Gas Evolution in All-Solid-State Battery Cells
Timo Bartsch
1
,
Florian Strauss
1
,
Toru Hatsukade
1
,
Alexander Schiele
1
,
A Young Kim
1
,
Pascal Hartmann
1, 2
,
Jürgen Janek
1, 3
,
2
BASF SE, 67056 Ludwigshafen, Germany
|
Publication type: Journal Article
Publication date: 2018-09-25
scimago Q1
wos Q1
SJR: 6.799
CiteScore: 29.6
Impact factor: 18.2
ISSN: 23808195
Materials Chemistry
Chemistry (miscellaneous)
Energy Engineering and Power Technology
Fuel Technology
Renewable Energy, Sustainability and the Environment
Abstract
The formation of gaseous side products in liquid electrolyte-based lithium-ion batteries has been intensively studied in recent years and identified as being one of the sources of degradation (an indication of electrolyte and electrode instabilities). Herein, we demonstrate, to our knowledge for the first time, that gassing can also arise in all-solid-state battery cells made of Ni-rich layered oxide cathode materials and thiophosphate-based solid electrolytes. Combining isotopic labeling, titration for quantitative carbonate determination, and operando gas analysis, our findings reveal the evolution of CO2 stemming from carbonate species on the cathode surface as well as O2 from the bulk of the oxide cathode at potentials above 4.5 V with respect to Li+/Li, among others.
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Metrics
132
Total citations:
132
Citations from 2024:
37
(28%)
Cite this
GOST |
RIS |
BibTex |
MLA
Cite this
GOST
Copy
Bartsch T. et al. Gas Evolution in All-Solid-State Battery Cells // ACS Energy Letters. 2018. Vol. 3. No. 10. pp. 2539-2543.
GOST all authors (up to 50)
Copy
Bartsch T., Strauss F., Hatsukade T., Schiele A., Kim A. Y., Hartmann P., Janek J., Brezesinski T. Gas Evolution in All-Solid-State Battery Cells // ACS Energy Letters. 2018. Vol. 3. No. 10. pp. 2539-2543.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/acsenergylett.8b01457
UR - https://doi.org/10.1021/acsenergylett.8b01457
TI - Gas Evolution in All-Solid-State Battery Cells
T2 - ACS Energy Letters
AU - Bartsch, Timo
AU - Strauss, Florian
AU - Hatsukade, Toru
AU - Schiele, Alexander
AU - Kim, A Young
AU - Hartmann, Pascal
AU - Janek, Jürgen
AU - Brezesinski, Torsten
PY - 2018
DA - 2018/09/25
PB - American Chemical Society (ACS)
SP - 2539-2543
IS - 10
VL - 3
SN - 2380-8195
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Bartsch,
author = {Timo Bartsch and Florian Strauss and Toru Hatsukade and Alexander Schiele and A Young Kim and Pascal Hartmann and Jürgen Janek and Torsten Brezesinski},
title = {Gas Evolution in All-Solid-State Battery Cells},
journal = {ACS Energy Letters},
year = {2018},
volume = {3},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/acsenergylett.8b01457},
number = {10},
pages = {2539--2543},
doi = {10.1021/acsenergylett.8b01457}
}
Cite this
MLA
Copy
Bartsch, Timo, et al. “Gas Evolution in All-Solid-State Battery Cells.” ACS Energy Letters, vol. 3, no. 10, Sep. 2018, pp. 2539-2543. https://doi.org/10.1021/acsenergylett.8b01457.