Open Access

Nature Communications, volume 14, issue 1, publication number 699

Mode locking of hole spin coherences in CsPb(Cl, Br)3 perovskite nanocrystals

Kirstein E. ¹

Kopteva N. E. ¹

Yakovlev D G ^{1, 2, 3}

Zhukov E. A. ^{1, 2}

Kolobkova E V ^{4, 5}

Kuznetsova Daria S. ⁶

Belykh V. V. ³

Yugova Irina A. ⁶

Glazov Mikhail M. ²

Bayer M. ¹

Greilich A. ¹

Hide authors affiliations Show authors affiliations: 6 affiliations

Experimentelle Physik 2, Technische Universität Dortmund, Dortmund, Germany |

Ioffe Institute, Russian Academy of Sciences, St. Petersburg, Russia |

P. N. Lebedev Physical Institute of the Russian Academy of Sciences, Moscow, Russia |

⁴

ITMO University, St. Petersburg, Russia |

⁵

St. Petersburg State Institute of Technology, St. Petersburg, Russia |

⁶

Spin Optics Laboratory, St. Petersburg State University, St. Petersburg, Russia |

Publication type: Journal Article

Publication date: 2023-02-08

Springer Nature

Journal: Nature Communications

Quartile SCImago

Quartile WOS

Impact factor: 16.6

ISSN: 20411723

DOI: 10.1038/s41467-023-36165-0

Copy DOI

General Chemistry

General Biochemistry, Genetics and Molecular Biology

Multidisciplinary

General Physics and Astronomy

Abstract

The spin physics of perovskite nanocrystals with confined electrons or holes is attracting increasing attention, both for fundamental studies and spintronic applications. Here, stable $${{{{{{{\rm{CsPb}}}}}}}}{({{{{{{{{\rm{Cl}}}}}}}}}_{0.56}{{{{{{{{\rm{Br}}}}}}}}}_{0.44})}_{3}$$ CsPb ( Cl 0.56 Br 0.44 ) 3 lead halide perovskite nanocrystals embedded in a fluorophosphate glass matrix are studied by time-resolved optical spectroscopy to unravel the coherent spin dynamics of holes and their interaction with nuclear spins of the ²⁰⁷Pb isotope. We demonstrate the spin mode locking effect provided by the synchronization of the Larmor precession of single hole spins in each nanocrystal in the ensemble that are excited periodically by a laser in an external magnetic field. The mode locking is enhanced by nuclei-induced frequency focusing. An ensemble spin dephasing time $${T}_{2}^{ * }$$ T 2 * of a nanosecond and a single hole spin coherence time of T₂ = 13 ns are measured. The developed theoretical model accounting for the mode locking and nuclear focusing for randomly oriented nanocrystals with perovskite band structure describes the experimental data very well.

By date By citations

Citations by journals

	1 2
Nanomaterials	Nanomaterials, 2, 25% Nanomaterials 2 publications, 25%
Photonics	Photonics, 1, 12.5% Photonics 1 publication, 12.5%
Nano Letters	Nano Letters, 1, 12.5% Nano Letters 1 publication, 12.5%
Advances in Physics: X	Advances in Physics: X, 1, 12.5% Advances in Physics: X 1 publication, 12.5%
Nano Research	Nano Research, 1, 12.5% Nano Research 1 publication, 12.5%
	1 2

Citations by publishers

	1 2 3
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 3, 37.5% Multidisciplinary Digital Publishing Institute (MDPI) 3 publications, 37.5%
American Chemical Society (ACS)	American Chemical Society (ACS), 1, 12.5% American Chemical Society (ACS) 1 publication, 12.5%
Taylor & Francis	Taylor & Francis, 1, 12.5% Taylor & Francis 1 publication, 12.5%
Springer Nature	Springer Nature, 1, 12.5% Springer Nature 1 publication, 12.5%
	1 2 3

We do not take into account publications that without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

