Nature Energy, volume 1, issue 4, publication number 16030

High-power all-solid-state batteries using sulfide superionic conductors

Yuki Kato ^{1, 2, 3}

Satoshi Hori ²

Toshiya Saito ¹

Kota Suzuki ²

Masaaki Hirayama ²

Akio Mitsui ⁴

Masao Yonemura ⁵

Hideki Iba ¹

Ryoji Kanno ²

Hide authors affiliations Show authors affiliations: 5 affiliations

Battery Research Division, Higashifuji Technical Center, Toyota Motor Corporation, 1200 Mishuku, Susono, Shizuoka 410-1193, Japan |

Department of Electronic Chemistry, Interdisciplinary Graduate School of Science and Engineering, Tokyo Institute of Technology, 4259 Nagatsuta, Midori, Yokohama 226-8502, Japan |

Battery AT, Advanced Technology 1, Toyota Motor Europe NV/SA, Hoge Wei 33A B-1930, Zaventem, Belgium |

⁴

Material analysis Department, Material Engineering Division, Toyota Motor Corporation, 1 Toyota-cho, Toyota, Aichi 471-8572, Japan |

⁵

Institute of Materials Structure Science (IMSS), High Energy Accelerator Research Organization (KEK), Shirakata, Tokai, Ibaraki 319-1106, Japan |

Publication type: Journal Article

Publication date: 2016-03-21

Springer Nature

Journal: Nature Energy

Quartile SCImago

Quartile WOS

Impact factor: 56.7

ISSN: 20587546

DOI: 10.1038/nenergy.2016.30

Copy DOI

Electronic, Optical and Magnetic Materials

Energy Engineering and Power Technology

Fuel Technology

Renewable Energy, Sustainability and the Environment

Abstract

Compared with lithium-ion batteries with liquid electrolytes, all-solid-state batteries offer an attractive option owing to their potential in improving the safety and achieving both high power and high energy densities. Despite extensive research efforts, the development of all-solid-state batteries still falls short of expectation largely because of the lack of suitable candidate materials for the electrolyte required for practical applications. Here we report lithium superionic conductors with an exceptionally high conductivity (25 mS cm−1 for Li9.54Si1.74P1.44S11.7Cl0.3), as well as high stability ( ∼0 V versus Li metal for Li9.6P3S12). A fabricated all-solid-state cell based on this lithium conductor is found to have very small internal resistance, especially at 100 ∘C. The cell possesses high specific power that is superior to that of conventional cells with liquid electrolytes. Stable cycling with a high current density of 18 C (charging/discharging in just three minutes; where C is the C-rate) is also demonstrated. The development of all-solid-state batteries requires fast lithium conductors. Here, the authors report a lithium compound, Li9.54Si1.74P1.44S11.7Cl0.3, with an exceptionally high conductivity and demonstrate that all-solid-state batteries based on the compound have high power densities.

