - JOUR
DO - 10.1021/acscatal.8b01595
UR - https://doi.org/10.1021/acscatal.8b01595
TI - Selenium-π-Acid Catalyzed Oxidative Functionalization of Alkynes: Facile Access to Ynones and Multisubstituted Oxazoles
T2 - ACS Catalysis
AU - Liao, Lihao
AU - Hang, Zhang
AU - Zhao, Xiaodan
PY - 2018
DA - 2018/06/19
PB - American Chemical Society (ACS)
SP - 6745-6750
IS - 7
VL - 8
SN - 2155-5435
ER -
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BibTex (до 50 авторов)
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@article{2018_Liao,
author = {Lihao Liao and Zhang Hang and Xiaodan Zhao},
title = {Selenium-π-Acid Catalyzed Oxidative Functionalization of Alkynes: Facile Access to Ynones and Multisubstituted Oxazoles},
journal = {ACS Catalysis},
year = {2018},
volume = {8},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acscatal.8b01595},
number = {7},
pages = {6745--6750},
doi = {10.1021/acscatal.8b01595}
}
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MLA
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Liao, Lihao, et al. “Selenium-π-Acid Catalyzed Oxidative Functionalization of Alkynes: Facile Access to Ynones and Multisubstituted Oxazoles.” ACS Catalysis, vol. 8, no. 7, Jun. 2018, pp. 6745-6750. https://doi.org/10.1021/acscatal.8b01595.