Oligomerization of Fischer−Tropsch Olefins: Effect of Feed and Operating Conditions on Hydrogenated Motor-Gasoline Quality
1
Fischer−Tropsch Refinery Catalysis, Sasol Technology Research and Development, P.O. Box 1, Sasolburg 1947, South Africa
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Publication type: Journal Article
Publication date: 2004-10-15
scimago Q1
wos Q2
SJR: 0.828
CiteScore: 6.7
Impact factor: 3.9
ISSN: 08885885, 15205045
General Chemistry
General Chemical Engineering
Industrial and Manufacturing Engineering
Abstract
Oligomerization of Fischer−Tropsch-derived olefins over a solid phosphoric acid catalyst was studied to improve the quality of the hydrogenated motor-gasoline. It was shown that, with a narrow-cut Fischer−Tropsch butene mixture, rich in 1-butene and low in isobutene, a hydrogenated motor-gasoline with an RON and an MON of 86−88 could be produced at 80% olefin conversion. The influence of propene and pentenes was investigated, and a reactivity sequence for C3−C5 mixtures could be established: isobutene > methylbutenes > n-butenes = propene > n-pentenes. It was noted that 1-butene was closer in behavior to isobutene than to 2-butene and had to be treated as such to yield the highest-quality product. It was advantageous to oligomerize 1-butene-rich feed at 160 °C or less and to exclude propene and n-pentenes from the reaction mixture. These effects could be explained.
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Citations from 2024:
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(6%)
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GOST
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De Klerk A., Engelbrecht D. J., Boikanyo H. Oligomerization of Fischer−Tropsch Olefins: Effect of Feed and Operating Conditions on Hydrogenated Motor-Gasoline Quality // Industrial & Engineering Chemistry Research. 2004. Vol. 43. No. 23. pp. 7449-7455.
GOST all authors (up to 50)
Copy
De Klerk A., Engelbrecht D. J., Boikanyo H. Oligomerization of Fischer−Tropsch Olefins: Effect of Feed and Operating Conditions on Hydrogenated Motor-Gasoline Quality // Industrial & Engineering Chemistry Research. 2004. Vol. 43. No. 23. pp. 7449-7455.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/ie0495675
UR - https://doi.org/10.1021/ie0495675
TI - Oligomerization of Fischer−Tropsch Olefins: Effect of Feed and Operating Conditions on Hydrogenated Motor-Gasoline Quality
T2 - Industrial & Engineering Chemistry Research
AU - De Klerk, Arno
AU - Engelbrecht, Dan J
AU - Boikanyo, Herman
PY - 2004
DA - 2004/10/15
PB - American Chemical Society (ACS)
SP - 7449-7455
IS - 23
VL - 43
SN - 0888-5885
SN - 1520-5045
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2004_De Klerk,
author = {Arno De Klerk and Dan J Engelbrecht and Herman Boikanyo},
title = {Oligomerization of Fischer−Tropsch Olefins: Effect of Feed and Operating Conditions on Hydrogenated Motor-Gasoline Quality},
journal = {Industrial & Engineering Chemistry Research},
year = {2004},
volume = {43},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/ie0495675},
number = {23},
pages = {7449--7455},
doi = {10.1021/ie0495675}
}
Cite this
MLA
Copy
De Klerk, Arno, et al. “Oligomerization of Fischer−Tropsch Olefins: Effect of Feed and Operating Conditions on Hydrogenated Motor-Gasoline Quality.” Industrial & Engineering Chemistry Research, vol. 43, no. 23, Oct. 2004, pp. 7449-7455. https://doi.org/10.1021/ie0495675.