Open Access

Nature Communications, volume 6, issue 1, publication number 6293

Exploring atomic defects in molybdenum disulphide monolayers

Hong Jinhua ¹

Hu Zhixin ²

Probert Matt ³

Li Kun ⁴

Lv Danhui ¹

YANG XINAN ⁵

Gu Lin ⁵

Mao Nannan ^{6, 7}

Feng Qingliang ⁶

Xie Liming ⁶

Zhang Jin ⁷

Wu Dianzhong ⁸

Zhang Zhiyong ⁸

Jin Chuanhong ¹

Ji Wei ^{2, 9}

Zhang Xixiang ⁴

Yuan Jun ^{1, 3}

Zhang Ze ¹

Hide authors affiliations Show authors affiliations: 9 affiliations

State Key Laboratory of Silicon Materials, Key Laboratory of Advanced Materials and Applications for Batteries of Zhejiang Province, School of Materials Science and Engineering, Zhejiang University, Hangzhou, China |

Department of Physics, Beijing Key Laboratory of Optoelectronic Functional Materials and Micro-Nano Devices, Renmin University of China, Beijing, China |

Department of Physics, University of York, Heslington, York YO10 5DD, UK, |

⁴

Advanced Nanofabrication, Imaging and Characterization Core Lab, King Abdullah University of Science and Technology (KAUST), Thuwal, Kingdom of Saudi Arabia |

⁵

Instituteof Physics, Chinese Academy of Sciences, c/o Collaborative Innovation Center of Quantum Matter, Beijing, China |

⁶

CAS Key Laboratory of Standardization and Measurement for Nanotechnology, National Center for Nanoscience and Technology, Beijing, China |

⁷

Center for Nanochemistry, Beijing National Laboratory for Molecular Sciences, Key Laboratory for the Physics and Chemistry of Nanodevices, State Key Laboratory for Structural Chemistry of Unstable and Stable Species, College of Chemistry and Molecular Engineering, Peking University, Beijing, China |

⁸

Key Laboratory for the Physics and Chemistry of Nanodevices and Department of Electronics, Peking University, Beijing, China |

⁹

Department of Physics and Astronomy, Collaborative Innovation Center of Advanced Microstructures, Shanghai Jiao Tong University, Shanghai, China |

Publication type: Journal Article

Publication date: 2015-02-19

Springer Nature

Journal: Nature Communications

Quartile SCImago

Quartile WOS

Impact factor: 16.6

ISSN: 20411723

DOI: 10.1038/ncomms7293

Copy DOI

PubMed ID: 25695374

General Chemistry

General Biochemistry, Genetics and Molecular Biology

General Physics and Astronomy

Abstract

Defects usually play an important role in tailoring various properties of two-dimensional materials. Defects in two-dimensional monolayer molybdenum disulphide may be responsible for large variation of electric and optical properties. Here we present a comprehensive joint experiment–theory investigation of point defects in monolayer molybdenum disulphide prepared by mechanical exfoliation, physical and chemical vapour deposition. Defect species are systematically identified and their concentrations determined by aberration-corrected scanning transmission electron microscopy, and also studied by ab-initio calculation. Defect density up to 3.5 × 1013 cm−2 is found and the dominant category of defects changes from sulphur vacancy in mechanical exfoliation and chemical vapour deposition samples to molybdenum antisite in physical vapour deposition samples. Influence of defects on electronic structure and charge-carrier mobility are predicted by calculation and observed by electric transport measurement. In light of these results, the growth of ultra-high-quality monolayer molybdenum disulphide appears a primary task for the community pursuing high-performance electronic devices. Imperfections can greatly alter a material’s properties. Here, the authors investigate the influence of point defects on the electronic structure, charge-carrier mobility and optical absorption of molybdenum disulphide prepared by mechanical exfoliation, physical and chemical vapour deposition.

