Journal of Physical Chemistry B, volume 102, issue 2, pages 372-375
Relationship between Activation Energy and Bottleneck Size for Li+ Ion Conduction in NASICON Materials of Composition LiMM‘(PO4)3; M, M‘ = Ge, Ti, Sn, Hf
1
Instituto Ciencia de Materiales de Madrid, Consejo Superior de Investigaciones Científicas (CSIC), Cantoblanco, 28049 Madrid, Spain
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Publication type: Journal Article
Publication date: 1998-01-01
Journal:
Journal of Physical Chemistry B
Quartile SCImago
Q1
Quartile WOS
Q3
Impact factor: 3.3
ISSN: 15206106, 15205207
Materials Chemistry
Surfaces, Coatings and Films
Physical and Theoretical Chemistry
Abstract
The activation energy involved in the motion of Li+ ions along the conduction channels of the NASICON framework has been determined from electrical conductivity measurements in samples of composition LiM2(PO4)3 and LiMM‘(PO4)3, where M and M‘ are Ge, Ti, Sn, and Hf, all compounds belonging to space group R3c. Two lithium sites, M1 and M2, inside the channels, can be distinguished. The sites are connected through triangular bottlenecks of oxygen atoms, and the size of the bottleneck has been estimated from refined and simulated structures for each composition. The plot of activation energy vs bottleneck size shows two regimes: for sizes up to 2.04 A the activation energy decreases steeply, but above 2.04 A the activation energy is almost constant. These regimes are discussed on the basis of the effective Li+ ionic radius for the compounds analyzed.
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35
40
45
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Martínez Juárez A. et al. Relationship between Activation Energy and Bottleneck Size for Li+ Ion Conduction in NASICON Materials of Composition LiMM‘(PO4)3; M, M‘ = Ge, Ti, Sn, Hf // Journal of Physical Chemistry B. 1998. Vol. 102. No. 2. pp. 372-375.
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Martínez Juárez A., Pecharroman C., Iglesias J. E., Ribeiro A. P. C. Relationship between Activation Energy and Bottleneck Size for Li+ Ion Conduction in NASICON Materials of Composition LiMM‘(PO4)3; M, M‘ = Ge, Ti, Sn, Hf // Journal of Physical Chemistry B. 1998. Vol. 102. No. 2. pp. 372-375.
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TY - JOUR
DO - 10.1021/jp973296c
UR - https://doi.org/10.1021/jp973296c
TI - Relationship between Activation Energy and Bottleneck Size for Li+ Ion Conduction in NASICON Materials of Composition LiMM‘(PO4)3; M, M‘ = Ge, Ti, Sn, Hf
T2 - Journal of Physical Chemistry B
AU - Martínez Juárez, Ana
AU - Iglesias, Juan E
AU - Pecharroman, Carlos
AU - Ribeiro, A. P. C.
PY - 1998
DA - 1998/01/01 00:00:00
PB - American Chemical Society (ACS)
SP - 372-375
IS - 2
VL - 102
SN - 1520-6106
SN - 1520-5207
ER -
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@article{1998_Martínez Juárez,
author = {Ana Martínez Juárez and Juan E Iglesias and Carlos Pecharroman and A. P. C. Ribeiro},
title = {Relationship between Activation Energy and Bottleneck Size for Li+ Ion Conduction in NASICON Materials of Composition LiMM‘(PO4)3; M, M‘ = Ge, Ti, Sn, Hf},
journal = {Journal of Physical Chemistry B},
year = {1998},
volume = {102},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/jp973296c},
number = {2},
pages = {372--375},
doi = {10.1021/jp973296c}
}
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Martínez Juárez, Ana, et al. “Relationship between Activation Energy and Bottleneck Size for Li+ Ion Conduction in NASICON Materials of Composition LiMM‘(PO4)3; M, M‘ = Ge, Ti, Sn, Hf.” Journal of Physical Chemistry B, vol. 102, no. 2, Jan. 1998, pp. 372-375. https://doi.org/10.1021/jp973296c.