Langmuir, volume 27, issue 11, pages 7294-7300

Photodeposition of Ag₂S Quantum Dots and Application to Photoelectrochemical Cells for Hydrogen Production under Simulated Sunlight

Kazuki Nagasuna ¹

Tomoki Akita ²

Musashi Fujishima ¹

HIROAKI TADA ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

Department of Applied Chemistry, School of Science and Engineering, Kinki University, 3-4-1, Kowakae, Higashi-Osaka, Osaka 577-8502, Japan |

National Institute of Advanced Industrial Science and Technology, Midorigaoka 1-8-31, Ikeda, Osaka 563-8577, Japan |

Publication type: Journal Article

Publication date: 2011-05-09

American Chemical Society (ACS)

Journal: Langmuir

Quartile SCImago

Quartile WOS

Impact factor: 3.9

ISSN: 07437463, 15205827

DOI: 10.1021/la200587s

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Spectroscopy

Electrochemistry

Condensed Matter Physics

General Materials Science

Surfaces and Interfaces

Abstract

UV light irradiation of TiO(2) (λ > 320 nm) in a mixed solution of AgNO(3) and S(8) has led to the formation of Ag(2)S quantum dots (QDs) on TiO(2), while Ag nanoparticles (NPs) are photodeposited without S(8). Photoelectrochemical measurements indicated that the Ag(2)S photodeposition proceeds via the preferential reduction of Ag(+) ions to Ag(0), followed by the chemical reaction with S(8). The application of this in situ photodeposition technique to mesoporous (mp) TiO(2) nanocrystalline films coated on fluorine-doped SnO(2) (FTO) electrodes enables formation of Ag(2)S QDs (Ag(2)S/mp-TiO(2)/FTO). Ag(2)S/mp-TiO(2)/FTO has the interband transition absorption in the whole visible region, while in the spectrum of Ag/mp-TiO(2)/FTO, a localized surface plasmon resonance absorption of Ag NPs is present centered at 490 nm. Ag(2)S QD-sensitized photoelectrochemical cells using the Ag(2)S/mp-TiO(2)/FTO and Ag/mp-TiO(2)/FTO photoanodes were fabricated. Under illumination of one sun, the Ag(2)S photoanode cell yielded H(2) at a rate of 0.8 mL·h(-1) with a total conversion efficiency of 0.29%, whereas the Ag/mp-TiO(2)/FTO photoanode is inactive.

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Nagasuna K. et al. Photodeposition of Ag2S Quantum Dots and Application to Photoelectrochemical Cells for Hydrogen Production under Simulated Sunlight // Langmuir. 2011. Vol. 27. No. 11. pp. 7294-7300.

GOST all authors (up to 50) Copy

Nagasuna K., Akita T., Fujishima M., TADA H. Photodeposition of Ag2S Quantum Dots and Application to Photoelectrochemical Cells for Hydrogen Production under Simulated Sunlight // Langmuir. 2011. Vol. 27. No. 11. pp. 7294-7300.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/la200587s

UR - https://doi.org/10.1021/la200587s

TI - Photodeposition of Ag2S Quantum Dots and Application to Photoelectrochemical Cells for Hydrogen Production under Simulated Sunlight

T2 - Langmuir

AU - Nagasuna, Kazuki

AU - Akita, Tomoki

AU - Fujishima, Musashi

AU - TADA, HIROAKI

PY - 2011

DA - 2011/05/09 00:00:00

PB - American Chemical Society (ACS)

SP - 7294-7300

IS - 11

VL - 27

SN - 0743-7463

SN - 1520-5827

ER -

BibTex |

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BibTex Copy

@article{2011_Nagasuna,

author = {Kazuki Nagasuna and Tomoki Akita and Musashi Fujishima and HIROAKI TADA},

title = {Photodeposition of Ag2S Quantum Dots and Application to Photoelectrochemical Cells for Hydrogen Production under Simulated Sunlight},

journal = {Langmuir},

year = {2011},

volume = {27},

publisher = {American Chemical Society (ACS)},

month = {may},

url = {https://doi.org/10.1021/la200587s},

number = {11},

pages = {7294--7300},

doi = {10.1021/la200587s}

}

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Nagasuna, Kazuki, et al. “Photodeposition of Ag2S Quantum Dots and Application to Photoelectrochemical Cells for Hydrogen Production under Simulated Sunlight.” Langmuir, vol. 27, no. 11, May. 2011, pp. 7294-7300. https://doi.org/10.1021/la200587s.

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Publisher

American Chemical Society (ACS)

Journal

Langmuir

Quartile SCImago

Quartile WOS

Impact factor

3.9

ISSN

07437463 (Print)
15205827 (Electronic)