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ACS Nano	ACS Nano, 70, 6.4% ACS Nano 70 publications, 6.4%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 52, 4.76% Journal of Physical Chemistry C 52 publications, 4.76%
ACS applied materials & interfaces	ACS applied materials & interfaces, 47, 4.3% ACS applied materials & interfaces 47 publications, 4.3%
Physical Review B	Physical Review B, 43, 3.93% Physical Review B 43 publications, 3.93%
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Nature Communications	Nature Communications, 26, 2.38% Nature Communications 26 publications, 2.38%
Nanoscale	Nanoscale, 26, 2.38% Nanoscale 26 publications, 2.38%
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2D Materials	2D Materials, 21, 1.92% 2D Materials 21 publications, 1.92%
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Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 18, 1.65% Physical Chemistry Chemical Physics 18 publications, 1.65%
Applied Physics Letters	Applied Physics Letters, 17, 1.56% Applied Physics Letters 17 publications, 1.56%
Scientific Reports	Scientific Reports, 16, 1.46% Scientific Reports 16 publications, 1.46%
Nano Research	Nano Research, 15, 1.37% Nano Research 15 publications, 1.37%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 14, 1.28% Journal of Physical Chemistry Letters 14 publications, 1.28%
Journal of Applied Physics	Journal of Applied Physics, 12, 1.1% Journal of Applied Physics 12 publications, 1.1%
Physical Review Materials	Physical Review Materials, 11, 1.01% Physical Review Materials 11 publications, 1.01%
Chemical Society Reviews	Chemical Society Reviews, 10, 0.91% Chemical Society Reviews 10 publications, 0.91%
RSC Advances	RSC Advances, 10, 0.91% RSC Advances 10 publications, 0.91%
Nanomaterials	Nanomaterials, 10, 0.91% Nanomaterials 10 publications, 0.91%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 10, 0.91% Journal of Materials Chemistry A 10 publications, 0.91%
ACS Applied Nano Materials	ACS Applied Nano Materials, 9, 0.82% ACS Applied Nano Materials 9 publications, 0.82%
Journal Physics D: Applied Physics	Journal Physics D: Applied Physics, 9, 0.82% Journal Physics D: Applied Physics 9 publications, 0.82%
Physical Review Letters	Physical Review Letters, 8, 0.73% Physical Review Letters 8 publications, 0.73%
npj 2D Materials and Applications	npj 2D Materials and Applications, 8, 0.73% npj 2D Materials and Applications 8 publications, 0.73%
Chemical Reviews	Chemical Reviews, 7, 0.64% Chemical Reviews 7 publications, 0.64%
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Citations by publishers

