Magnetism of Cyano-Bridged Hetero-One-Dimensional Ln3+−M3+ Complexes (Ln3+ = Sm, Gd, Yb; M3+ = FeLS, Co)
Publication type: Journal Article
Publication date: 2003-07-19
scimago Q1
wos Q1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
12924899
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
The reaction of Ln(NO3)3·aq with K3[Fe(CN)6] or K3[Co(CN)6] and 2,2‘-bipyridine in water led to five one-dimensional complexes: trans-[M(CN)4(μ-CN)2Ln(H2O)4 (bpy)]n·XnH2O·1.5nbpy (M = Fe3+ or Co3+; Ln = Sm3+, Gd3+, or Yb3+; X = 4 or 5). The structures for [Fe3+−Sm3+] (1), [Fe3+−Gd3+] (2), [Fe3+−Yb3+] (3), [Co3+−Gd3+] (4), and [Co3+−Yb3+] (5) have been solved; they crystallize in the triclinic space P1̄ and are isomorphous. The [Fe3+−Sm3+] complex is a ferrimagnet, its magnetic studies suggesting the onset of weak ferromagnetic 3-D ordering at 3.5 K. The [Fe3+−Gd3+] interaction is weakly antiferromagnetic. The isotropic nature of Gd3+ allowed us to evaluate the exchange interaction (J = 0.77 cm-1).
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Figuerola A. et al. Magnetism of Cyano-Bridged Hetero-One-Dimensional Ln3+−M3+ Complexes (Ln3+ = Sm, Gd, Yb; M3+ = FeLS, Co) // Inorganic Chemistry. 2003. Vol. 42. No. 17. pp. 5274-5281.
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Figuerola A., Diaz C., Ribas J., Tangoulis V., Sangregorio C., Gatteschi D., Mourino A., Mahía J. Magnetism of Cyano-Bridged Hetero-One-Dimensional Ln3+−M3+ Complexes (Ln3+ = Sm, Gd, Yb; M3+ = FeLS, Co) // Inorganic Chemistry. 2003. Vol. 42. No. 17. pp. 5274-5281.
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TY - JOUR
DO - 10.1021/ic034051j
UR - https://doi.org/10.1021/ic034051j
TI - Magnetism of Cyano-Bridged Hetero-One-Dimensional Ln3+−M3+ Complexes (Ln3+ = Sm, Gd, Yb; M3+ = FeLS, Co)
T2 - Inorganic Chemistry
AU - Figuerola, Albert
AU - Diaz, Carmen
AU - Ribas, Joan
AU - Tangoulis, Vassilis
AU - Sangregorio, Claudio
AU - Gatteschi, Dante
AU - Mourino, A.
AU - Mahía, José
PY - 2003
DA - 2003/07/19
PB - American Chemical Society (ACS)
SP - 5274-5281
IS - 17
VL - 42
PMID - 12924899
SN - 0020-1669
SN - 1520-510X
ER -
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@article{2003_Figuerola,
author = {Albert Figuerola and Carmen Diaz and Joan Ribas and Vassilis Tangoulis and Claudio Sangregorio and Dante Gatteschi and A. Mourino and José Mahía},
title = {Magnetism of Cyano-Bridged Hetero-One-Dimensional Ln3+−M3+ Complexes (Ln3+ = Sm, Gd, Yb; M3+ = FeLS, Co)},
journal = {Inorganic Chemistry},
year = {2003},
volume = {42},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/ic034051j},
number = {17},
pages = {5274--5281},
doi = {10.1021/ic034051j}
}
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Figuerola, Albert, et al. “Magnetism of Cyano-Bridged Hetero-One-Dimensional Ln3+−M3+ Complexes (Ln3+ = Sm, Gd, Yb; M3+ = FeLS, Co).” Inorganic Chemistry, vol. 42, no. 17, Jul. 2003, pp. 5274-5281. https://doi.org/10.1021/ic034051j.