Chemistry of Materials, volume 16, issue 23, pages 4772-4776
Enhanced Mobility of Poly(3-hexylthiophene) Transistors by Spin-Coating from High-Boiling-Point Solvents
Jui Fen Chang
1
,
Baoquan Sun
1
,
D. W. Breiby
1
,
Martin R. Nielsen
1
,
Theis I. Sølling
1
,
Mark Giles
1
,
Iain McCulloch
1
,
Publication type: Journal Article
Publication date: 2004-07-17
Journal:
Chemistry of Materials
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 8.6
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Abstract
Chloroform is a general solvent for poly(3-hexylthiophene) (P3HT) active layers in field-effect transistors. However, its low boiling point and rapid evaporation limit the time for crystallization during the spin-coating process, and field-effect mobilities achieved for P3HT films spin-coated from chloroform are typically on the order of 0.01 cm2/(V s). Here we investigate a range of solvents with higher boiling points. We find that 1,2,4-trichlorobenzene with good solubility and a high boiling point significantly improves the field-effect mobilities up to 0.12 cm2/(V s) with on:off ratios of 106. By controlling the microstructure through the choice of solvent while keeping the molecular weight fixed, we observe a clear correlation between the field-effect mobility and the degree of microcrystalline order as measured by X-ray diffraction, as well as the strength of polaronic relaxation of charge carriers in the accumulation layer as measured by optical spectroscopy of field-induced charge.
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Citations by publishers
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198 publications, 23.43%
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The Chemical Society of Japan
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- We do not take into account publications without a DOI.
- Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
- Statistics recalculated weekly.
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Chang J. F. et al. Enhanced Mobility of Poly(3-hexylthiophene) Transistors by Spin-Coating from High-Boiling-Point Solvents // Chemistry of Materials. 2004. Vol. 16. No. 23. pp. 4772-4776.
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Chang J. F., Sun B., Breiby D. W., Nielsen M. R., Sølling T. I., Giles M., McCulloch I., Sirringhaus H. Enhanced Mobility of Poly(3-hexylthiophene) Transistors by Spin-Coating from High-Boiling-Point Solvents // Chemistry of Materials. 2004. Vol. 16. No. 23. pp. 4772-4776.
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TY - JOUR
DO - 10.1021/cm049617w
UR - https://doi.org/10.1021/cm049617w
TI - Enhanced Mobility of Poly(3-hexylthiophene) Transistors by Spin-Coating from High-Boiling-Point Solvents
T2 - Chemistry of Materials
AU - Giles, Mark
AU - Chang, Jui Fen
AU - Sun, Baoquan
AU - Breiby, D. W.
AU - Nielsen, Martin R.
AU - Sølling, Theis I.
AU - McCulloch, Iain
AU - Sirringhaus, Henning
PY - 2004
DA - 2004/07/17 00:00:00
PB - American Chemical Society (ACS)
SP - 4772-4776
IS - 23
VL - 16
SN - 0897-4756
SN - 1520-5002
ER -
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@article{2004_Chang,
author = {Mark Giles and Jui Fen Chang and Baoquan Sun and D. W. Breiby and Martin R. Nielsen and Theis I. Sølling and Iain McCulloch and Henning Sirringhaus},
title = {Enhanced Mobility of Poly(3-hexylthiophene) Transistors by Spin-Coating from High-Boiling-Point Solvents},
journal = {Chemistry of Materials},
year = {2004},
volume = {16},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/cm049617w},
number = {23},
pages = {4772--4776},
doi = {10.1021/cm049617w}
}
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Chang, Jui Fen, et al. “Enhanced Mobility of Poly(3-hexylthiophene) Transistors by Spin-Coating from High-Boiling-Point Solvents.” Chemistry of Materials, vol. 16, no. 23, Jul. 2004, pp. 4772-4776. https://doi.org/10.1021/cm049617w.