	50 100 150 200 250 300
American Chemical Society (ACS)	American Chemical Society (ACS), 277, 25.34% American Chemical Society (ACS) 277 publications, 25.34%
Elsevier	Elsevier, 167, 15.28% Elsevier 167 publications, 15.28%
Wiley	Wiley, 129, 11.8% Wiley 129 publications, 11.8%
Springer Nature	Springer Nature, 109, 9.97% Springer Nature 109 publications, 9.97%
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IOP Publishing	IOP Publishing, 83, 7.59% IOP Publishing 83 publications, 7.59%
American Physical Society (APS)	American Physical Society (APS), 63, 5.76% American Physical Society (APS) 63 publications, 5.76%
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Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 27, 2.47% Multidisciplinary Digital Publishing Institute (MDPI) 27 publications, 2.47%
IEEE	IEEE, 10, 0.91% IEEE 10 publications, 0.91%
Optical Society of America	Optical Society of America, 8, 0.73% Optical Society of America 8 publications, 0.73%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 7, 0.64% American Association for the Advancement of Science (AAAS) 7 publications, 0.64%
Cambridge University Press	Cambridge University Press, 5, 0.46% Cambridge University Press 5 publications, 0.46%
Walter de Gruyter	Walter de Gruyter, 4, 0.37% Walter de Gruyter 4 publications, 0.37%
The Electrochemical Society	The Electrochemical Society, 3, 0.27% The Electrochemical Society 3 publications, 0.27%
Taylor & Francis	Taylor & Francis, 3, 0.27% Taylor & Francis 3 publications, 0.27%
Oxford University Press	Oxford University Press, 3, 0.27% Oxford University Press 3 publications, 0.27%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 3, 0.27% Proceedings of the National Academy of Sciences (PNAS) 3 publications, 0.27%
Higher Education Press	Higher Education Press, 2, 0.18% Higher Education Press 2 publications, 0.18%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 2, 0.18% Taiwan Institute of Chemical Engineers 2 publications, 0.18%
SAGE	SAGE, 1, 0.09% SAGE 1 publication, 0.09%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.09% Frontiers Media S.A. 1 publication, 0.09%
Korean Ceramic Society	Korean Ceramic Society, 1, 0.09% Korean Ceramic Society 1 publication, 0.09%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.09% Nonferrous Metals Society of China 1 publication, 0.09%
The Korean Society of Precision Engineering	The Korean Society of Precision Engineering, 1, 0.09% The Korean Society of Precision Engineering 1 publication, 0.09%
Science in China Press	Science in China Press, 1, 0.09% Science in China Press 1 publication, 0.09%
Materials Research Society	Materials Research Society, 1, 0.09% Materials Research Society 1 publication, 0.09%
Japan Society of Applied Physics	Japan Society of Applied Physics, 1, 0.09% Japan Society of Applied Physics 1 publication, 0.09%
Hindawi Limited	Hindawi Limited, 1, 0.09% Hindawi Limited 1 publication, 0.09%
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Hong J. et al. Exploring atomic defects in molybdenum disulphide monolayers // Nature Communications. 2015. Vol. 6. No. 1. 6293

GOST all authors (up to 50) Copy

Hong J., Hu Z., Probert M., Li K., Lv D., YANG X., Gu L., Mao N., Feng Q., Xie L., Zhang J., Wu D., Zhang Z., Jin C., Ji W., Zhang X., Yuan J., Zhang Z. Exploring atomic defects in molybdenum disulphide monolayers // Nature Communications. 2015. Vol. 6. No. 1. 6293

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1038/ncomms7293

UR - https://doi.org/10.1038%2Fncomms7293

TI - Exploring atomic defects in molybdenum disulphide monolayers

T2 - Nature Communications

AU - Hong, Jinhua

AU - Hu, Zhixin

AU - Probert, Matt

AU - Li, Kun

AU - Lv, Danhui

AU - YANG, XINAN

AU - Gu, Lin

AU - Mao, Nannan

AU - Feng, Qingliang

AU - Xie, Liming

AU - Zhang, Jin

AU - Wu, Dianzhong

AU - Zhang, Zhiyong

AU - Jin, Chuanhong

AU - Ji, Wei

AU - Zhang, Xixiang

AU - Yuan, Jun

AU - Zhang, Ze

PY - 2015

DA - 2015/02/19 00:00:00

PB - Springer Nature

IS - 1

VL - 6

PMID - 25695374

SN - 2041-1723

ER -

BibTex

Cite this

BibTex Copy

@article{2015_Hong,

author = {Jinhua Hong and Zhixin Hu and Matt Probert and Kun Li and Danhui Lv and XINAN YANG and Lin Gu and Nannan Mao and Qingliang Feng and Liming Xie and Jin Zhang and Dianzhong Wu and Zhiyong Zhang and Chuanhong Jin and Wei Ji and Xixiang Zhang and Jun Yuan and Ze Zhang},

title = {Exploring atomic defects in molybdenum disulphide monolayers},

journal = {Nature Communications},

year = {2015},

volume = {6},

publisher = {Springer Nature},

month = {feb},

url = {https://doi.org/10.1038%2Fncomms7293},

number = {1},

doi = {10.1038/ncomms7293}

}

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Springer Nature

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Nature Communications

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20411723 (Print)