Dihydrolevoglucosenone (Cyrene) As a Green Alternative to N,N-Dimethylformamide (DMF) in MOF Synthesis
Тип публикации: Journal Article
Дата публикации: 2016-10-13
scimago Q1
wos Q1
БС1
SJR: 1.623
CiteScore: 12.5
Impact factor: 7.3
ISSN: 21680485
General Chemistry
General Chemical Engineering
Environmental Chemistry
Renewable Energy, Sustainability and the Environment
Краткое описание
Cyrene, a green bioderived solvent from waste cellulose, was applied into the synthesis of metal–organic frameworks (MOFs). The MOF, HKUST-1, exhibited an even better Brunauer–Emmett–Teller surface area than HKUST-1 synthesized with DMF. Four additional archetypal MOFs were also synthesized to verify the universal application of Cyrene in MOF manufacturing. However, the BET surface areas were lower than DMF-made MOFs. It was observed that an aldol-condensation product of two Cyrene molecules in addition to Cyrene trapped within the pores are responsible for the lower than expected surface area. The use of Cyrene has led to a series of design principles that eliminate the need for problematic solvents such as DMF and can be applied to the synthesis of a wide range of MOFs.
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ГОСТ
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Zhang J. et al. Dihydrolevoglucosenone (Cyrene) As a Green Alternative to N,N-Dimethylformamide (DMF) in MOF Synthesis // ACS Sustainable Chemistry and Engineering. 2016. Vol. 4. No. 12. pp. 7186-7192.
ГОСТ со всеми авторами (до 50)
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Zhang J., White G. B., Ryan M. D., Hunt A. E., Katz M. J. Dihydrolevoglucosenone (Cyrene) As a Green Alternative to N,N-Dimethylformamide (DMF) in MOF Synthesis // ACS Sustainable Chemistry and Engineering. 2016. Vol. 4. No. 12. pp. 7186-7192.
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TY - JOUR
DO - 10.1021/acssuschemeng.6b02115
UR - https://doi.org/10.1021/acssuschemeng.6b02115
TI - Dihydrolevoglucosenone (Cyrene) As a Green Alternative to N,N-Dimethylformamide (DMF) in MOF Synthesis
T2 - ACS Sustainable Chemistry and Engineering
AU - Zhang, Jinfeng
AU - White, Gabrielle B
AU - Ryan, Michaela D
AU - Hunt, Andrew E.
AU - Katz, Michael J
PY - 2016
DA - 2016/10/13
PB - American Chemical Society (ACS)
SP - 7186-7192
IS - 12
VL - 4
SN - 2168-0485
ER -
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BibTex (до 50 авторов)
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@article{2016_Zhang,
author = {Jinfeng Zhang and Gabrielle B White and Michaela D Ryan and Andrew E. Hunt and Michael J Katz},
title = {Dihydrolevoglucosenone (Cyrene) As a Green Alternative to N,N-Dimethylformamide (DMF) in MOF Synthesis},
journal = {ACS Sustainable Chemistry and Engineering},
year = {2016},
volume = {4},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/acssuschemeng.6b02115},
number = {12},
pages = {7186--7192},
doi = {10.1021/acssuschemeng.6b02115}
}
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MLA
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Zhang, Jinfeng, et al. “Dihydrolevoglucosenone (Cyrene) As a Green Alternative to N,N-Dimethylformamide (DMF) in MOF Synthesis.” ACS Sustainable Chemistry and Engineering, vol. 4, no. 12, Oct. 2016, pp. 7186-7192. https://doi.org/10.1021/acssuschemeng.6b02115.