Reactivity of Carbon in Lithium–Oxygen Battery Positive Electrodes
Daniil Itkis
1
,
Dmitry A Semenenko
1
,
Elmar Yu Kataev
1
,
Anna P. Sirotina
2
,
Michael Hävecker
3
,
D Teschner
3
,
Axel Knop-Gericke
3
,
Pavel Dudin
4
,
Alexei Barinov
4
,
Eugene Goodilin
1
,
Yang Shao-Horn
5
,
4
Sincrotrone Trieste S.C.p.A., Area Science Park, I-34012 Basovizza, Trieste, Italy
|
Publication type: Journal Article
Publication date: 2013-09-10
scimago Q1
wos Q1
SJR: 2.967
CiteScore: 14.9
Impact factor: 9.1
ISSN: 15306984, 15306992
PubMed ID:
24004050
General Chemistry
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Bioengineering
Abstract
Unfortunately, the practical applications of Li-O2 batteries are impeded by poor rechargeability. Here, for the first time we show that superoxide radicals generated at the cathode during discharge react with carbon that contains activated double bonds or aromatics to form epoxy groups and carbonates, which limits the rechargeability of Li-O2 cells. Carbon materials with a low amount of functional groups and defects demonstrate better stability thus keeping the carbon will-o'-the-wisp lit for lithium-air batteries.
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Metrics
273
Total citations:
273
Citations from 2024:
21
(7.7%)
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MLA
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GOST
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Itkis D. et al. Reactivity of Carbon in Lithium–Oxygen Battery Positive Electrodes // Nano Letters. 2013. Vol. 13. No. 10. pp. 4697-4701.
GOST all authors (up to 50)
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Itkis D., Semenenko D. A., Kataev E. Yu., Inozemtseva A. I., Neudachina V. S., Sirotina A. P., Hävecker M., Teschner D., Knop-Gericke A., Dudin P., Barinov A., Goodilin E., Shao-Horn Y., Yashina L. V. Reactivity of Carbon in Lithium–Oxygen Battery Positive Electrodes // Nano Letters. 2013. Vol. 13. No. 10. pp. 4697-4701.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/nl4021649
UR - https://doi.org/10.1021/nl4021649
TI - Reactivity of Carbon in Lithium–Oxygen Battery Positive Electrodes
T2 - Nano Letters
AU - Itkis, Daniil
AU - Semenenko, Dmitry A
AU - Kataev, Elmar Yu
AU - Inozemtseva, Alina I
AU - Neudachina, Vera S.
AU - Sirotina, Anna P.
AU - Hävecker, Michael
AU - Teschner, D
AU - Knop-Gericke, Axel
AU - Dudin, Pavel
AU - Barinov, Alexei
AU - Goodilin, Eugene
AU - Shao-Horn, Yang
AU - Yashina, Lada V.
PY - 2013
DA - 2013/09/10
PB - American Chemical Society (ACS)
SP - 4697-4701
IS - 10
VL - 13
PMID - 24004050
SN - 1530-6984
SN - 1530-6992
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2013_Itkis,
author = {Daniil Itkis and Dmitry A Semenenko and Elmar Yu Kataev and Alina I Inozemtseva and Vera S. Neudachina and Anna P. Sirotina and Michael Hävecker and D Teschner and Axel Knop-Gericke and Pavel Dudin and Alexei Barinov and Eugene Goodilin and Yang Shao-Horn and Lada V. Yashina},
title = {Reactivity of Carbon in Lithium–Oxygen Battery Positive Electrodes},
journal = {Nano Letters},
year = {2013},
volume = {13},
publisher = {American Chemical Society (ACS)},
month = {sep},
url = {https://doi.org/10.1021/nl4021649},
number = {10},
pages = {4697--4701},
doi = {10.1021/nl4021649}
}
Cite this
MLA
Copy
Itkis, Daniil, et al. “Reactivity of Carbon in Lithium–Oxygen Battery Positive Electrodes.” Nano Letters, vol. 13, no. 10, Sep. 2013, pp. 4697-4701. https://doi.org/10.1021/nl4021649.