Polyacrylonitrile Fiber Supported N-Heterocyclic Carbene Ag(I) As Efficient Catalysts for Three-Component Coupling and Intramolecular 1,3-Dipolar Cycloaddition Reactions under Flow Conditions
Publication type: Journal Article
Publication date: 2017-03-14
scimago Q1
wos Q1
SJR: 1.623
CiteScore: 12.5
Impact factor: 7.3
ISSN: 21680485
General Chemistry
General Chemical Engineering
Environmental Chemistry
Renewable Energy, Sustainability and the Environment
Abstract
A series of recoverable and reusable N-heterocyclic carbene silver complexes supported on polyacrylonitrile fiber were prepared and characterized. Their catalytic performances in three-component coupling reactions of aldehydes, amines, and alkynes (A3 coupling) to synthesize propargylamines were evaluated. The catalysts were also used to prepare fused triazoles in one-pot reactions with excellent yields and diastereoselectivities. In these reactions, the substrates underwent A3 coupling followed by intramolecular 1,3-dipolar cycloaddition. The above reactions were also successfully performed in a continuous-flow process, and sustainable, modular, and efficient syntheses of propargylamines and fused triazoles were achieved.
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58
Total citations:
58
Citations from 2025:
5
(8.62%)
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GOST
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Cao J. et al. Polyacrylonitrile Fiber Supported N-Heterocyclic Carbene Ag(I) As Efficient Catalysts for Three-Component Coupling and Intramolecular 1,3-Dipolar Cycloaddition Reactions under Flow Conditions // ACS Sustainable Chemistry and Engineering. 2017. Vol. 5. No. 4. pp. 3438-3447.
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Cao J., Xu G., Li P., Tao M., Zhang W. Polyacrylonitrile Fiber Supported N-Heterocyclic Carbene Ag(I) As Efficient Catalysts for Three-Component Coupling and Intramolecular 1,3-Dipolar Cycloaddition Reactions under Flow Conditions // ACS Sustainable Chemistry and Engineering. 2017. Vol. 5. No. 4. pp. 3438-3447.
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RIS
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TY - JOUR
DO - 10.1021/acssuschemeng.7b00103
UR - https://doi.org/10.1021/acssuschemeng.7b00103
TI - Polyacrylonitrile Fiber Supported N-Heterocyclic Carbene Ag(I) As Efficient Catalysts for Three-Component Coupling and Intramolecular 1,3-Dipolar Cycloaddition Reactions under Flow Conditions
T2 - ACS Sustainable Chemistry and Engineering
AU - Cao, Jian
AU - Xu, Gang
AU - Li, Pengyu
AU - Tao, Minli
AU - Zhang, Wen-qin
PY - 2017
DA - 2017/03/14
PB - American Chemical Society (ACS)
SP - 3438-3447
IS - 4
VL - 5
SN - 2168-0485
ER -
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@article{2017_Cao,
author = {Jian Cao and Gang Xu and Pengyu Li and Minli Tao and Wen-qin Zhang},
title = {Polyacrylonitrile Fiber Supported N-Heterocyclic Carbene Ag(I) As Efficient Catalysts for Three-Component Coupling and Intramolecular 1,3-Dipolar Cycloaddition Reactions under Flow Conditions},
journal = {ACS Sustainable Chemistry and Engineering},
year = {2017},
volume = {5},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://doi.org/10.1021/acssuschemeng.7b00103},
number = {4},
pages = {3438--3447},
doi = {10.1021/acssuschemeng.7b00103}
}
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Cao, Jian, et al. “Polyacrylonitrile Fiber Supported N-Heterocyclic Carbene Ag(I) As Efficient Catalysts for Three-Component Coupling and Intramolecular 1,3-Dipolar Cycloaddition Reactions under Flow Conditions.” ACS Sustainable Chemistry and Engineering, vol. 5, no. 4, Mar. 2017, pp. 3438-3447. https://doi.org/10.1021/acssuschemeng.7b00103.