By date By citations

Top-30

Citations by journals

	20 40 60 80 100 120 140
ACS applied materials & interfaces	ACS applied materials & interfaces, 133, 5.22% ACS applied materials & interfaces 133 publications, 5.22%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 124, 4.86% Journal of Materials Chemistry A 124 publications, 4.86%
Advanced Energy Materials	Advanced Energy Materials, 117, 4.59% Advanced Energy Materials 117 publications, 4.59%
Journal of Power Sources	Journal of Power Sources, 109, 4.28% Journal of Power Sources 109 publications, 4.28%
Chemistry of Materials	Chemistry of Materials, 105, 4.12% Chemistry of Materials 105 publications, 4.12%
Energy Storage Materials	Energy Storage Materials, 90, 3.53% Energy Storage Materials 90 publications, 3.53%
ACS Applied Energy Materials	ACS Applied Energy Materials, 60, 2.35% ACS Applied Energy Materials 60 publications, 2.35%
Advanced Functional Materials	Advanced Functional Materials, 58, 2.28% Advanced Functional Materials 58 publications, 2.28%
ACS Energy Letters	ACS Energy Letters, 54, 2.12% ACS Energy Letters 54 publications, 2.12%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 48, 1.88% Journal of the Electrochemical Society 48 publications, 1.88%
Solid State Ionics	Solid State Ionics, 46, 1.8% Solid State Ionics 46 publications, 1.8%
Advanced Materials	Advanced Materials, 42, 1.65% Advanced Materials 42 publications, 1.65%
Chemical Engineering Journal	Chemical Engineering Journal, 38, 1.49% Chemical Engineering Journal 38 publications, 1.49%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 38, 1.49% Journal of Physical Chemistry C 38 publications, 1.49%
Energy and Environmental Science	Energy and Environmental Science, 35, 1.37% Energy and Environmental Science 35 publications, 1.37%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 34, 1.33% Angewandte Chemie - International Edition 34 publications, 1.33%
Electrochimica Acta	Electrochimica Acta, 34, 1.33% Electrochimica Acta 34 publications, 1.33%
Angewandte Chemie	Angewandte Chemie, 34, 1.33% Angewandte Chemie 34 publications, 1.33%
Nano Energy	Nano Energy, 32, 1.26% Nano Energy 32 publications, 1.26%
Small	Small, 29, 1.14% Small 29 publications, 1.14%
Nano Letters	Nano Letters, 28, 1.1% Nano Letters 28 publications, 1.1%
Nature Communications	Nature Communications, 26, 1.02% Nature Communications 26 publications, 1.02%
Journal of the American Chemical Society	Journal of the American Chemical Society, 24, 0.94% Journal of the American Chemical Society 24 publications, 0.94%
Electrochemistry	Electrochemistry, 24, 0.94% Electrochemistry 24 publications, 0.94%
Batteries & Supercaps	Batteries & Supercaps, 21, 0.82% Batteries & Supercaps 21 publications, 0.82%
Journal of Energy Chemistry	Journal of Energy Chemistry, 20, 0.78% Journal of Energy Chemistry 20 publications, 0.78%
Joule	Joule, 19, 0.75% Joule 19 publications, 0.75%
Ceramics International	Ceramics International, 19, 0.75% Ceramics International 19 publications, 0.75%
Journal of Energy Storage	Journal of Energy Storage, 18, 0.71% Journal of Energy Storage 18 publications, 0.71%
	20 40 60 80 100 120 140

