Three-dimensional elemental mapping at the atomic scale in bimetallic nanocrystals
Bart Goris
1
,
A. I. De Backer
1
,
Sandra Van Aert
1
,
S. Gomez-Grana
2
,
Luis Liz-Marzan
2, 3, 4
,
Gustaaf Van Tendeloo
1
,
Publication type: Journal Article
Publication date: 2013-08-20
scimago Q1
wos Q1
SJR: 2.967
CiteScore: 14.9
Impact factor: 9.1
ISSN: 15306984, 15306992
PubMed ID:
23952010
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
A thorough understanding of the three-dimensional (3D) atomic structure and composition of core-shell nanostructures is indispensable to obtain a deeper insight on their physical behavior. Such 3D information can be reconstructed from two-dimensional (2D) projection images using electron tomography. Recently, different electron tomography techniques have enabled the 3D characterization of a variety of nanostructures down to the atomic level. However, these methods have all focused on the investigation of nanomaterials containing only one type of chemical element. Here, we combine statistical parameter estimation theory with compressive sensing based tomography to determine the positions and atom type of each atom in heteronanostructures. The approach is applied here to investigate the interface in core-shell Au@Ag nanorods but it is of great interest in the investigation of a broad range of nanostructures.
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Total citations:
99
Citations from 2024:
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GOST
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Goris B. et al. Three-dimensional elemental mapping at the atomic scale in bimetallic nanocrystals // Nano Letters. 2013. Vol. 13. No. 9. pp. 4236-4241.
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Goris B., De Backer A. I., Van Aert S., Gomez-Grana S., Liz-Marzan L., Van Tendeloo G., Bals S. Three-dimensional elemental mapping at the atomic scale in bimetallic nanocrystals // Nano Letters. 2013. Vol. 13. No. 9. pp. 4236-4241.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/nl401945b
UR - https://doi.org/10.1021/nl401945b
TI - Three-dimensional elemental mapping at the atomic scale in bimetallic nanocrystals
T2 - Nano Letters
AU - Goris, Bart
AU - De Backer, A. I.
AU - Van Aert, Sandra
AU - Gomez-Grana, S.
AU - Liz-Marzan, Luis
AU - Van Tendeloo, Gustaaf
AU - Bals, Sara
PY - 2013
DA - 2013/08/20
PB - American Chemical Society (ACS)
SP - 4236-4241
IS - 9
VL - 13
PMID - 23952010
SN - 1530-6984
SN - 1530-6992
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2013_Goris,
author = {Bart Goris and A. I. De Backer and Sandra Van Aert and S. Gomez-Grana and Luis Liz-Marzan and Gustaaf Van Tendeloo and Sara Bals},
title = {Three-dimensional elemental mapping at the atomic scale in bimetallic nanocrystals},
journal = {Nano Letters},
year = {2013},
volume = {13},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/nl401945b},
number = {9},
pages = {4236--4241},
doi = {10.1021/nl401945b}
}
Cite this
MLA
Copy
Goris, Bart, et al. “Three-dimensional elemental mapping at the atomic scale in bimetallic nanocrystals.” Nano Letters, vol. 13, no. 9, Aug. 2013, pp. 4236-4241. https://doi.org/10.1021/nl401945b.