Nature Materials, volume 16, issue 2, pages 258-263

Hybrid organic-inorganic inks flatten the energy landscape in colloidal quantum dot solids.

Mengxia Liu ¹

Oleksandr Voznyy ¹

Randy Sabatini ¹

F Pelayo García De Arquer ¹

Rahim Munir ²

Ahmed Hesham Balawi ²

Xinzheng Lan ¹

Fengjia Fan ¹

Grant Walters ¹

Ahmad R Kirmani ²

Sjoerd Hoogland ¹

Frédéric Laquai ²

Aram Amassian ²

Edward H Sargent ¹

Hide authors affiliations Show authors affiliations: 2 affiliations

Department of Electrical and Computer Engineering, University of Toronto, 10 King’s College Road, Toronto, Ontario M5S 3G4, Canada |

and Physical Sciences and Engineering Division, King Abdullah University of Science and Technology (KAUST), KAUST Solar Center (KSC), 4700 KAUST, Thuwal 23955-6900, Saudi Arabia |

Publication type: Journal Article

Publication date: 2016-11-14

Springer Nature

Journal: Nature Materials

Quartile SCImago

Quartile WOS

Impact factor: 41.2

ISSN: 14761122, 14764660

DOI: 10.1038/nmat4800

Copy DOI

General Chemistry

Condensed Matter Physics

General Materials Science

Mechanical Engineering

Mechanics of Materials

Abstract

Bandtail states in disordered semiconductor materials result in losses in open-circuit voltage (Voc) and inhibit carrier transport in photovoltaics. For colloidal quantum dot (CQD) films that promise low-cost, large-area, air-stable photovoltaics, bandtails are determined by CQD synthetic polydispersity and inhomogeneous aggregation during the ligand-exchange process. Here we introduce a new method for the synthesis of solution-phase ligand-exchanged CQD inks that enable a flat energy landscape and an advantageously high packing density. In the solid state, these materials exhibit a sharper bandtail and reduced energy funnelling compared with the previous best CQD thin films for photovoltaics. Consequently, we demonstrate solar cells with higher Voc and more efficient charge injection into the electron acceptor, allowing the use of a closer-to-optimum bandgap to absorb more light. These enable the fabrication of CQD solar cells made via a solution-phase ligand exchange, with a certified power conversion efficiency of 11.28%. The devices are stable when stored in air, unencapsulated, for over 1,000 h.

By date By citations

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Citations by journals

	5 10 15 20 25 30 35 40 45
Advanced Materials	Advanced Materials, 45, 7.71% Advanced Materials 45 publications, 7.71%
ACS applied materials & interfaces	ACS applied materials & interfaces, 38, 6.51% ACS applied materials & interfaces 38 publications, 6.51%
ACS Energy Letters	ACS Energy Letters, 30, 5.14% ACS Energy Letters 30 publications, 5.14%
Advanced Energy Materials	Advanced Energy Materials, 22, 3.77% Advanced Energy Materials 22 publications, 3.77%
Advanced Functional Materials	Advanced Functional Materials, 16, 2.74% Advanced Functional Materials 16 publications, 2.74%
Journal of Materials Chemistry C	Journal of Materials Chemistry C, 16, 2.74% Journal of Materials Chemistry C 16 publications, 2.74%
Nano Letters	Nano Letters, 14, 2.4% Nano Letters 14 publications, 2.4%
Chemistry of Materials	Chemistry of Materials, 13, 2.23% Chemistry of Materials 13 publications, 2.23%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 13, 2.23% Journal of Materials Chemistry A 13 publications, 2.23%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 12, 2.05% Journal of Physical Chemistry Letters 12 publications, 2.05%
Nature Communications	Nature Communications, 12, 2.05% Nature Communications 12 publications, 2.05%
Solar RRL	Solar RRL, 12, 2.05% Solar RRL 12 publications, 2.05%
ACS Applied Energy Materials	ACS Applied Energy Materials, 10, 1.71% ACS Applied Energy Materials 10 publications, 1.71%
Energy and Environmental Science	Energy and Environmental Science, 10, 1.71% Energy and Environmental Science 10 publications, 1.71%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 9, 1.54% Journal of Physical Chemistry C 9 publications, 1.54%
Nano Energy	Nano Energy, 9, 1.54% Nano Energy 9 publications, 1.54%
Small	Small, 9, 1.54% Small 9 publications, 1.54%
ACS Nano	ACS Nano, 9, 1.54% ACS Nano 9 publications, 1.54%
Chemical Engineering Journal	Chemical Engineering Journal, 8, 1.37% Chemical Engineering Journal 8 publications, 1.37%
Advanced Optical Materials	Advanced Optical Materials, 8, 1.37% Advanced Optical Materials 8 publications, 1.37%
Nanoscale	Nanoscale, 8, 1.37% Nanoscale 8 publications, 1.37%
Solar Energy Materials and Solar Cells	Solar Energy Materials and Solar Cells, 7, 1.2% Solar Energy Materials and Solar Cells 7 publications, 1.2%
Nano Research	Nano Research, 6, 1.03% Nano Research 6 publications, 1.03%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 6, 1.03% Angewandte Chemie - International Edition 6 publications, 1.03%
Angewandte Chemie	Angewandte Chemie, 6, 1.03% Angewandte Chemie 6 publications, 1.03%
ACS Applied Nano Materials	ACS Applied Nano Materials, 6, 1.03% ACS Applied Nano Materials 6 publications, 1.03%
ACS Photonics	ACS Photonics, 5, 0.86% ACS Photonics 5 publications, 0.86%
Journal of Materials Science: Materials in Electronics	Journal of Materials Science: Materials in Electronics, 5, 0.86% Journal of Materials Science: Materials in Electronics 5 publications, 0.86%
Solar Energy	Solar Energy, 5, 0.86% Solar Energy 5 publications, 0.86%
	5 10 15 20 25 30 35 40 45

