Surface state of a silver catalyst for ethylene glycol oxidation
A. S. Knyazev
1
,
A.I. BORONIN
2
,
S.V Koshcheev
2
,
A N Salanov
2
,
O V Vodyankina
3
,
L.N. Kurina
1, 3
1
Institute of Petrochemistry, Siberian Division, Russian Academy of Sciences, Tomsk, Russia
|
2
Publication type: Journal Article
Publication date: 2003-09-15
scimago Q3
wos Q4
SJR: 0.260
CiteScore: 1.9
Impact factor: 1.4
ISSN: 00231584, 16083210
General Chemistry
Catalysis
Computer Science Applications
Modeling and Simulation
Abstract
The surface state of electrolytic silver before and after treatment with a reaction mixture in the course of ethylene glycol oxidation to glyoxal was studied using X-ray photoelectron spectroscopy and scanning electron microscopy. It was found that electrophilic forms of adsorbed oxygen, which participate in the selective conversion of ethylene glycol, were formed on the surface of electrolytic silver crystals under exposure to oxygen under conditions similar to catalytic process conditions. The treatment of the catalyst with a reaction mixture resulted in the formation of filamentous carbon deposition products. A mechanism of formation of carbon-containing products was proposed.
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GOST
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Knyazev A. S. et al. Surface state of a silver catalyst for ethylene glycol oxidation // Kinetics and Catalysis. 2003. Vol. 44. No. 3. pp. 408-413.
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Knyazev A. S., BORONIN A., Koshcheev S., Salanov A. N., Vodyankina O. V., Kurina L. Surface state of a silver catalyst for ethylene glycol oxidation // Kinetics and Catalysis. 2003. Vol. 44. No. 3. pp. 408-413.
Cite this
RIS
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TY - JOUR
DO - 10.1023/A:1024403220572
UR - https://doi.org/10.1023/A:1024403220572
TI - Surface state of a silver catalyst for ethylene glycol oxidation
T2 - Kinetics and Catalysis
AU - Knyazev, A. S.
AU - BORONIN, A.I.
AU - Koshcheev, S.V
AU - Salanov, A N
AU - Vodyankina, O V
AU - Kurina, L.N.
PY - 2003
DA - 2003/09/15
PB - Pleiades Publishing
SP - 408-413
IS - 3
VL - 44
SN - 0023-1584
SN - 1608-3210
ER -
Cite this
BibTex (up to 50 authors)
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@article{2003_Knyazev,
author = {A. S. Knyazev and A.I. BORONIN and S.V Koshcheev and A N Salanov and O V Vodyankina and L.N. Kurina},
title = {Surface state of a silver catalyst for ethylene glycol oxidation},
journal = {Kinetics and Catalysis},
year = {2003},
volume = {44},
publisher = {Pleiades Publishing},
month = {sep},
url = {https://doi.org/10.1023/A:1024403220572},
number = {3},
pages = {408--413},
doi = {10.1023/A:1024403220572}
}
Cite this
MLA
Copy
Knyazev, A. S., et al. “Surface state of a silver catalyst for ethylene glycol oxidation.” Kinetics and Catalysis, vol. 44, no. 3, Sep. 2003, pp. 408-413. https://doi.org/10.1023/A:1024403220572.