ACS Nano, volume 8, issue 8, pages 8676-8682

Mercury Telluride Colloidal Quantum Dots: Electronic Structure, Size-Dependent Spectra, and Photocurrent Detection up to 12 μm

Sean E. Keuleyan ¹

Philippe Guyot-Sionnest ¹

Jing Li ²

Guy Allan ²

Hide authors affiliations Show authors affiliations: 2 affiliations

James Franck Institute, University of Chicago, 929 East 57th Street, Chicago, Illinois 60637, United States, |

IEMN, Dept ISEN, 41 boulevard Vauban, 59046 Lille Cedex, France |

Publication type: Journal Article

Publication date: 2014-08-14

American Chemical Society (ACS)

Journal: ACS Nano

Quartile SCImago

Quartile WOS

Impact factor: 17.1

ISSN: 19360851, 1936086X

DOI: 10.1021/nn503805h

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General Physics and Astronomy

General Materials Science

General Engineering

Abstract

HgTe colloidal quantum dots are synthesized with high monodispersivity with sizes up to ∼15 nm corresponding to a room temperature absorption edge at ∼5 μm. The shape is tetrahedral for larger sizes and up to five peaks are seen in the absorption spectra with a clear size dependence. The size range of the HgTe quantum dots is extended to ∼20 nm using regrowth. The corresponding room temperature photoluminescence and absorption edge reach into the long-wave infrared, past 8 μm. Upon cooling to liquid nitrogen temperature, a photoconductive response is obtained in the long-wave infrared region up to 12 μm. Configuration-interaction tight-binding calculations successfully explain the spectra and the size dependence. The five optical features can be assigned to sets of single hole to single electron transitions whose strengths are strongly influenced by the multiband/multiorbital character of the quantum-dot electronic states.

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ACS Nano	ACS Nano, 11, 8.21% ACS Nano 11 publications, 8.21%
ACS Photonics	ACS Photonics, 7, 5.22% ACS Photonics 7 publications, 5.22%
Nano Letters	Nano Letters, 6, 4.48% Nano Letters 6 publications, 4.48%
Coatings	Coatings, 5, 3.73% Coatings 5 publications, 3.73%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 5, 3.73% Journal of Physical Chemistry C 5 publications, 3.73%
Chemistry of Materials	Chemistry of Materials, 5, 3.73% Chemistry of Materials 5 publications, 3.73%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 5, 3.73% Journal of Materials Chemistry C 5 publications, 3.73%
Advanced Materials	Advanced Materials, 3, 2.24% Advanced Materials 3 publications, 2.24%
Advanced Functional Materials	Advanced Functional Materials, 3, 2.24% Advanced Functional Materials 3 publications, 2.24%
Chemical Reviews	Chemical Reviews, 3, 2.24% Chemical Reviews 3 publications, 2.24%
ACS applied materials & interfaces	ACS applied materials & interfaces, 3, 2.24% ACS applied materials & interfaces 3 publications, 2.24%
Materials	Materials, 2, 1.49% Materials 2 publications, 1.49%
Nature Photonics	Nature Photonics, 2, 1.49% Nature Photonics 2 publications, 1.49%
Nature Materials	Nature Materials, 2, 1.49% Nature Materials 2 publications, 1.49%
Light: Science and Applications	Light: Science and Applications, 2, 1.49% Light: Science and Applications 2 publications, 1.49%
Nanotechnology	Nanotechnology, 2, 1.49% Nanotechnology 2 publications, 1.49%
Infrared Physics and Technology	Infrared Physics and Technology, 2, 1.49% Infrared Physics and Technology 2 publications, 1.49%
Small	Small, 2, 1.49% Small 2 publications, 1.49%
Advanced Materials Technologies	Advanced Materials Technologies, 2, 1.49% Advanced Materials Technologies 2 publications, 1.49%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 2, 1.49% Journal of Physical Chemistry Letters 2 publications, 1.49%
Nanoscale	Nanoscale, 2, 1.49% Nanoscale 2 publications, 1.49%
Journal of Nanomaterials	Journal of Nanomaterials, 1, 0.75% Journal of Nanomaterials 1 publication, 0.75%
Applied Physics Letters	Applied Physics Letters, 1, 0.75% Applied Physics Letters 1 publication, 0.75%
Journal of Chemical Physics	Journal of Chemical Physics, 1, 0.75% Journal of Chemical Physics 1 publication, 0.75%
International Journal of Nanoscience	International Journal of Nanoscience, 1, 0.75% International Journal of Nanoscience 1 publication, 0.75%
Applied Sciences (Switzerland)	Applied Sciences (Switzerland), 1, 0.75% Applied Sciences (Switzerland) 1 publication, 0.75%
Frontiers in Chemistry	Frontiers in Chemistry, 1, 0.75% Frontiers in Chemistry 1 publication, 0.75%
Frontiers in Energy Research	Frontiers in Energy Research, 1, 0.75% Frontiers in Energy Research 1 publication, 0.75%
Nature Electronics	Nature Electronics, 1, 0.75% Nature Electronics 1 publication, 0.75%
	2 4 6 8 10 12