Citations by publishers

	100 200 300 400 500 600 700
Elsevier	Elsevier, 660, 25.89% Elsevier 660 publications, 25.89%
American Chemical Society (ACS)	American Chemical Society (ACS), 532, 20.87% American Chemical Society (ACS) 532 publications, 20.87%
Wiley	Wiley, 514, 20.16% Wiley 514 publications, 20.16%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 270, 10.59% Royal Society of Chemistry (RSC) 270 publications, 10.59%
Springer Nature	Springer Nature, 180, 7.06% Springer Nature 180 publications, 7.06%
The Electrochemical Society	The Electrochemical Society, 50, 1.96% The Electrochemical Society 50 publications, 1.96%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 48, 1.88% Multidisciplinary Digital Publishing Institute (MDPI) 48 publications, 1.88%
IOP Publishing	IOP Publishing, 30, 1.18% IOP Publishing 30 publications, 1.18%
The Electrochemical Society of Japan	The Electrochemical Society of Japan, 24, 0.94% The Electrochemical Society of Japan 24 publications, 0.94%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 20, 0.78% American Institute of Physics (AIP) 20 publications, 0.78%
Frontiers Media S.A.	Frontiers Media S.A., 18, 0.71% Frontiers Media S.A. 18 publications, 0.71%
Ceramic Society of Japan	Ceramic Society of Japan, 17, 0.67% Ceramic Society of Japan 17 publications, 0.67%
Cambridge University Press	Cambridge University Press, 14, 0.55% Cambridge University Press 14 publications, 0.55%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 12, 0.47% American Association for the Advancement of Science (AAAS) 12 publications, 0.47%
American Physical Society (APS)	American Physical Society (APS), 11, 0.43% American Physical Society (APS) 11 publications, 0.43%
Japan Institute of Metals and Materials	Japan Institute of Metals and Materials, 11, 0.43% Japan Institute of Metals and Materials 11 publications, 0.43%
The Chemical Society of Japan	The Chemical Society of Japan, 9, 0.35% The Chemical Society of Japan 9 publications, 0.35%
Japan Society of Applied Physics	Japan Society of Applied Physics, 8, 0.31% Japan Society of Applied Physics 8 publications, 0.31%
Chinese Physical Society	Chinese Physical Society, 7, 0.27% Chinese Physical Society 7 publications, 0.27%
Oxford University Press	Oxford University Press, 6, 0.24% Oxford University Press 6 publications, 0.24%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 5, 0.2% Korean Society of Industrial Engineering Chemistry 5 publications, 0.2%
Taylor & Francis	Taylor & Francis, 4, 0.16% Taylor & Francis 4 publications, 0.16%
IEEE	IEEE, 4, 0.16% IEEE 4 publications, 0.16%
Pleiades Publishing	Pleiades Publishing, 3, 0.12% Pleiades Publishing 3 publications, 0.12%
ASME	ASME, 3, 0.12% ASME 3 publications, 0.12%
World Scientific	World Scientific, 3, 0.12% World Scientific 3 publications, 0.12%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 3, 0.12% Nonferrous Metals Society of China 3 publications, 0.12%
Chinese Ceramic Society	Chinese Ceramic Society, 3, 0.12% Chinese Ceramic Society 3 publications, 0.12%
Proceedings of the National Academy of Sciences (PNAS)	Proceedings of the National Academy of Sciences (PNAS), 3, 0.12% Proceedings of the National Academy of Sciences (PNAS) 3 publications, 0.12%
	100 200 300 400 500 600 700

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Kato Y. et al. High-power all-solid-state batteries using sulfide superionic conductors // Nature Energy. 2016. Vol. 1. No. 4. 16030

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Kato Y., Hori S., Saito T., Suzuki K., Hirayama M., Mitsui A., Yonemura M., Iba H., Kanno R. High-power all-solid-state batteries using sulfide superionic conductors // Nature Energy. 2016. Vol. 1. No. 4. 16030

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RIS Copy

TY - JOUR

DO - 10.1038/nenergy.2016.30

UR - https://doi.org/10.1038/nenergy.2016.30

TI - High-power all-solid-state batteries using sulfide superionic conductors

T2 - Nature Energy

AU - Kato, Yuki

AU - Hori, Satoshi

AU - Saito, Toshiya

AU - Suzuki, Kota

AU - Hirayama, Masaaki

AU - Mitsui, Akio

AU - Yonemura, Masao

AU - Iba, Hideki

AU - Kanno, Ryoji

PY - 2016

DA - 2016/03/21 00:00:00

PB - Springer Nature

IS - 4

VL - 1

SN - 2058-7546

ER -

BibTex

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BibTex Copy

@article{2016_Kato,

author = {Yuki Kato and Satoshi Hori and Toshiya Saito and Kota Suzuki and Masaaki Hirayama and Akio Mitsui and Masao Yonemura and Hideki Iba and Ryoji Kanno},

title = {High-power all-solid-state batteries using sulfide superionic conductors},

journal = {Nature Energy},

year = {2016},

volume = {1},

publisher = {Springer Nature},

month = {mar},

url = {https://doi.org/10.1038/nenergy.2016.30},

number = {4},

doi = {10.1038/nenergy.2016.30}

}

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Publisher

Springer Nature

Journal

Nature Energy

Quartile SCImago

Quartile WOS

Impact factor

56.7

ISSN

20587546 (Electronic)