Journal of the American Chemical Society, volume 135, issue 3, pages 975-978

Anomalous High Ionic Conductivity of Nanoporous β-Li3PS4

Zengcai Liu ¹

Wujun Fu ¹

E.Andrew Payzant ^{1, 2}

Xiang Yu ¹

Zili Wu ^{1, 3}

Nancy J. Dudney ²

Jim Kiggans ²

Kunlun Hong ¹

Adam J. Rondinone ¹

Chengdu Liang ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, United States |

Materials Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, United States |

Chemical Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37830, United States |

Publication type: Journal Article

Publication date: 2013-01-14

American Chemical Society (ACS)

Journal: Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

Impact factor: 15

ISSN: 00027863, 15205126

DOI: 10.1021/ja3110895

Copy DOI

General Chemistry

Catalysis

Biochemistry

Colloid and Surface Chemistry

Abstract

Lithium-ion-conducting solid electrolytes hold promise for enabling high-energy battery chemistries and circumventing safety issues of conventional lithium batteries. Achieving the combination of high ionic conductivity and a broad electrochemical window in solid electrolytes is a grand challenge for the synthesis of battery materials. Herein we show an enhancement of the room-temperature lithium-ion conductivity by 3 orders of magnitude through the creation of nanostructured Li(3)PS(4). This material has a wide electrochemical window (5 V) and superior chemical stability against lithium metal. The nanoporous structure of Li(3)PS(4) reconciles two vital effects that enhance the ionic conductivity: (1) the reduction of the dimensions to a nanometer-sized framework stabilizes the high-conduction β phase that occurs at elevated temperatures, and (2) the high surface-to-bulk ratio of nanoporous β-Li(3)PS(4) promotes surface conduction. Manipulating the ionic conductivity of solid electrolytes has far-reaching implications for materials design and synthesis in a broad range of applications, including batteries, fuel cells, sensors, photovoltaic systems, and so forth.

By date By citations

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Citations by journals

	5 10 15 20 25 30 35 40
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 40, 5.59% Journal of Materials Chemistry A 40 publications, 5.59%
Chemistry of Materials	Chemistry of Materials, 39, 5.45% Chemistry of Materials 39 publications, 5.45%
ACS applied materials & interfaces	ACS applied materials & interfaces, 38, 5.31% ACS applied materials & interfaces 38 publications, 5.31%
Advanced Energy Materials	Advanced Energy Materials, 33, 4.62% Advanced Energy Materials 33 publications, 4.62%
Journal of Power Sources	Journal of Power Sources, 29, 4.06% Journal of Power Sources 29 publications, 4.06%
Energy Storage Materials	Energy Storage Materials, 23, 3.22% Energy Storage Materials 23 publications, 3.22%
Solid State Ionics	Solid State Ionics, 16, 2.24% Solid State Ionics 16 publications, 2.24%
ACS Applied Energy Materials	ACS Applied Energy Materials, 14, 1.96% ACS Applied Energy Materials 14 publications, 1.96%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 13, 1.82% Journal of the Electrochemical Society 13 publications, 1.82%
Advanced Functional Materials	Advanced Functional Materials, 12, 1.68% Advanced Functional Materials 12 publications, 1.68%
Energy and Environmental Science	Energy and Environmental Science, 12, 1.68% Energy and Environmental Science 12 publications, 1.68%
Inorganic Chemistry	Inorganic Chemistry, 11, 1.54% Inorganic Chemistry 11 publications, 1.54%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 11, 1.54% Journal of Physical Chemistry C 11 publications, 1.54%
ACS Energy Letters	ACS Energy Letters, 10, 1.4% ACS Energy Letters 10 publications, 1.4%
Advanced Materials	Advanced Materials, 10, 1.4% Advanced Materials 10 publications, 1.4%
Small	Small, 9, 1.26% Small 9 publications, 1.26%
Journal of the American Chemical Society	Journal of the American Chemical Society, 9, 1.26% Journal of the American Chemical Society 9 publications, 1.26%
Nature Communications	Nature Communications, 8, 1.12% Nature Communications 8 publications, 1.12%
Chemical Reviews	Chemical Reviews, 8, 1.12% Chemical Reviews 8 publications, 1.12%
Scientific Reports	Scientific Reports, 8, 1.12% Scientific Reports 8 publications, 1.12%
Chemical Communications	Chemical Communications, 8, 1.12% Chemical Communications 8 publications, 1.12%
Journal of Energy Storage	Journal of Energy Storage, 7, 0.98% Journal of Energy Storage 7 publications, 0.98%
Frontiers in Energy Research	Frontiers in Energy Research, 7, 0.98% Frontiers in Energy Research 7 publications, 0.98%
Nano Energy	Nano Energy, 7, 0.98% Nano Energy 7 publications, 0.98%
Angewandte Chemie	Angewandte Chemie, 7, 0.98% Angewandte Chemie 7 publications, 0.98%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 7, 0.98% Angewandte Chemie - International Edition 7 publications, 0.98%
Batteries & Supercaps	Batteries & Supercaps, 7, 0.98% Batteries & Supercaps 7 publications, 0.98%
Nano Letters	Nano Letters, 6, 0.84% Nano Letters 6 publications, 0.84%
Chemical Engineering Journal	Chemical Engineering Journal, 6, 0.84% Chemical Engineering Journal 6 publications, 0.84%
	5 10 15 20 25 30 35 40

