Hydrogenolysis of Glycerol by the Combined Use of Zeolite and Ni/Al2O3 as Catalysts: A Route for Achieving High Selectivity to 1-Propanol
Тип публикации: Journal Article
Дата публикации: 2014-04-25
scimago Q1
wos Q1
БС1
SJR: 1.124
CiteScore: 9.5
Impact factor: 5.3
ISSN: 08870624, 15205029
General Chemical Engineering
Energy Engineering and Power Technology
Fuel Technology
Краткое описание
Sequential two-layer catalysts were used for the hydrogenolysis of glycerol to remove its oxygen content in a continuous-flow fixed-bed reactor. The acidic H-β catalyst layer was packed before the Ni/Al2O3 catalyst layer in the reactor. The sequential two-layer catalysts can provide good 1-propanol (1-PO) selectivities at high glycerol conversions (up to 69% selectivity at ∼100% conversion). To our knowledge, the catalytic system in this work presented one of the best selectivities to 1-PO using non-noble metal based catalytic systems. A preliminary mechanistic study indicated that most of 1-PO in the products was generated from glycerol via a “sequential two-time dehydration-hydrogenation” mechanism.
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ГОСТ
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Lin X. et al. Hydrogenolysis of Glycerol by the Combined Use of Zeolite and Ni/Al2O3 as Catalysts: A Route for Achieving High Selectivity to 1-Propanol // Energy & Fuels. 2014. Vol. 28. No. 5. pp. 3345-3351.
ГОСТ со всеми авторами (до 50)
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Lin X., LV Y., Xi Y., Qu Y., Phillips D. L., Liu C. Hydrogenolysis of Glycerol by the Combined Use of Zeolite and Ni/Al2O3 as Catalysts: A Route for Achieving High Selectivity to 1-Propanol // Energy & Fuels. 2014. Vol. 28. No. 5. pp. 3345-3351.
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RIS
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TY - JOUR
DO - 10.1021/ef500147k
UR - https://doi.org/10.1021/ef500147k
TI - Hydrogenolysis of Glycerol by the Combined Use of Zeolite and Ni/Al2O3 as Catalysts: A Route for Achieving High Selectivity to 1-Propanol
T2 - Energy & Fuels
AU - Lin, Xufeng
AU - LV, YANHONG
AU - Xi, Yanyan
AU - Qu, Yuanyuan
AU - Phillips, David Lee
AU - Liu, Chenguang
PY - 2014
DA - 2014/04/25
PB - American Chemical Society (ACS)
SP - 3345-3351
IS - 5
VL - 28
SN - 0887-0624
SN - 1520-5029
ER -
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BibTex (до 50 авторов)
Скопировать
@article{2014_Lin,
author = {Xufeng Lin and YANHONG LV and Yanyan Xi and Yuanyuan Qu and David Lee Phillips and Chenguang Liu},
title = {Hydrogenolysis of Glycerol by the Combined Use of Zeolite and Ni/Al2O3 as Catalysts: A Route for Achieving High Selectivity to 1-Propanol},
journal = {Energy & Fuels},
year = {2014},
volume = {28},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/ef500147k},
number = {5},
pages = {3345--3351},
doi = {10.1021/ef500147k}
}
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MLA
Скопировать
Lin, Xufeng, et al. “Hydrogenolysis of Glycerol by the Combined Use of Zeolite and Ni/Al2O3 as Catalysts: A Route for Achieving High Selectivity to 1-Propanol.” Energy & Fuels, vol. 28, no. 5, Apr. 2014, pp. 3345-3351. https://doi.org/10.1021/ef500147k.