Citations by publishers

	20 40 60 80 100 120 140 160 180
American Chemical Society (ACS)	American Chemical Society (ACS), 166, 28.42% American Chemical Society (ACS) 166 publications, 28.42%
Wiley	Wiley, 155, 26.54% Wiley 155 publications, 26.54%
Elsevier	Elsevier, 80, 13.7% Elsevier 80 publications, 13.7%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 76, 13.01% Royal Society of Chemistry (RSC) 76 publications, 13.01%
Springer Nature	Springer Nature, 54, 9.25% Springer Nature 54 publications, 9.25%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 12, 2.05% Multidisciplinary Digital Publishing Institute (MDPI) 12 publications, 2.05%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 9, 1.54% American Institute of Physics (AIP) 9 publications, 1.54%
IOP Publishing	IOP Publishing, 6, 1.03% IOP Publishing 6 publications, 1.03%
Optical Society of America	Optical Society of America, 3, 0.51% Optical Society of America 3 publications, 0.51%
Japan Society of Applied Physics	Japan Society of Applied Physics, 2, 0.34% Japan Society of Applied Physics 2 publications, 0.34%
IEEE	IEEE, 2, 0.34% IEEE 2 publications, 0.34%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 2, 0.34% American Association for the Advancement of Science (AAAS) 2 publications, 0.34%
International Union of Crystallography (IUCr)	International Union of Crystallography (IUCr), 1, 0.17% International Union of Crystallography (IUCr) 1 publication, 0.17%
Science in China Press	Science in China Press, 1, 0.17% Science in China Press 1 publication, 0.17%
Cambridge University Press	Cambridge University Press, 1, 0.17% Cambridge University Press 1 publication, 0.17%
University of Electronic Science and Technology of China	University of Electronic Science and Technology of China, 1, 0.17% University of Electronic Science and Technology of China 1 publication, 0.17%
American Physical Society (APS)	American Physical Society (APS), 1, 0.17% American Physical Society (APS) 1 publication, 0.17%
Taylor & Francis	Taylor & Francis, 1, 0.17% Taylor & Francis 1 publication, 0.17%
Walter de Gruyter	Walter de Gruyter, 1, 0.17% Walter de Gruyter 1 publication, 0.17%
SPIE	SPIE, 1, 0.17% SPIE 1 publication, 0.17%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.17% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.17%
	20 40 60 80 100 120 140 160 180

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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GOST Copy

Liu M. et al. Hybrid organic-inorganic inks flatten the energy landscape in colloidal quantum dot solids. // Nature Materials. 2016. Vol. 16. No. 2. pp. 258-263.

GOST all authors (up to 50) Copy

Liu M., Voznyy O., Sabatini R., García De Arquer F. P., Munir R., Balawi A. H., Lan X., Fan F., Walters G., Kirmani A. R., Hoogland S., Laquai F., Amassian A., Sargent E. H. Hybrid organic-inorganic inks flatten the energy landscape in colloidal quantum dot solids. // Nature Materials. 2016. Vol. 16. No. 2. pp. 258-263.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1038/nmat4800

UR - https://doi.org/10.1038/nmat4800

TI - Hybrid organic-inorganic inks flatten the energy landscape in colloidal quantum dot solids.

T2 - Nature Materials

AU - Liu, Mengxia

AU - Voznyy, Oleksandr

AU - Sabatini, Randy

AU - García De Arquer, F Pelayo

AU - Munir, Rahim

AU - Balawi, Ahmed Hesham

AU - Lan, Xinzheng

AU - Fan, Fengjia

AU - Walters, Grant

AU - Kirmani, Ahmad R

AU - Hoogland, Sjoerd

AU - Laquai, Frédéric

AU - Amassian, Aram

AU - Sargent, Edward H

PY - 2016

DA - 2016/11/14 00:00:00

PB - Springer Nature

SP - 258-263

IS - 2

VL - 16

SN - 1476-1122

SN - 1476-4660

ER -

BibTex |

Cite this

BibTex Copy

@article{2016_Liu,

author = {Mengxia Liu and Oleksandr Voznyy and Randy Sabatini and F Pelayo García De Arquer and Rahim Munir and Ahmed Hesham Balawi and Xinzheng Lan and Fengjia Fan and Grant Walters and Ahmad R Kirmani and Sjoerd Hoogland and Frédéric Laquai and Aram Amassian and Edward H Sargent},

title = {Hybrid organic-inorganic inks flatten the energy landscape in colloidal quantum dot solids.},

journal = {Nature Materials},

year = {2016},

volume = {16},

publisher = {Springer Nature},

month = {nov},

url = {https://doi.org/10.1038/nmat4800},

number = {2},

pages = {258--263},

doi = {10.1038/nmat4800}

}

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Liu, Mengxia, et al. “Hybrid organic-inorganic inks flatten the energy landscape in colloidal quantum dot solids..” Nature Materials, vol. 16, no. 2, Nov. 2016, pp. 258-263. https://doi.org/10.1038/nmat4800.

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Publisher

Springer Nature

Journal

Nature Materials

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41.2

ISSN

14761122 (Print)
14764660 (Electronic)