Mechanical Oscillation Coupled with the Belousov−Zhabotinsky Reaction in Gel
Publication type: Journal Article
Publication date: 2003-06-10
scimago Q1
wos Q2
SJR: 0.763
CiteScore: 6.0
Impact factor: 3.9
ISSN: 07437463, 15205827
Spectroscopy
Electrochemistry
Condensed Matter Physics
General Materials Science
Surfaces and Interfaces
Abstract
We succeed in measuring the oscillating force of cylindrical poly(N-isopropylacrylamide) gel having a side group of ruthenium tris(2,2‘-bipyridine) (Ru(bpy)3) accompanied with the periodic redox reaction of Ru(bpy)32+/3+, the Belousov−Zhabotinsky (BZ) reaction. The measurements are made for three gels with different diameters, 0.65, 1.17, and 1.88 mm, at 15 °C. It is found that the amplitude of oscillatory tensile stress of the reacting cylindrical gel with a diameter of 0.65 mm is much higher than the stress theoretically expected from the Donnan osmotic pressure. The amplitude is explained by an oscillatory change of the interaction parameter, χ, which might be induced by the hydration and dehydration of the chain due to the oscillatory charge density on the polymer chain. The oscillation behavior of the BZ reaction is found to be strongly dependent on the diameter of the gel. The staying period in the oxidative state and the period of the oscillation increase with a decrease in the diameter of the cylindrical gel.
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GOST
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SASAKI S. et al. Mechanical Oscillation Coupled with the Belousov−Zhabotinsky Reaction in Gel // Langmuir. 2003. Vol. 19. No. 14. pp. 5595-5600.
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SASAKI S., Koga S., Yoshida R., Yamaguchi T. Mechanical Oscillation Coupled with the Belousov−Zhabotinsky Reaction in Gel // Langmuir. 2003. Vol. 19. No. 14. pp. 5595-5600.
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RIS
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TY - JOUR
DO - 10.1021/la0270035
UR - https://doi.org/10.1021/la0270035
TI - Mechanical Oscillation Coupled with the Belousov−Zhabotinsky Reaction in Gel
T2 - Langmuir
AU - SASAKI, Shigeo
AU - Koga, Shogo
AU - Yoshida, Ryo
AU - Yamaguchi, Tomohiko
PY - 2003
DA - 2003/06/10
PB - American Chemical Society (ACS)
SP - 5595-5600
IS - 14
VL - 19
SN - 0743-7463
SN - 1520-5827
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2003_SASAKI,
author = {Shigeo SASAKI and Shogo Koga and Ryo Yoshida and Tomohiko Yamaguchi},
title = {Mechanical Oscillation Coupled with the Belousov−Zhabotinsky Reaction in Gel},
journal = {Langmuir},
year = {2003},
volume = {19},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/la0270035},
number = {14},
pages = {5595--5600},
doi = {10.1021/la0270035}
}
Cite this
MLA
Copy
SASAKI, Shigeo, et al. “Mechanical Oscillation Coupled with the Belousov−Zhabotinsky Reaction in Gel.” Langmuir, vol. 19, no. 14, Jun. 2003, pp. 5595-5600. https://doi.org/10.1021/la0270035.