ACS Catalysis

, том 9 , издание 3 , страницы 2664-2673

Enhanced Electrocatalytic Activities by Substitutional Tuning of Nickel-Based Ruddlesden–Popper Catalysts for the Oxidation of Urea and Small Alcohols

Тип публикации: Journal Article

Дата публикации: 2019-02-11

American Chemical Society (ACS)

ACS Catalysis

scimago Q1

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SJR: 3.782

CiteScore: 19.5

Impact factor: 13.1

ISSN: 21555435

DOI: 10.1021/acscatal.8b04103

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General Chemistry

Catalysis

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The electrooxidation of urea continues to attract considerable interest as an alternative to the oxygen evolution reaction (OER) as the anodic reaction in the electrochemical generation of hydrogen due to the lower potential required to drive the reaction and the abundance of urea available in waste streams. Herein, we investigate the effect of Sr substitution in a series of La2–xSrxNiO4+δ Ruddlesden–Popper catalysts on the electrooxidations of urea, methanol, and ethanol and conclude that activities toward the urea oxidation reaction increase with increasing Ni oxidation state. The 75% Sr-substituted La0.5Sr1.5NiO4+δ catalyst exhibits a mass activity of 588 mA mgox–1 and 7.85 A mg–1 cmox–2 for the electrooxidation of urea in 1 M KOH containing 0.33 M urea, demonstrating the potential applications of Ni-based Ruddlesden–Popper materials for direct urea fuel cells and low-cost hydrogen production. Additionally, we find the same correlations between Ni oxidation state and activities for the electrooxidation...

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Садыков Владислав

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Институт катализа им. Г.К. Борескова СО РАН

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Forslund R. et al. Enhanced Electrocatalytic Activities by Substitutional Tuning of Nickel-Based Ruddlesden–Popper Catalysts for the Oxidation of Urea and Small Alcohols // ACS Catalysis. 2019. Vol. 9. No. 3. pp. 2664-2673.

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Forslund R., Alexander C., Abakumov A. M., Johnston K. P., Stevenson K. J. Enhanced Electrocatalytic Activities by Substitutional Tuning of Nickel-Based Ruddlesden–Popper Catalysts for the Oxidation of Urea and Small Alcohols // ACS Catalysis. 2019. Vol. 9. No. 3. pp. 2664-2673.

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TY - JOUR

DO - 10.1021/acscatal.8b04103

UR - https://doi.org/10.1021/acscatal.8b04103

TI - Enhanced Electrocatalytic Activities by Substitutional Tuning of Nickel-Based Ruddlesden–Popper Catalysts for the Oxidation of Urea and Small Alcohols

T2 - ACS Catalysis

AU - Forslund, Robin

AU - Alexander, Caleb

AU - Abakumov, Artem M.

AU - Johnston, Keith P.

AU - Stevenson, Keith J

PY - 2019

DA - 2019/02/11

PB - American Chemical Society (ACS)

SP - 2664-2673

IS - 3

VL - 9

SN - 2155-5435

ER -

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@article{2019_Forslund,

author = {Robin Forslund and Caleb Alexander and Artem M. Abakumov and Keith P. Johnston and Keith J Stevenson},

title = {Enhanced Electrocatalytic Activities by Substitutional Tuning of Nickel-Based Ruddlesden–Popper Catalysts for the Oxidation of Urea and Small Alcohols},

journal = {ACS Catalysis},

year = {2019},

volume = {9},

publisher = {American Chemical Society (ACS)},

month = {feb},

url = {https://doi.org/10.1021/acscatal.8b04103},

number = {3},

pages = {2664--2673},

doi = {10.1021/acscatal.8b04103}

}

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Forslund, Robin, et al. “Enhanced Electrocatalytic Activities by Substitutional Tuning of Nickel-Based Ruddlesden–Popper Catalysts for the Oxidation of Urea and Small Alcohols.” ACS Catalysis, vol. 9, no. 3, Feb. 2019, pp. 2664-2673. https://doi.org/10.1021/acscatal.8b04103.