{"yearsCitations":{"type":"bar","data":{"show":true,"labels":[2023,2024],"ids":[0,0],"codes":[0,0],"imageUrls":["",""],"datasets":[{"label":"Citations number","data":[7,1],"backgroundColor":["#3B82F6","#3B82F6"],"percentage":["87.5","12.5"],"barThickness":null}]},"options":{"indexAxis":"x","maintainAspectRatio":true,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"}},"x":{"ticks":{"stepSize":1,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"}}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Citations per year","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}},"journals":{"type":"bar","data":{"show":true,"labels":["Nanomaterials","Photonics","Nano Letters","Advances in Physics: X","Nano Research"],"ids":[10051,12741,10312,21999,12211],"codes":[0,0,0,0,0],"imageUrls":["\/storage\/images\/resized\/MjH1ITP7lMYGxeqUZfkt2BnVLgjkk413jwBV97XX_medium.webp","\/storage\/images\/resized\/MjH1ITP7lMYGxeqUZfkt2BnVLgjkk413jwBV97XX_medium.webp","\/storage\/images\/resized\/iLiQsFqFaSEx6chlGQ5fbAwF6VYU3WWa08hkss0g_medium.webp","\/storage\/images\/resized\/5YZtvLvkPZuc2JHOaZsjCvGSHFCuC3drUwN3YAc5_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp"],"datasets":[{"label":"","data":[2,1,1,1,1],"backgroundColor":["#3B82F6","#3B82F6","#3B82F6","#3B82F6","#3B82F6"],"percentage":[25,12.5,12.5,12.5,12.5],"barThickness":13}]},"options":{"indexAxis":"y","maintainAspectRatio":false,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"}},"x":{"ticks":{"stepSize":null,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"}}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Journals","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}},"publishers":{"type":"bar","data":{"show":true,"labels":["Multidisciplinary Digital Publishing Institute (MDPI)","American Chemical Society (ACS)","Taylor & Francis","Springer Nature"],"ids":[202,40,18,8],"codes":[0,0,0,0],"imageUrls":["\/storage\/images\/resized\/MjH1ITP7lMYGxeqUZfkt2BnVLgjkk413jwBV97XX_medium.webp","\/storage\/images\/resized\/iLiQsFqFaSEx6chlGQ5fbAwF6VYU3WWa08hkss0g_medium.webp","\/storage\/images\/resized\/5YZtvLvkPZuc2JHOaZsjCvGSHFCuC3drUwN3YAc5_medium.webp","\/storage\/images\/resized\/voXLqlsvTwv5p3iMQ8Dhs95nqB4AXOG7Taj7G4ra_medium.webp"],"datasets":[{"label":"","data":[3,1,1,1],"backgroundColor":["#3B82F6","#3B82F6","#3B82F6","#3B82F6"],"percentage":[37.5,12.5,12.5,12.5],"barThickness":13}]},"options":{"indexAxis":"y","maintainAspectRatio":false,"scales":{"y":{"ticks":{"precision":0,"autoSkip":false,"font":{"family":"Montserrat"},"color":"#000000"}},"x":{"ticks":{"stepSize":null,"precision":0,"font":{"family":"Montserrat"},"color":"#000000"}}},"plugins":{"legend":{"position":"top","labels":{"font":{"family":"Montserrat"},"color":"#000000"}},"title":{"display":true,"text":"Publishers","font":{"size":24,"family":"Montserrat","weight":600},"color":"#000000"}}}}}

Publication PDF

Metrics

Cite this

GOST |

Cite this

GOST Copy

Kirstein E. et al. Mode locking of hole spin coherences in CsPb(Cl, Br)3 perovskite nanocrystals // Nature Communications. 2023. Vol. 14. No. 1. 699

GOST all authors (up to 50) Copy

Kirstein E., Kopteva N. E., Yakovlev D. G., Zhukov E. A., Kolobkova E. V., Kuznetsova D. S., Belykh V., Yugova I. A., Glazov M. M., Bayer M., Greilich A. Mode locking of hole spin coherences in CsPb(Cl, Br)3 perovskite nanocrystals // Nature Communications. 2023. Vol. 14. No. 1. 699

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1038/s41467-023-36165-0

UR - https://doi.org/10.1038%2Fs41467-023-36165-0

TI - Mode locking of hole spin coherences in CsPb(Cl, Br)3 perovskite nanocrystals

T2 - Nature Communications

AU - Kirstein, E.

AU - Kopteva, N. E.

AU - Yakovlev, D G

AU - Zhukov, E. A.

AU - Kolobkova, E V

AU - Kuznetsova, Daria S.

AU - Belykh, V. V.

AU - Yugova, Irina A.

AU - Glazov, Mikhail M.

AU - Bayer, M.

AU - Greilich, A.

PY - 2023

DA - 2023/02/08 00:00:00

PB - Springer Nature

IS - 1

VL - 14

SN - 2041-1723

ER -

BibTex

Cite this

BibTex Copy

@article{2023_Kirstein,

author = {E. Kirstein and N. E. Kopteva and D G Yakovlev and E. A. Zhukov and E V Kolobkova and Daria S. Kuznetsova and V. V. Belykh and Irina A. Yugova and Mikhail M. Glazov and M. Bayer and A. Greilich},

title = {Mode locking of hole spin coherences in CsPb(Cl, Br)3 perovskite nanocrystals},

journal = {Nature Communications},

year = {2023},

volume = {14},

publisher = {Springer Nature},

month = {feb},

url = {https://doi.org/10.1038%2Fs41467-023-36165-0},

number = {1},

doi = {10.1038/s41467-023-36165-0}

}

Found error?

Publisher

Springer Nature

Journal

Nature Communications

Quartile SCImago

Quartile WOS

Impact factor

16.6

ISSN

20411723 (Print)

Labs

Laboratory of Spin Physics of two-dimensional Materials

Profiles