Adsorption of Sodium Poly(styrenesulfonate) to the Air Surface of Water by Neutron and X-ray Reflectivity and Surface Tension Measurements: Polymer Concentration Dependence
Тип публикации: Journal Article
Дата публикации: 2002-11-14
scimago Q1
wos Q1
БС1
SJR: 1.352
CiteScore: 9
Impact factor: 5.2
ISSN: 00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Краткое описание
The adsorption of the strong polyelectrolyte sodium poly(styrenesulfonate) (NaPSS) to the air surface of water was investigated as a function of polymer concentration from the dilute regime to the beginning of the semidilute regime. Detailed segment profiles of the deuterated polymer were determined by neutron reflection (NR). Data were obtained for 0.67 and 2.50 M KCl. For two samples differing widely in molecular weight (1150 and 56.1 kg/mol), we find that with increasing polymer concentration the adsorbed amount first increases, reaches a maximum, and then decreases strongly. The PSS concentration at which the maximum is reached is dependent on both the molecular weight and the salt concentration in a manner that correlates with the chain overlap concentration. Regarding the segment profiles, at low polymer concentration the profiles are composed of a thin layer of high concentration at the air surface (trains), followed by a distinct second layer of much lower segment concentration that extends to lar...
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YIM H. et al. Adsorption of Sodium Poly(styrenesulfonate) to the Air Surface of Water by Neutron and X-ray Reflectivity and Surface Tension Measurements: Polymer Concentration Dependence // Macromolecules. 2002. Vol. 35. No. 26. pp. 9737-9747.
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YIM H., Kent M. L., Matheson A., Stevens M., Ivkov R., Satija S., Majewski J., Smith G. S. Adsorption of Sodium Poly(styrenesulfonate) to the Air Surface of Water by Neutron and X-ray Reflectivity and Surface Tension Measurements: Polymer Concentration Dependence // Macromolecules. 2002. Vol. 35. No. 26. pp. 9737-9747.
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TY - JOUR
DO - 10.1021/ma0200468
UR - https://doi.org/10.1021/ma0200468
TI - Adsorption of Sodium Poly(styrenesulfonate) to the Air Surface of Water by Neutron and X-ray Reflectivity and Surface Tension Measurements: Polymer Concentration Dependence
T2 - Macromolecules
AU - YIM, H.
AU - Kent, M. L.
AU - Matheson, A.
AU - Stevens, Mark
AU - Ivkov, Robert
AU - Satija, S.
AU - Majewski, Jaroslaw
AU - Smith, G S
PY - 2002
DA - 2002/11/14
PB - American Chemical Society (ACS)
SP - 9737-9747
IS - 26
VL - 35
SN - 0024-9297
SN - 1520-5835
ER -
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@article{2002_YIM,
author = {H. YIM and M. L. Kent and A. Matheson and Mark Stevens and Robert Ivkov and S. Satija and Jaroslaw Majewski and G S Smith},
title = {Adsorption of Sodium Poly(styrenesulfonate) to the Air Surface of Water by Neutron and X-ray Reflectivity and Surface Tension Measurements: Polymer Concentration Dependence},
journal = {Macromolecules},
year = {2002},
volume = {35},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/ma0200468},
number = {26},
pages = {9737--9747},
doi = {10.1021/ma0200468}
}
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MLA
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YIM, H., et al. “Adsorption of Sodium Poly(styrenesulfonate) to the Air Surface of Water by Neutron and X-ray Reflectivity and Surface Tension Measurements: Polymer Concentration Dependence.” Macromolecules, vol. 35, no. 26, Nov. 2002, pp. 9737-9747. https://doi.org/10.1021/ma0200468.