Thorpe−Ingold Effect on Photoinduced Electron Transfer of Dialkylsilylene-Spaced Divinylarene Copolymers Having Alternating Donor and Acceptor Chromophores
Тип публикации: Journal Article
Дата публикации: 2007-11-21
scimago Q1
wos Q1
БС1
SJR: 1.352
CiteScore: 9
Impact factor: 5.2
ISSN: 00249297, 15205835
Materials Chemistry
Organic Chemistry
Inorganic Chemistry
Polymers and Plastics
Краткое описание
Dialkylsilylene-spaced divinylarene copolymers having alternating donor and acceptor chromophores are designed and synthesized. The rates of photoinduced electron transfer (PET) depend on the nature of the substituent on silicon. A replacement of the methyl substituent by the bulky isopropyl group has been shown to enhance the rate of PET. The results are rationalized in terms of the Thorpe-Ingold effect, which would bring the neighboring donor and acceptor chromophores in closer proximity. The STM images of the isopropyl-substituted copolymers are more folded than those of the methyl-substituted analogues, and these results are consistent with the outcome of photophysical studies of these copolymers.
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Yeh M. et al. Thorpe−Ingold Effect on Photoinduced Electron Transfer of Dialkylsilylene-Spaced Divinylarene Copolymers Having Alternating Donor and Acceptor Chromophores // Macromolecules. 2007. Vol. 40. No. 26. pp. 9238-9243.
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Yeh M., Lin H., Lim T., Lee S. L., Chen C., Fann W., Luh T. Y. Thorpe−Ingold Effect on Photoinduced Electron Transfer of Dialkylsilylene-Spaced Divinylarene Copolymers Having Alternating Donor and Acceptor Chromophores // Macromolecules. 2007. Vol. 40. No. 26. pp. 9238-9243.
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TY - JOUR
DO - 10.1021/ma702197k
UR - https://doi.org/10.1021/ma702197k
TI - Thorpe−Ingold Effect on Photoinduced Electron Transfer of Dialkylsilylene-Spaced Divinylarene Copolymers Having Alternating Donor and Acceptor Chromophores
T2 - Macromolecules
AU - Yeh, Mei-Yu
AU - Lin, Hsin-Chieh
AU - Lim, Tsong-Shin
AU - Lee, Shern Long
AU - Chen, Chi-Lin
AU - Fann, Wunshain
AU - Luh, T. Y.
PY - 2007
DA - 2007/11/21
PB - American Chemical Society (ACS)
SP - 9238-9243
IS - 26
VL - 40
SN - 0024-9297
SN - 1520-5835
ER -
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@article{2007_Yeh,
author = {Mei-Yu Yeh and Hsin-Chieh Lin and Tsong-Shin Lim and Shern Long Lee and Chi-Lin Chen and Wunshain Fann and T. Y. Luh},
title = {Thorpe−Ingold Effect on Photoinduced Electron Transfer of Dialkylsilylene-Spaced Divinylarene Copolymers Having Alternating Donor and Acceptor Chromophores},
journal = {Macromolecules},
year = {2007},
volume = {40},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/ma702197k},
number = {26},
pages = {9238--9243},
doi = {10.1021/ma702197k}
}
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MLA
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Yeh, Mei-Yu, et al. “Thorpe−Ingold Effect on Photoinduced Electron Transfer of Dialkylsilylene-Spaced Divinylarene Copolymers Having Alternating Donor and Acceptor Chromophores.” Macromolecules, vol. 40, no. 26, Nov. 2007, pp. 9238-9243. https://doi.org/10.1021/ma702197k.