Citations by publishers

	5 10 15 20 25 30 35 40 45
American Chemical Society (ACS)	American Chemical Society (ACS), 45, 33.58% American Chemical Society (ACS) 45 publications, 33.58%
Wiley	Wiley, 16, 11.94% Wiley 16 publications, 11.94%
Springer Nature	Springer Nature, 11, 8.21% Springer Nature 11 publications, 8.21%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 11, 8.21% Royal Society of Chemistry (RSC) 11 publications, 8.21%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 8, 5.97% Multidisciplinary Digital Publishing Institute (MDPI) 8 publications, 5.97%
Elsevier	Elsevier, 7, 5.22% Elsevier 7 publications, 5.22%
IOP Publishing	IOP Publishing, 4, 2.99% IOP Publishing 4 publications, 2.99%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 3, 2.24% American Institute of Physics (AIP) 3 publications, 2.24%
Frontiers Media S.A.	Frontiers Media S.A., 2, 1.49% Frontiers Media S.A. 2 publications, 1.49%
Pleiades Publishing	Pleiades Publishing, 2, 1.49% Pleiades Publishing 2 publications, 1.49%
Hindawi Limited	Hindawi Limited, 1, 0.75% Hindawi Limited 1 publication, 0.75%
World Scientific	World Scientific, 1, 0.75% World Scientific 1 publication, 0.75%
Materials Research Society	Materials Research Society, 1, 0.75% Materials Research Society 1 publication, 0.75%
IEEE	IEEE, 1, 0.75% IEEE 1 publication, 0.75%
Walter de Gruyter	Walter de Gruyter, 1, 0.75% Walter de Gruyter 1 publication, 0.75%
Optical Society of America	Optical Society of America, 1, 0.75% Optical Society of America 1 publication, 0.75%
SPIE	SPIE, 1, 0.75% SPIE 1 publication, 0.75%
Taylor & Francis	Taylor & Francis, 1, 0.75% Taylor & Francis 1 publication, 0.75%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.75% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.75%
American Physical Society (APS)	American Physical Society (APS), 1, 0.75% American Physical Society (APS) 1 publication, 0.75%
	5 10 15 20 25 30 35 40 45

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Keuleyan S. E. et al. Mercury Telluride Colloidal Quantum Dots: Electronic Structure, Size-Dependent Spectra, and Photocurrent Detection up to 12 μm // ACS Nano. 2014. Vol. 8. No. 8. pp. 8676-8682.

GOST all authors (up to 50) Copy

Keuleyan S. E., Guyot-Sionnest P., Li J., Allan G. Mercury Telluride Colloidal Quantum Dots: Electronic Structure, Size-Dependent Spectra, and Photocurrent Detection up to 12 μm // ACS Nano. 2014. Vol. 8. No. 8. pp. 8676-8682.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/nn503805h

UR - https://doi.org/10.1021/nn503805h

TI - Mercury Telluride Colloidal Quantum Dots: Electronic Structure, Size-Dependent Spectra, and Photocurrent Detection up to 12 μm

T2 - ACS Nano

AU - Allan, Guy

AU - Keuleyan, Sean E.

AU - Guyot-Sionnest, Philippe

AU - Li, Jing

PY - 2014

DA - 2014/08/14 00:00:00

PB - American Chemical Society (ACS)

SP - 8676-8682

IS - 8

VL - 8

SN - 1936-0851

SN - 1936-086X

ER -

BibTex |

Cite this

BibTex Copy

@article{2014_Keuleyan,

author = {Guy Allan and Sean E. Keuleyan and Philippe Guyot-Sionnest and Jing Li},

title = {Mercury Telluride Colloidal Quantum Dots: Electronic Structure, Size-Dependent Spectra, and Photocurrent Detection up to 12 μm},

journal = {ACS Nano},

year = {2014},

volume = {8},

publisher = {American Chemical Society (ACS)},

month = {aug},

url = {https://doi.org/10.1021/nn503805h},

number = {8},

pages = {8676--8682},

doi = {10.1021/nn503805h}

}

MLA

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MLA Copy

Keuleyan, Sean E., et al. “Mercury Telluride Colloidal Quantum Dots: Electronic Structure, Size-Dependent Spectra, and Photocurrent Detection up to 12 μm.” ACS Nano, vol. 8, no. 8, Aug. 2014, pp. 8676-8682. https://doi.org/10.1021/nn503805h.

Found error?

Publisher

American Chemical Society (ACS)

Journal

ACS Nano

Quartile SCImago

Quartile WOS

Impact factor

17.1

ISSN

19360851 (Print)
1936086X (Electronic)