Shape Selectivity in the Conversion of Methanol to Hydrocarbons: The Catalytic Performance of One-Dimensional 10-Ring Zeolites: ZSM-22, ZSM-23, ZSM-48, and EU-1
Shewangizaw Teketel
1
,
Wegard Skistad
1
,
Sandrine Benard
1
,
U. Olsbye
1
,
K. P. Lillerud
1
,
Pablo Beato
2
,
Stian Svelle
1
2
Haldor Topsøe, Nymøllevej 55, DK-2800 Kgs. Lyngby, Denmark
|
Publication type: Journal Article
Publication date: 2011-11-23
scimago Q1
wos Q1
SJR: 3.782
CiteScore: 19.5
Impact factor: 13.1
ISSN: 21555435
General Chemistry
Catalysis
Abstract
The methanol-to-hydrocarbon (MTH) reaction, a process in which low-value carbon-rich feedstocks are converted to value-added petrochemical products, is studied over one-dimensional 10-ring zeolites: ZSM-22 (TON), ZSM-23 (MTT), ZSM-48 (*MRE), and EU-1 (EUO). The latter three are little studied as MTH catalysts and were expected to display interesting product-shape-selective properties. The influence of slight differences in channel systems of the materials (size and shape) on product distribution and stability is investigated under various reaction conditions. In addition, the influence of coke deposition on product selectivity is investigated. Temperatures between 350 and 500 °C and WHSV between 2 and 6 g g–1 h–1 are investigated using a fixed bed reactor. The products are analyzed using online GC, and hydrocarbons trapped in the channels of the material during the reaction were liberated using the standard HF dissolution procedure and analyzed using GC/MS. Despite the small differences in the channel sha...
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Teketel S. et al. Shape Selectivity in the Conversion of Methanol to Hydrocarbons: The Catalytic Performance of One-Dimensional 10-Ring Zeolites: ZSM-22, ZSM-23, ZSM-48, and EU-1 // ACS Catalysis. 2011. Vol. 2. No. 1. pp. 26-37.
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Teketel S., Skistad W., Benard S., Olsbye U., Lillerud K. P., Beato P., Svelle S. Shape Selectivity in the Conversion of Methanol to Hydrocarbons: The Catalytic Performance of One-Dimensional 10-Ring Zeolites: ZSM-22, ZSM-23, ZSM-48, and EU-1 // ACS Catalysis. 2011. Vol. 2. No. 1. pp. 26-37.
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RIS
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TY - JOUR
DO - 10.1021/cs200517u
UR - https://doi.org/10.1021/cs200517u
TI - Shape Selectivity in the Conversion of Methanol to Hydrocarbons: The Catalytic Performance of One-Dimensional 10-Ring Zeolites: ZSM-22, ZSM-23, ZSM-48, and EU-1
T2 - ACS Catalysis
AU - Teketel, Shewangizaw
AU - Skistad, Wegard
AU - Benard, Sandrine
AU - Olsbye, U.
AU - Lillerud, K. P.
AU - Beato, Pablo
AU - Svelle, Stian
PY - 2011
DA - 2011/11/23
PB - American Chemical Society (ACS)
SP - 26-37
IS - 1
VL - 2
SN - 2155-5435
ER -
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@article{2011_Teketel,
author = {Shewangizaw Teketel and Wegard Skistad and Sandrine Benard and U. Olsbye and K. P. Lillerud and Pablo Beato and Stian Svelle},
title = {Shape Selectivity in the Conversion of Methanol to Hydrocarbons: The Catalytic Performance of One-Dimensional 10-Ring Zeolites: ZSM-22, ZSM-23, ZSM-48, and EU-1},
journal = {ACS Catalysis},
year = {2011},
volume = {2},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/cs200517u},
number = {1},
pages = {26--37},
doi = {10.1021/cs200517u}
}
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MLA
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Teketel, Shewangizaw, et al. “Shape Selectivity in the Conversion of Methanol to Hydrocarbons: The Catalytic Performance of One-Dimensional 10-Ring Zeolites: ZSM-22, ZSM-23, ZSM-48, and EU-1.” ACS Catalysis, vol. 2, no. 1, Nov. 2011, pp. 26-37. https://doi.org/10.1021/cs200517u.