Drawing a Soft Interface: An Effective Interfacial Modification Strategy for Garnet-Type Solid-State Li Batteries
Yuanjun Shao
1, 2
,
Hongchun Wang
2
,
Zhengliang Gong
2
,
Dawei Wang
3
,
Bizhu Zheng
3
,
Jianping Zhu
3
,
Yaxiang Lu
1
,
Yong-Sheng Hu
1
,
Xiangxin Guo
4
,
Hong Li
1
,
Xuejie Huang
1
,
Yong Yang
2, 3
,
Ce Wen Nan
5
,
Liquan Chen
1
Publication type: Journal Article
Publication date: 2018-05-01
scimago Q1
wos Q1
SJR: 6.799
CiteScore: 29.6
Impact factor: 18.2
ISSN: 23808195
Materials Chemistry
Chemistry (miscellaneous)
Energy Engineering and Power Technology
Fuel Technology
Renewable Energy, Sustainability and the Environment
Abstract
Garnet-type solid-state electrolytes (SSEs) are considered to be a good choice for solid-state batteries, yet the interfacial issues with metallic Li limit their applications. Herein, we propose an ultrasimple and effective strategy to enhance the interfacial connection between garnet SSEs and Li metal just by drawing a graphite-based soft interface with a pencil. Both experimental analysis and theoretical calculations confirm that the reaction between the graphite-based interfacial layer and metallic lithium forms a lithiated connection interface with good lithium-ionic and electronic conductivity. Compared to the reported interfacial materials, the graphite provides a soft interface with better ductility and compressibility. With improvement by this soft interface, the impedance of symmetric Li cells significantly decreases and the cell cycle is stable for over 1000 h. Moreover, a solid-state battery with Li-metal anode, ternary NCM523 cathode, and treated-garnet SSEs is fabricated and displays excellen...
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353
Total citations:
353
Citations from 2024:
62
(17%)
Cite this
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GOST
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Shao Y. et al. Drawing a Soft Interface: An Effective Interfacial Modification Strategy for Garnet-Type Solid-State Li Batteries // ACS Energy Letters. 2018. Vol. 3. No. 6. pp. 1212-1218.
GOST all authors (up to 50)
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Shao Y., Wang H., Gong Z., Wang D., Zheng B., Zhu J., Lu Y., Hu Y., Guo X., Li H., Huang X., Yang Y., Nan C. W., Chen L. Drawing a Soft Interface: An Effective Interfacial Modification Strategy for Garnet-Type Solid-State Li Batteries // ACS Energy Letters. 2018. Vol. 3. No. 6. pp. 1212-1218.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acsenergylett.8b00453
UR - https://doi.org/10.1021/acsenergylett.8b00453
TI - Drawing a Soft Interface: An Effective Interfacial Modification Strategy for Garnet-Type Solid-State Li Batteries
T2 - ACS Energy Letters
AU - Shao, Yuanjun
AU - Wang, Hongchun
AU - Gong, Zhengliang
AU - Wang, Dawei
AU - Zheng, Bizhu
AU - Zhu, Jianping
AU - Lu, Yaxiang
AU - Hu, Yong-Sheng
AU - Guo, Xiangxin
AU - Li, Hong
AU - Huang, Xuejie
AU - Yang, Yong
AU - Nan, Ce Wen
AU - Chen, Liquan
PY - 2018
DA - 2018/05/01
PB - American Chemical Society (ACS)
SP - 1212-1218
IS - 6
VL - 3
SN - 2380-8195
ER -
Cite this
BibTex (up to 50 authors)
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@article{2018_Shao,
author = {Yuanjun Shao and Hongchun Wang and Zhengliang Gong and Dawei Wang and Bizhu Zheng and Jianping Zhu and Yaxiang Lu and Yong-Sheng Hu and Xiangxin Guo and Hong Li and Xuejie Huang and Yong Yang and Ce Wen Nan and Liquan Chen},
title = {Drawing a Soft Interface: An Effective Interfacial Modification Strategy for Garnet-Type Solid-State Li Batteries},
journal = {ACS Energy Letters},
year = {2018},
volume = {3},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/acsenergylett.8b00453},
number = {6},
pages = {1212--1218},
doi = {10.1021/acsenergylett.8b00453}
}
Cite this
MLA
Copy
Shao, Yuanjun, et al. “Drawing a Soft Interface: An Effective Interfacial Modification Strategy for Garnet-Type Solid-State Li Batteries.” ACS Energy Letters, vol. 3, no. 6, May. 2018, pp. 1212-1218. https://doi.org/10.1021/acsenergylett.8b00453.
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