Reasons for the Differences in the Kinetics of Thermal Oxidation of the Support in Pt/C Electrocatalysts
Тип публикации: Journal Article
Дата публикации: 2014-10-06
scimago Q1
wos Q3
БС1
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Краткое описание
High-temperature oxidation processes of carbon microparticles Vulcan XC72 coated with platinum nanoparticles (Pt/C) were studied by thermogravimetric analysis (TGA) and differential scanning calorimetry (DSC). The presence of different specific temperature ranges in the oxidation of carbon support was shown to be due to both the peculiarities of granulometric composition of carbon black microparticles, different size, and uneven spatial distribution of platinum nanoparticles in the pores and on the surface of the carbon support. The correlation between the length of a section in the thermograms and the fraction of carbon microparticles poorly coated with platinum can be used to analyze the uniformity of Pt nanoparticle spatial distribution in the metal–carbon catalysts and therefore to select electrocatalysts with optimal microstructure. This analysis is expected to be effectively utilized in order to assess the uniformity of platinum distribution on carbon microparticles and also to provide additional in...
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Guterman V. E. et al. Reasons for the Differences in the Kinetics of Thermal Oxidation of the Support in Pt/C Electrocatalysts // Journal of Physical Chemistry C. 2014. Vol. 118. No. 41. pp. 23835-23844.
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Guterman V. E., Belenov S., Krikov V. V., Vysochina L. L., Yohannes W., Tabachkova N. Yu., Balakshina E. N. Reasons for the Differences in the Kinetics of Thermal Oxidation of the Support in Pt/C Electrocatalysts // Journal of Physical Chemistry C. 2014. Vol. 118. No. 41. pp. 23835-23844.
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TY - JOUR
DO - 10.1021/jp507801f
UR - https://doi.org/10.1021/jp507801f
TI - Reasons for the Differences in the Kinetics of Thermal Oxidation of the Support in Pt/C Electrocatalysts
T2 - Journal of Physical Chemistry C
AU - Guterman, V. E.
AU - Belenov, Sergey
AU - Krikov, Vladimir V
AU - Vysochina, Larisa L
AU - Yohannes, Weldegebriel
AU - Tabachkova, Natalya Yu
AU - Balakshina, Elena N
PY - 2014
DA - 2014/10/06
PB - American Chemical Society (ACS)
SP - 23835-23844
IS - 41
VL - 118
SN - 1932-7447
SN - 1932-7455
ER -
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@article{2014_Guterman,
author = {V. E. Guterman and Sergey Belenov and Vladimir V Krikov and Larisa L Vysochina and Weldegebriel Yohannes and Natalya Yu Tabachkova and Elena N Balakshina},
title = {Reasons for the Differences in the Kinetics of Thermal Oxidation of the Support in Pt/C Electrocatalysts},
journal = {Journal of Physical Chemistry C},
year = {2014},
volume = {118},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/jp507801f},
number = {41},
pages = {23835--23844},
doi = {10.1021/jp507801f}
}
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MLA
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Guterman, V. E., et al. “Reasons for the Differences in the Kinetics of Thermal Oxidation of the Support in Pt/C Electrocatalysts.” Journal of Physical Chemistry C, vol. 118, no. 41, Oct. 2014, pp. 23835-23844. https://doi.org/10.1021/jp507801f.