Temperature-Induced Modifications of PdZn Layers on Pd(111)
Тип публикации: Journal Article
Дата публикации: 2010-05-28
scimago Q1
wos Q3
БС1
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Краткое описание
Ultrathin PdZn surface alloys on Pd(111) are model systems well-suited for obtaining a microscopic understanding of the mechanisms of Pd/Zn-based catalysis for methanol steam reforming. The temperature-induced compositional and structural changes of these alloy films are investigated in the catalytically relevant temperature range. Heating of multilayer Zn films to 500 K results in the formation of multilayer PdZn alloy films with surface and near-surface composition close to 1:1. In the temperature regime above 550 K the subsurface layers deplete quickly in Zn due to diffusion of Zn atoms into the Pd bulk. In contrast, the composition of the surface layer changes only slightly, indicating formation of a PdZn film with strong monolayer character. This change in subsurface composition triggers a change of the original Zn-out/Pd-in surface corrugation, leading ultimately to a Pd-out/Zn-in situation for annealing temperatures beyond 700 K. The altered corrugation pattern is also obtained when submonolayer am...
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Stadlmayr W. et al. Temperature-Induced Modifications of PdZn Layers on Pd(111) // Journal of Physical Chemistry C. 2010. Vol. 114. No. 24. pp. 10850-10856.
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Stadlmayr W., Rameshan C., Weilach C., Lorenz H., Hävecker M., Blume R., Rocha T. C. R., Teschner D., KNOP-GERICKE A., Zemlyanov D., Penner S., Schlögl R., Rupprechter G., Klötzer B., Memmel N. Temperature-Induced Modifications of PdZn Layers on Pd(111) // Journal of Physical Chemistry C. 2010. Vol. 114. No. 24. pp. 10850-10856.
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TY - JOUR
DO - 10.1021/jp1008835
UR - https://doi.org/10.1021/jp1008835
TI - Temperature-Induced Modifications of PdZn Layers on Pd(111)
T2 - Journal of Physical Chemistry C
AU - Stadlmayr, W.
AU - Rameshan, Christoph
AU - Weilach, Ch
AU - Lorenz, H.
AU - Hävecker, M.
AU - Blume, R.
AU - Rocha, Tulio C. R.
AU - Teschner, D
AU - KNOP-GERICKE, A.
AU - Zemlyanov, D
AU - Penner, Simon
AU - Schlögl, R.
AU - Rupprechter, Günther
AU - Klötzer, Bernhard
AU - Memmel, Norbert
PY - 2010
DA - 2010/05/28
PB - American Chemical Society (ACS)
SP - 10850-10856
IS - 24
VL - 114
SN - 1932-7447
SN - 1932-7455
ER -
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@article{2010_Stadlmayr,
author = {W. Stadlmayr and Christoph Rameshan and Ch Weilach and H. Lorenz and M. Hävecker and R. Blume and Tulio C. R. Rocha and D Teschner and A. KNOP-GERICKE and D Zemlyanov and Simon Penner and R. Schlögl and Günther Rupprechter and Bernhard Klötzer and Norbert Memmel},
title = {Temperature-Induced Modifications of PdZn Layers on Pd(111)},
journal = {Journal of Physical Chemistry C},
year = {2010},
volume = {114},
publisher = {American Chemical Society (ACS)},
month = {may},
url = {https://doi.org/10.1021/jp1008835},
number = {24},
pages = {10850--10856},
doi = {10.1021/jp1008835}
}
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Stadlmayr, W., et al. “Temperature-Induced Modifications of PdZn Layers on Pd(111).” Journal of Physical Chemistry C, vol. 114, no. 24, May. 2010, pp. 10850-10856. https://doi.org/10.1021/jp1008835.