ACS Energy Letters, volume 2, issue 4, pages 739-744

Suppressing Deep Traps in PbS Colloidal Quantum Dots via Facile Iodide Substitutional Doping for Solar Cells with Efficiency >10%

Alexandros Stavrinadis ¹

S Pradhan ¹

Paris Papagiorgis ²

G. Itskos ²

Gerasimos Konstantatos ^{1, 3}

Hide authors affiliations Show authors affiliations: 3 affiliations

ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain |

Department of Physics, Experimental Condensed Matter Physics Laboratory, University of Cyprus, Nicosia 1678, Cyprus |

ICREA—Institució Catalana de Recerca i Estudis Avançats, Passeig Lluís Companys 23, 08010 Barcelona, Spain |

Publication type: Journal Article

Publication date: 2017-03-06

American Chemical Society (ACS)

Journal: ACS Energy Letters

Quartile SCImago

Quartile WOS

Impact factor: 22

ISSN: 23808195, 23808195

DOI: 10.1021/acsenergylett.7b00091

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Materials Chemistry

Chemistry (miscellaneous)

Energy Engineering and Power Technology

Fuel Technology

Renewable Energy, Sustainability and the Environment

Abstract

Surface passivation of PbS colloidal quantum dots (QDs) with iodide has been used in highly efficient solar cells. Iodide passivation is typically achieved by ligand-exchange processes on QD films. Complementary to this approach, herein we present a nonintrusive solution-based strategy for doping QDs with iodide to further optimize solar cell performance. The doping step is applied in situ at the end of the synthesis of the QDs. The optimum precursor I/Pb ratio is found to be in the 1.5–3% range at which iodide substitutes S without excessively altering the dots’ surface chemistry. This allows for band engineering and decreasing the density of deep trap states of the QDs, which taken together lead to PbS QD solar cells with efficiency in excess of 10%.

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	1 2 3 4 5 6 7 8 9
ACS applied materials & interfaces	ACS applied materials & interfaces, 9, 9.89% ACS applied materials & interfaces 9 publications, 9.89%
ACS Energy Letters	ACS Energy Letters, 6, 6.59% ACS Energy Letters 6 publications, 6.59%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 4, 4.4% Journal of Materials Chemistry A 4 publications, 4.4%
Nanoscale	Nanoscale, 4, 4.4% Nanoscale 4 publications, 4.4%
Solar Energy Materials and Solar Cells	Solar Energy Materials and Solar Cells, 3, 3.3% Solar Energy Materials and Solar Cells 3 publications, 3.3%
Advanced Materials	Advanced Materials, 3, 3.3% Advanced Materials 3 publications, 3.3%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 3, 3.3% Journal of Physical Chemistry C 3 publications, 3.3%
ACS Applied Nano Materials	ACS Applied Nano Materials, 3, 3.3% ACS Applied Nano Materials 3 publications, 3.3%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 3, 3.3% Journal of Materials Chemistry C 3 publications, 3.3%
Journal of Chemical Physics	Journal of Chemical Physics, 2, 2.2% Journal of Chemical Physics 2 publications, 2.2%
Solar RRL	Solar RRL, 2, 2.2% Solar RRL 2 publications, 2.2%
Small	Small, 2, 2.2% Small 2 publications, 2.2%
Advanced Functional Materials	Advanced Functional Materials, 2, 2.2% Advanced Functional Materials 2 publications, 2.2%
Applied Physics Reviews	Applied Physics Reviews, 1, 1.1% Applied Physics Reviews 1 publication, 1.1%
Physical Review Letters	Physical Review Letters, 1, 1.1% Physical Review Letters 1 publication, 1.1%
ACS Photonics	ACS Photonics, 1, 1.1% ACS Photonics 1 publication, 1.1%
Materials	Materials, 1, 1.1% Materials 1 publication, 1.1%
Energies	Energies, 1, 1.1% Energies 1 publication, 1.1%
Frontiers in Materials	Frontiers in Materials, 1, 1.1% Frontiers in Materials 1 publication, 1.1%
Nature Communications	Nature Communications, 1, 1.1% Nature Communications 1 publication, 1.1%
Scientific Reports	Scientific Reports, 1, 1.1% Scientific Reports 1 publication, 1.1%
Nano-Micro Letters	Nano-Micro Letters, 1, 1.1% Nano-Micro Letters 1 publication, 1.1%
NPG Asia Materials	NPG Asia Materials, 1, 1.1% NPG Asia Materials 1 publication, 1.1%
Journal of Electronic Materials	Journal of Electronic Materials, 1, 1.1% Journal of Electronic Materials 1 publication, 1.1%
Materials Chemistry and Physics	Materials Chemistry and Physics, 1, 1.1% Materials Chemistry and Physics 1 publication, 1.1%
Applied Surface Science	Applied Surface Science, 1, 1.1% Applied Surface Science 1 publication, 1.1%
Materials Today Sustainability	Materials Today Sustainability, 1, 1.1% Materials Today Sustainability 1 publication, 1.1%
Chinese Physics B	Chinese Physics B, 1, 1.1% Chinese Physics B 1 publication, 1.1%
Solar Energy	Solar Energy, 1, 1.1% Solar Energy 1 publication, 1.1%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 1, 1.1% Journal of Colloid and Interface Science 1 publication, 1.1%
	1 2 3 4 5 6 7 8 9

