Multimodality of Structural, Electrical, and Gravimetric Responses of Intercalated MXenes to Water
Publication type: Journal Article
Publication date: 2017-10-17
scimago Q1
wos Q1
SJR: 4.497
CiteScore: 24.2
Impact factor: 16.0
ISSN: 19360851, 1936086X
PubMed ID:
29019645
General Physics and Astronomy
General Materials Science
General Engineering
Abstract
Understanding of structural, electrical, and gravimetric peculiarities of water vapor interaction with ion-intercalated MXenes led to design of a multimodal humidity sensor. Neutron scattering coupled to molecular dynamics and ab initio calculations showed that a small amount of hydration results in a significant increase in the spacing between MXene layers in the presence of K and Mg intercalants between the layers. Films of K- and Mg-intercalated MXenes exhibited relative humidity (RH) detection thresholds of ∼0.8% RH and showed monotonic RH response in the 0-85% RH range. We found that MXene gravimetric response to water is 10 times faster than their electrical response, suggesting that H2O-induced swelling/contraction of channels between MXene sheets results in trapping of H2O molecules that act as charge-depleting dopants. The results demonstrate the use of MXenes as humidity sensors and infer potential impact of water on structural and electrical performance of MXene-based devices.
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240
Total citations:
240
Citations from 2024:
74
(30.84%)
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Muckley E. S. et al. Multimodality of Structural, Electrical, and Gravimetric Responses of Intercalated MXenes to Water // ACS Nano. 2017. Vol. 11. No. 11. pp. 11118-11126.
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Muckley E. S., Tyagi M. B., Nanda J., Ivanov I. N. Multimodality of Structural, Electrical, and Gravimetric Responses of Intercalated MXenes to Water // ACS Nano. 2017. Vol. 11. No. 11. pp. 11118-11126.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acsnano.7b05264
UR - https://doi.org/10.1021/acsnano.7b05264
TI - Multimodality of Structural, Electrical, and Gravimetric Responses of Intercalated MXenes to Water
T2 - ACS Nano
AU - Muckley, Eric S.
AU - Tyagi, Madhu B
AU - Nanda, Jagjit
AU - Ivanov, Ilia N.
PY - 2017
DA - 2017/10/17
PB - American Chemical Society (ACS)
SP - 11118-11126
IS - 11
VL - 11
PMID - 29019645
SN - 1936-0851
SN - 1936-086X
ER -
Cite this
BibTex (up to 50 authors)
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@article{2017_Muckley,
author = {Eric S. Muckley and Madhu B Tyagi and Jagjit Nanda and Ilia N. Ivanov},
title = {Multimodality of Structural, Electrical, and Gravimetric Responses of Intercalated MXenes to Water},
journal = {ACS Nano},
year = {2017},
volume = {11},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/acsnano.7b05264},
number = {11},
pages = {11118--11126},
doi = {10.1021/acsnano.7b05264}
}
Cite this
MLA
Copy
Muckley, Eric S., et al. “Multimodality of Structural, Electrical, and Gravimetric Responses of Intercalated MXenes to Water.” ACS Nano, vol. 11, no. 11, Oct. 2017, pp. 11118-11126. https://doi.org/10.1021/acsnano.7b05264.