C60 Cluster as an Electron Shuttle in a Ru(II)-Polypyridyl Sensitizer-Based Photochemical Solar Cell
Тип публикации: Journal Article
Дата публикации: 2004-04-01
scimago Q1
wos Q3
БС2
SJR: 0.742
CiteScore: 5.3
Impact factor: 2.9
ISSN: 15206106, 15205207, 10895647
Materials Chemistry
Surfaces, Coatings and Films
Physical and Theoretical Chemistry
Краткое описание
The interaction between the excited sensitizer and the redox couple in a photochemical solar cell is an important factor that can decrease the photon-conversion efficiency. We have now employed C60 clusters to separate the Ru(bpy)2(dcbpy)2+ (Ru(II) complex) and I3-/I- couple to minimize the sensitizer−redox couple interactions. The C60-modified electrodes (viz., OTE/SnO2/Ru(II)/C60 and OTE/TiO2/Ru(II)/C60) delivered photocurrent with greater efficiency than did the SnO2 and TiO2 films modified with only a Ru(II) dye (viz., OTE/SnO2/Ru(II) and OTE/TiO2/Ru(II)). The luminescence quenching of Ru(II)* by I3-, which occurs with a rate constant of 1.9 × 1010 M-1 s-1, is suppressed following the deposition of a layer of C60 clusters. This paper presents a novel concept of employing a redox-active molecular assembly as an electron relay that greatly minimizes the interaction with the excited dye while maintaining the effectiveness of the regeneration cycle.
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Kamat P. V., Haria M., Hotchandani S. C60 Cluster as an Electron Shuttle in a Ru(II)-Polypyridyl Sensitizer-Based Photochemical Solar Cell // Journal of Physical Chemistry B. 2004. Vol. 108. No. 17. pp. 5166-5170.
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Kamat P. V., Haria M., Hotchandani S. C60 Cluster as an Electron Shuttle in a Ru(II)-Polypyridyl Sensitizer-Based Photochemical Solar Cell // Journal of Physical Chemistry B. 2004. Vol. 108. No. 17. pp. 5166-5170.
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TY - JOUR
DO - 10.1021/jp0496699
UR - https://doi.org/10.1021/jp0496699
TI - C60 Cluster as an Electron Shuttle in a Ru(II)-Polypyridyl Sensitizer-Based Photochemical Solar Cell
T2 - Journal of Physical Chemistry B
AU - Kamat, Prashant V.
AU - Haria, Mehul
AU - Hotchandani, Surat
PY - 2004
DA - 2004/04/01
PB - American Chemical Society (ACS)
SP - 5166-5170
IS - 17
VL - 108
SN - 1520-6106
SN - 1520-5207
SN - 1089-5647
ER -
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@article{2004_Kamat,
author = {Prashant V. Kamat and Mehul Haria and Surat Hotchandani},
title = {C60 Cluster as an Electron Shuttle in a Ru(II)-Polypyridyl Sensitizer-Based Photochemical Solar Cell},
journal = {Journal of Physical Chemistry B},
year = {2004},
volume = {108},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/jp0496699},
number = {17},
pages = {5166--5170},
doi = {10.1021/jp0496699}
}
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Kamat, Prashant V., et al. “C60 Cluster as an Electron Shuttle in a Ru(II)-Polypyridyl Sensitizer-Based Photochemical Solar Cell.” Journal of Physical Chemistry B, vol. 108, no. 17, Apr. 2004, pp. 5166-5170. https://doi.org/10.1021/jp0496699.