Citations by publishers

	5 10 15 20 25 30
American Chemical Society (ACS)	American Chemical Society (ACS), 26, 28.57% American Chemical Society (ACS) 26 publications, 28.57%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 17, 18.68% Royal Society of Chemistry (RSC) 17 publications, 18.68%
Elsevier	Elsevier, 17, 18.68% Elsevier 17 publications, 18.68%
Wiley	Wiley, 13, 14.29% Wiley 13 publications, 14.29%
Springer Nature	Springer Nature, 5, 5.49% Springer Nature 5 publications, 5.49%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 3, 3.3% American Institute of Physics (AIP) 3 publications, 3.3%
American Physical Society (APS)	American Physical Society (APS), 2, 2.2% American Physical Society (APS) 2 publications, 2.2%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 2.2% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 2.2%
IOP Publishing	IOP Publishing, 2, 2.2% IOP Publishing 2 publications, 2.2%
Frontiers Media S.A.	Frontiers Media S.A., 1, 1.1% Frontiers Media S.A. 1 publication, 1.1%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 1.1% American Association for the Advancement of Science (AAAS) 1 publication, 1.1%
Pleiades Publishing	Pleiades Publishing, 1, 1.1% Pleiades Publishing 1 publication, 1.1%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 1.1% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 1.1%
	5 10 15 20 25 30

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Stavrinadis A. et al. Suppressing Deep Traps in PbS Colloidal Quantum Dots via Facile Iodide Substitutional Doping for Solar Cells with Efficiency >10% // ACS Energy Letters. 2017. Vol. 2. No. 4. pp. 739-744.

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Stavrinadis A., Pradhan S., Papagiorgis P., Itskos G., Konstantatos G. Suppressing Deep Traps in PbS Colloidal Quantum Dots via Facile Iodide Substitutional Doping for Solar Cells with Efficiency >10% // ACS Energy Letters. 2017. Vol. 2. No. 4. pp. 739-744.

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RIS Copy

TY - JOUR

DO - 10.1021/acsenergylett.7b00091

UR - https://doi.org/10.1021/acsenergylett.7b00091

TI - Suppressing Deep Traps in PbS Colloidal Quantum Dots via Facile Iodide Substitutional Doping for Solar Cells with Efficiency >10%

T2 - ACS Energy Letters

AU - Stavrinadis, Alexandros

AU - Konstantatos, Gerasimos

AU - Pradhan, S

AU - Papagiorgis, Paris

AU - Itskos, G.

PY - 2017

DA - 2017/03/06 00:00:00

PB - American Chemical Society (ACS)

SP - 739-744

IS - 4

VL - 2

SN - 2380-8195

ER -

BibTex |

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BibTex Copy

@article{2017_Stavrinadis,

author = {Alexandros Stavrinadis and Gerasimos Konstantatos and S Pradhan and Paris Papagiorgis and G. Itskos},

title = {Suppressing Deep Traps in PbS Colloidal Quantum Dots via Facile Iodide Substitutional Doping for Solar Cells with Efficiency >10%},

journal = {ACS Energy Letters},

year = {2017},

volume = {2},

publisher = {American Chemical Society (ACS)},

month = {mar},

url = {https://doi.org/10.1021/acsenergylett.7b00091},

number = {4},

pages = {739--744},

doi = {10.1021/acsenergylett.7b00091}

}

MLA

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Stavrinadis, Alexandros, et al. “Suppressing Deep Traps in PbS Colloidal Quantum Dots via Facile Iodide Substitutional Doping for Solar Cells with Efficiency >10%.” ACS Energy Letters, vol. 2, no. 4, Mar. 2017, pp. 739-744. https://doi.org/10.1021/acsenergylett.7b00091.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS Energy Letters

Quartile SCImago

Quartile WOS

Impact factor

ISSN

23808195 (Electronic)
23808195 (Print)