Citations by publishers

	20 40 60 80 100 120 140 160 180
American Chemical Society (ACS)	American Chemical Society (ACS), 169, 23.64% American Chemical Society (ACS) 169 publications, 23.64%
Elsevier	Elsevier, 160, 22.38% Elsevier 160 publications, 22.38%
Wiley	Wiley, 134, 18.74% Wiley 134 publications, 18.74%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 92, 12.87% Royal Society of Chemistry (RSC) 92 publications, 12.87%
Springer Nature	Springer Nature, 59, 8.25% Springer Nature 59 publications, 8.25%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 19, 2.66% Multidisciplinary Digital Publishing Institute (MDPI) 19 publications, 2.66%
The Electrochemical Society	The Electrochemical Society, 13, 1.82% The Electrochemical Society 13 publications, 1.82%
Frontiers Media S.A.	Frontiers Media S.A., 7, 0.98% Frontiers Media S.A. 7 publications, 0.98%
American Physical Society (APS)	American Physical Society (APS), 6, 0.84% American Physical Society (APS) 6 publications, 0.84%
IOP Publishing	IOP Publishing, 5, 0.7% IOP Publishing 5 publications, 0.7%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 4, 0.56% American Institute of Physics (AIP) 4 publications, 0.56%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 4, 0.56% American Association for the Advancement of Science (AAAS) 4 publications, 0.56%
Cambridge University Press	Cambridge University Press, 3, 0.42% Cambridge University Press 3 publications, 0.42%
Walter de Gruyter	Walter de Gruyter, 3, 0.42% Walter de Gruyter 3 publications, 0.42%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 3, 0.42% Proceedings of the National Academy of Sciences (PNAS) 3 publications, 0.42%
The Chemical Society of Japan	The Chemical Society of Japan, 2, 0.28% The Chemical Society of Japan 2 publications, 0.28%
World Scientific	World Scientific, 2, 0.28% World Scientific 2 publications, 0.28%
Pleiades Publishing	Pleiades Publishing, 2, 0.28% Pleiades Publishing 2 publications, 0.28%
Funtai Funmatsu Yakin Kyokai	Funtai Funmatsu Yakin Kyokai, 2, 0.28% Funtai Funmatsu Yakin Kyokai 2 publications, 0.28%
Chinese Physical Society	Chinese Physical Society, 2, 0.28% Chinese Physical Society 2 publications, 0.28%
OAE Publishing Inc.	OAE Publishing Inc., 2, 0.28% OAE Publishing Inc. 2 publications, 0.28%
EDP Sciences	EDP Sciences, 1, 0.14% EDP Sciences 1 publication, 0.14%
The Royal Society	The Royal Society, 1, 0.14% The Royal Society 1 publication, 0.14%
Ceramic Society of Japan	Ceramic Society of Japan, 1, 0.14% Ceramic Society of Japan 1 publication, 0.14%
Korean Institute of Metals and Materials	Korean Institute of Metals and Materials, 1, 0.14% Korean Institute of Metals and Materials 1 publication, 0.14%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.14% Nonferrous Metals Society of China 1 publication, 0.14%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 1, 0.14% Korean Society of Industrial Engineering Chemistry 1 publication, 0.14%
Chinese Ceramic Society	Chinese Ceramic Society, 1, 0.14% Chinese Ceramic Society 1 publication, 0.14%
Social Science Electronic Publishing	Social Science Electronic Publishing, 1, 0.14% Social Science Electronic Publishing 1 publication, 0.14%
	20 40 60 80 100 120 140 160 180

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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GOST Copy

Liu Z. et al. Anomalous High Ionic Conductivity of Nanoporous β-Li3PS4 // Journal of the American Chemical Society. 2013. Vol. 135. No. 3. pp. 975-978.

GOST all authors (up to 50) Copy

Liu Z., Fu W., Payzant E., Yu X., Wu Z., Dudney N. J., Kiggans J., Hong K., Rondinone A. J., Liang C. Anomalous High Ionic Conductivity of Nanoporous β-Li3PS4 // Journal of the American Chemical Society. 2013. Vol. 135. No. 3. pp. 975-978.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/ja3110895

UR - https://doi.org/10.1021/ja3110895

TI - Anomalous High Ionic Conductivity of Nanoporous β-Li3PS4

T2 - Journal of the American Chemical Society

AU - Fu, Wujun

AU - Payzant, E.Andrew

AU - Kiggans, Jim

AU - Liu, Zengcai

AU - Yu, Xiang

AU - Wu, Zili

AU - Dudney, Nancy J.

AU - Hong, Kunlun

AU - Rondinone, Adam J.

AU - Liang, Chengdu

PY - 2013

DA - 2013/01/14 00:00:00

PB - American Chemical Society (ACS)

SP - 975-978

IS - 3

VL - 135

SN - 0002-7863

SN - 1520-5126

ER -

BibTex |

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BibTex Copy

@article{2013_Liu,

author = {Wujun Fu and E.Andrew Payzant and Jim Kiggans and Zengcai Liu and Xiang Yu and Zili Wu and Nancy J. Dudney and Kunlun Hong and Adam J. Rondinone and Chengdu Liang},

title = {Anomalous High Ionic Conductivity of Nanoporous β-Li3PS4},

journal = {Journal of the American Chemical Society},

year = {2013},

volume = {135},

publisher = {American Chemical Society (ACS)},

month = {jan},

url = {https://doi.org/10.1021/ja3110895},

number = {3},

pages = {975--978},

doi = {10.1021/ja3110895}

}

MLA

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MLA Copy

Liu, Zengcai, et al. “Anomalous High Ionic Conductivity of Nanoporous β-Li3PS4.” Journal of the American Chemical Society, vol. 135, no. 3, Jan. 2013, pp. 975-978. https://doi.org/10.1021/ja3110895.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

Impact factor

ISSN

00027863 (Print)
15205126 (Electronic)